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DE1029952B - Process for the production of magnetizable ferrite cores - Google Patents

Process for the production of magnetizable ferrite cores

Info

Publication number
DE1029952B
DE1029952B DES32842A DES0032842A DE1029952B DE 1029952 B DE1029952 B DE 1029952B DE S32842 A DES32842 A DE S32842A DE S0032842 A DES0032842 A DE S0032842A DE 1029952 B DE1029952 B DE 1029952B
Authority
DE
Germany
Prior art keywords
production
sintering
permeability
ferrite
cores
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Pending
Application number
DES32842A
Other languages
German (de)
Inventor
Dipl-Ing Josef Brackmann
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Siemens Corp
Original Assignee
Siemens Corp
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Siemens Corp filed Critical Siemens Corp
Priority to DES32842A priority Critical patent/DE1029952B/en
Publication of DE1029952B publication Critical patent/DE1029952B/en
Pending legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C04CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
    • C04BLIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
    • C04B35/00Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products
    • C04B35/01Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products based on oxide ceramics
    • C04B35/26Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products based on oxide ceramics based on ferrites
    • C04B35/2608Compositions containing one or more ferrites of the group comprising manganese, zinc, nickel, copper or cobalt and one or more ferrites of the group comprising rare earth metals, alkali metals, alkaline earth metals or lead
    • C04B35/2633Compositions containing one or more ferrites of the group comprising manganese, zinc, nickel, copper or cobalt and one or more ferrites of the group comprising rare earth metals, alkali metals, alkaline earth metals or lead containing barium, strontium or calcium
    • CCHEMISTRY; METALLURGY
    • C04CEMENTS; CONCRETE; ARTIFICIAL STONE; CERAMICS; REFRACTORIES
    • C04BLIME, MAGNESIA; SLAG; CEMENTS; COMPOSITIONS THEREOF, e.g. MORTARS, CONCRETE OR LIKE BUILDING MATERIALS; ARTIFICIAL STONE; CERAMICS; REFRACTORIES; TREATMENT OF NATURAL STONE
    • C04B35/00Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products
    • C04B35/01Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products based on oxide ceramics
    • C04B35/26Shaped ceramic products characterised by their composition; Ceramics compositions; Processing powders of inorganic compounds preparatory to the manufacturing of ceramic products based on oxide ceramics based on ferrites

Landscapes

  • Engineering & Computer Science (AREA)
  • Chemical & Material Sciences (AREA)
  • Ceramic Engineering (AREA)
  • Manufacturing & Machinery (AREA)
  • Materials Engineering (AREA)
  • Structural Engineering (AREA)
  • Organic Chemistry (AREA)
  • Soft Magnetic Materials (AREA)
  • Magnetic Ceramics (AREA)

Description

Verfahren zur Herstellung von magnetisierbaren Kernen aus Ferrit In manchen Anwendungsfällen ist es zweckmäßig, den Verlauf der Permeabilität eines Ferrithochfrequenzkörpers über der Temperatur zu beeinflussen, um in Filter- und Schwingkreisen od. dgl. gegebenenfalls eine Kompensation der Temperaturkoeffizienten anderer Schaltelemente vornehmen zu können.Process for the production of magnetizable cores from ferrite In In some applications it is useful to track the permeability of a Ferrite high-frequency body to influence the temperature in order to be used in filter and Oscillating circuits or the like, if necessary a compensation of the temperature coefficients to be able to make other switching elements.

Trägt man einmal die Permeabilitätskurve eines Ferritkernes über der Temperatur auf, dann ergibt sich eine Kurve, wie sie im Schaubild mit I bezeichnet ist. Von tieferen Temperaturen her steigt diese Kurve an bis zu einem Maximalwert, nach welchem sie plötzlich auf Null abfällt. Diese Temperatur, bei welcher die Permeabilität auf Null abfällt, ist der sogenannte Curiepunkt. Man bleibt mit der Gebrauchstemperatur eines solchen Kernwerkstoffes mit einem gewissen Sicherheitsabstand möglichst in der Nähe des Maximums, um höchste Permeabilitäten zu erzielen. Da die Kurve in dieser Gegend, durch den schraffiert dargestellten Bereich angedeutet, verhältnismäßig steil ansteigt, bedeutet dies, daß der Temperaturkoeffizient der Permeabilität in dieser Gegend sehr groß und positiv ist.If you take the permeability curve of a ferrite core over the If the temperature rises, a curve like the one indicated by I in the diagram results is. This curve rises from lower temperatures up to a maximum value, after which it suddenly drops to zero. This temperature at which the permeability drops to zero, is the so-called Curie point. You stay with the use temperature of such a core material with a certain safety margin if possible in close to the maximum in order to achieve the highest permeabilities. Because the curve in this Area, indicated by the hatched area, relatively rises steeply, it means that the temperature coefficient of permeability in this area is very big and positive.

