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RU2008135571A - METHOD FOR PRODUCING N1, N1, N4, N4-TETRAMETHYL-2-BUTEN-1,4-DIAMINE - Google Patents

METHOD FOR PRODUCING N1, N1, N4, N4-TETRAMETHYL-2-BUTEN-1,4-DIAMINE Download PDF

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RU2008135571A
RU2008135571A RU2008135571/04A RU2008135571A RU2008135571A RU 2008135571 A RU2008135571 A RU 2008135571A RU 2008135571/04 A RU2008135571/04 A RU 2008135571/04A RU 2008135571 A RU2008135571 A RU 2008135571A RU 2008135571 A RU2008135571 A RU 2008135571A
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Russia
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bisamine
diamine
tetramethyl
acac
hours
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RU2008135571/04A
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Russian (ru)
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RU2440329C2 (en
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Усеин Меметович Джемилев (RU)
Усеин Меметович Джемилев
Мария Геннадьевна Шайбакова (RU)
Мария Геннадьевна Шайбакова
Гилемдар Адыхамович Махмудияров (RU)
Гилемдар Адыхамович Махмудияров
Асхат Габдрахманович Ибрагимов (RU)
Асхат Габдрахманович Ибрагимов
Ирина Геннадьевна Титова (RU)
Ирина Геннадьевна Титова
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Институт нефтехимии и катализа РАН (RU)
Институт нефтехимии и катализа РАН
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Priority to RU2008135571/04A priority Critical patent/RU2440329C2/en
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Abstract

Способ получения N1,N1,N4,N4-тетраметил-2-бутен-1,4-диамина общей формулы (1): ! ! характеризующийся тем, что Nl,Nl,N4,N4-тeтpaмeтил-2-бутин-1,4-диамин (бисамин) подвергают взаимодействию с 3-кратным избытком газообразного ацетилена в присутствии катализатора ацетилацетоната ванадила (VO(acac)2), взятыми в мольном соотношении бисамин: VO(acac)2=10:(0.3-0.5) при температуре 70°С и атмосферном давлении в течение 3 ч, с последующим добавлением диизобутилалюминийгидрида (i-Bu2AlH) в трехкратном по отношению к бисамину избытке и перемешиванием реакционной массы в течение 4-6 ч при комнатной температуре (20-22°С).The method of obtaining N1, N1, N4, N4-tetramethyl-2-butene-1,4-diamine of the general formula (1):! ! characterized in that Nl, Nl, N4, N4-tetramethyl-2-butyn-1,4-diamine (bisamine) are reacted with a 3-fold excess of gaseous acetylene in the presence of a vanadyl acetylacetonate catalyst (VO (acac) 2) taken in the molar ratio of bisamine: VO (acac) 2 = 10: (0.3-0.5) at a temperature of 70 ° C and atmospheric pressure for 3 hours, followed by the addition of diisobutylaluminum hydride (i-Bu2AlH) in excess of bisamine three times with stirring of the reaction mass for 4-6 hours at room temperature (20-22 ° C).

Claims (1)

Способ получения N1,N1,N4,N4-тетраметил-2-бутен-1,4-диамина общей формулы (1):The method of obtaining N 1 , N 1 , N 4 , N 4- tetramethyl-2-butene-1,4-diamine of the general formula (1):
Figure 00000001
Figure 00000001
характеризующийся тем, что Nl,Nl,N4,N4-тeтpaмeтил-2-бутин-1,4-диамин (бисамин) подвергают взаимодействию с 3-кратным избытком газообразного ацетилена в присутствии катализатора ацетилацетоната ванадила (VO(acac)2), взятыми в мольном соотношении бисамин: VO(acac)2=10:(0.3-0.5) при температуре 70°С и атмосферном давлении в течение 3 ч, с последующим добавлением диизобутилалюминийгидрида (i-Bu2AlH) в трехкратном по отношению к бисамину избытке и перемешиванием реакционной массы в течение 4-6 ч при комнатной температуре (20-22°С). characterized in that N l , N l , N 4 , N 4 -tetmethyl-2-butyn-1,4-diamine (bisamine) is reacted with a 3-fold excess of gaseous acetylene in the presence of a vanadyl acetylacetonate catalyst (VO (acac) 2 ) taken in a molar ratio of bisamine: VO (acac) 2 = 10: (0.3-0.5) at a temperature of 70 ° C and atmospheric pressure for 3 hours, followed by the addition of diisobutylaluminum hydride (i-Bu 2 AlH) in triplicate with respect to bisamine excess and stirring the reaction mass for 4-6 hours at room temperature (20-22 ° C).
RU2008135571/04A 2008-09-02 2008-09-02 Method of producing n1,n1,n4,n4-tetramethyl-2-butene-1,4-diamine RU2440329C2 (en)

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RU2008135571/04A RU2440329C2 (en) 2008-09-02 2008-09-02 Method of producing n1,n1,n4,n4-tetramethyl-2-butene-1,4-diamine

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RU2008135571/04A RU2440329C2 (en) 2008-09-02 2008-09-02 Method of producing n1,n1,n4,n4-tetramethyl-2-butene-1,4-diamine

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RU2408572C2 (en) * 2008-08-05 2011-01-10 Учреждение Российской Академии Наук Институт Нефтехимии И Катализа Ран Method of producing n1,n1,n4,n4-tetramethyl-2-butyne-1,4-diamine

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Effective date: 20111112