Es wurde nun festgestellt, daß die Permeabilität, insbesondere das Permeabilitätsmaximum, sehr stark von der Größe der Kristalle des Werkstoffes abhängt. Da bislang nur höchste Permeabilitäten wichtig erschienen, hat man sich bemüht, den gesinterten Werkstoff so herzustellen, daß er möglichst wenige und dafür große Kristalle enthält. Aus den gleichen Ausgangssubstanzen hergestellte Kerne zeigen aber auch, wenn ihre Kristallbildung durch irgendeinen Einfluß verändert ist, wesentlich veränderte Permeabilitätswerte. Bildet man beispielsweise den gleichen Kernwerkstoff in kleinen Kristallen aus, dann ergibt sich ein Permeabilitätsverlauf, wie er im Schaubild mit der Kurve II wiedergegeben ist. Die Permeabilität ist abgefallen, jedoch, und das ist das Entscheidende für die Erfindung, ist im Gebrauchstemperaturintervall der Verlauf der Kurve ein wesentlich anderer, so daß sich also ein anderer TK-Wert ergeben muß. Durch entsprechende Beeinflussung der Kristallgröße ist es also möglich, jede beliebige Steilheit der Permeabilitätskurve zu erzwingen und damit den gewünschten TK-Wert für die Permeabilität zu erhalten.It has now been found that the permeability, especially that Maximum permeability, very much depends on the size of the crystals of the material. Since only the highest permeabilities appeared to be important up to now, efforts have been made to to produce the sintered material in such a way that it has as few and large as possible Contains crystals. Show cores made from the same starting substances but also if their crystal formation is altered by any influence, it is essential changed permeability values. For example, if the same core material is formed in small crystals, then the result is a permeability curve like the one in Diagram with curve II is reproduced. The permeability has dropped however, and this is the decisive factor for the invention, is in the use temperature range the course of the curve is significantly different, so that there is a different TK value must result. By influencing the crystal size accordingly, it is possible to to enforce any slope of the permeability curve and thus the desired one Get TK value for permeability.

Um magnetisierbare Kerne aus Ferrit mit kleinem Temperaturkoeffizienten der Permeabilität im Gebiet des Gebrauchstemperaturintervalls herzustellen, werden daher erfindungsgemäß reinste Ausgangsstoffe zur Herstellung der Ferritkerne verwendet, diese Ausgangsstoffe werden durch Mahlen oder Ätzen zu feinteiligem Pulver verarbeitet, und diesem Pulver wird - um bei der folgenden Sinterung die rasche Ausbildung großer Kristallite zu verhindern - Kobalt-Oxyd und/oder Bariumoxyd und/oder Kupferoxyd und/oder Kieselsäure und/oder Calziumfluorid, in Mengen zwischen 0,1 und 20/00 des Gesamtgewichtes zugegeben, dieses Gemisch wird gesintert und die Sinterung wird abgebrochen, bevor die sich bei der Sinterung bildenden Kristallite eine Größe von etwa 20 g erreicht haben.Around magnetizable cores made of ferrite with a small temperature coefficient to establish the permeability in the area of the use temperature interval therefore, according to the invention, the purest starting materials are used to manufacture the ferrite cores, these raw materials are processed into finely divided powder by grinding or etching, and this powder is - in order for the following sintering - the rapid formation greater To prevent crystallites - cobalt oxide and / or barium oxide and / or copper oxide and / or silica and / or calcium fluoride, in amounts between 0.1 and 20/00 des Total weight added, this mixture is sintered and the sintering is carried out aborted before the crystallites formed during sintering have a size of have reached about 20 g.

Die Zugabe von. Oxyden in kleiner Menge zu Ausgangsstoffen zur Ferritherstellung ist an sich bekannt. Es ist auch bekannt, daß diese Zuschläge einen Einfluß auf die Temperaturabhängigkeit der Permeabilität der Ferrite ausüben.The addition of. Oxides in small quantities to raw materials for ferrite production is known per se. It is also known that these surcharges have an impact exercise the temperature dependence of the permeability of ferrites.

Der im Rahmen der Erfindung beabsichtigte Einfluß, nämlich die Verminderung der Temperaturabhängigkeit der Permeabilität, macht sich bei Anwendung des erfindungsgemäßen Verfahrens nun nur dann bemerkbar, wenn 1. die beanspruchten Zuschlagstoffe (vielleicht neben einigen anderen) verwendet werden und wenn 2. die Sinterung abgebrochen wird, bevor die sich bei der Sinterung bildenden Kristallite eine Größe von 20 #t erreicht haben.The influence intended in the context of the invention, namely the reduction the temperature dependence of the permeability, makes itself when using the invention Process only noticeable if 1. the aggregates claimed (perhaps among some others) and if 2. the sintering is canceled, before the crystallites formed during sintering reach a size of 20 #t to have.

Die beanspruchten Zuschlagstoffe sind im übrigen in ihrer Wirkung untereinander nicht völlig gleichartig. Vielmehr wirken sie entweder kristallhemmend oder als Kristallkeime. Jedenfalls bewirken sie, daß bei der Sinterung der Zustand, bei dem verhältnismäßig kleine Kristallite vorliegen, verhältnismäßig lange währt. Es ist daher verfahrenstechnisch einfach, innerhalb dieses Zeitraumes die Sinterung abzubrechen.The aggregates claimed are otherwise in their effect not completely identical to one another. Rather, they either have a crystal-inhibiting effect or as crystal seeds. In any case, they have the effect that during sintering the state in which there are relatively small crystallites, lasts for a relatively long time. From a procedural point of view, it is therefore easy to sinter within this period of time cancel.

Um wiederholbar eine immer gleiche Kristallgröße im Sinterprodukt zu erzwingen, ist es vorteilhaft, den Ausgangssubstanzen genau dosierte Mengen der genannten Zuschlagstoffe zuzusetzen.To ensure that the crystal size is always the same in the sintered product to enforce, it is beneficial to use the Precisely dosed starting substances Add quantities of the specified additives.

Claims (1)

PATENTANSPRUCH: Verfahren zur Herstellung von magnetisierbaren Kernen aus Ferrit mit kleinem Temperaturkoeffizienten der Permeabilität im Gebiet des Gebrauchstemperaturintervalls, dadurch gekennzeichnet, daß reinste Ausgangsstoffe zur Herstellung der Ferritkerne verwendet werden, daß diese Ausgangsstoffe durch Mahlen und/oder Ätzen zu feinteiligem Pulver verarbeitet werden, daß diesem Pulver - um bei der folgenden Sinterung die rasche Ausbildung großer Kristallite zu verhindern - Kobaltoxyd und/oder Bariumoxyd und/oder Kupferoxyd und/oder Kieselsäure und/ oder Calziumfluorid zugegeben wird, und zwar in Mengen zwischen 0,1 und 20/00 des Gesamtgewichtes, daß dieses Gemisch gesintert wird und daß die Sinterung abgebrochen wird, bevor die sich bei der Sinterung bildenden Kristallite eine Größe von etwa 20 g erreicht haben. In Betracht gezogene Druckschriften: Schweizerische Patentschrift Nr. 260 717; Buch »New Developments in Ferromagnetic Materials« von S. L. Snoek, Elsevier Publishing Comp., Inc., New York, 1949, S. 77 bis 91.PATENT CLAIM: Process for the production of magnetizable cores from ferrite with a small temperature coefficient of permeability in the area of the service temperature range, characterized in that the purest starting materials are used for the production of the ferrite cores, that these starting materials are processed into finely divided powder by grinding and / or etching, that this Powder - in order to prevent the rapid formation of large crystallites during the subsequent sintering - cobalt oxide and / or barium oxide and / or copper oxide and / or silica and / or calcium fluoride is added in amounts between 0.1 and 20/00 of the total weight, that this mixture is sintered and that the sintering is terminated before the crystallites formed during the sintering have reached a size of about 20 g. Documents considered: Swiss Patent No. 260 717; Book "New Developments in Ferromagnetic Materials" by SL Snoek, Elsevier Publishing Comp., Inc., New York, 1949, pp. 77 to 91.
DES32842A 1953-03-28 1953-03-28 Process for the production of magnetizable ferrite cores Pending DE1029952B (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
DES32842A DE1029952B (en) 1953-03-28 1953-03-28 Process for the production of magnetizable ferrite cores

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
DES32842A DE1029952B (en) 1953-03-28 1953-03-28 Process for the production of magnetizable ferrite cores

Publications (1)

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DE1029952B true DE1029952B (en) 1958-05-14

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Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE1209036B (en) * 1962-08-10 1966-01-13 Siemens Ag Low-loss ferromagnetic manganese-zinc ferrite and process for its production

Citations (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CH260717A (en) * 1943-05-31 1949-03-31 Philips Nv A method of manufacturing a magnetic core, and a magnetic core manufactured by this method.

Patent Citations (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CH260717A (en) * 1943-05-31 1949-03-31 Philips Nv A method of manufacturing a magnetic core, and a magnetic core manufactured by this method.

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE1209036B (en) * 1962-08-10 1966-01-13 Siemens Ag Low-loss ferromagnetic manganese-zinc ferrite and process for its production

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