[go: up one dir, main page]

WO2008133177A1 - 高分子電解質材料及びこれを用いた燃料電池用膜・電極接合体 - Google Patents

高分子電解質材料及びこれを用いた燃料電池用膜・電極接合体 Download PDF

Info

Publication number
WO2008133177A1
WO2008133177A1 PCT/JP2008/057509 JP2008057509W WO2008133177A1 WO 2008133177 A1 WO2008133177 A1 WO 2008133177A1 JP 2008057509 W JP2008057509 W JP 2008057509W WO 2008133177 A1 WO2008133177 A1 WO 2008133177A1
Authority
WO
WIPO (PCT)
Prior art keywords
polymer electrolyte
membrane
electrolyte material
electrode assembly
fuel cell
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Ceased
Application number
PCT/JP2008/057509
Other languages
English (en)
French (fr)
Inventor
Tatsuo Fujinami
Tadao Kurokawa
Masayoshi Takami
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Shizuoka University NUC
Toyota Motor Corp
Original Assignee
Shizuoka University NUC
Toyota Motor Corp
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Shizuoka University NUC, Toyota Motor Corp filed Critical Shizuoka University NUC
Priority to US12/595,335 priority Critical patent/US20100151350A1/en
Priority to CA002683876A priority patent/CA2683876A1/en
Priority to EP08740579A priority patent/EP2148383A4/en
Priority to CN200880011904A priority patent/CN101689645A/zh
Publication of WO2008133177A1 publication Critical patent/WO2008133177A1/ja
Anticipated expiration legal-status Critical
Ceased legal-status Critical Current

Links

Classifications

    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01B—CABLES; CONDUCTORS; INSULATORS; SELECTION OF MATERIALS FOR THEIR CONDUCTIVE, INSULATING OR DIELECTRIC PROPERTIES
    • H01B1/00—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors
    • H01B1/06—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors mainly consisting of other non-metallic substances
    • H01B1/12—Conductors or conductive bodies characterised by the conductive materials; Selection of materials as conductors mainly consisting of other non-metallic substances organic substances
    • H01B1/122—Ionic conductors
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/90—Selection of catalytic material
    • H01M4/92—Metals of platinum group
    • H01M4/925—Metals of platinum group supported on carriers, e.g. powder carriers
    • H01M4/926—Metals of platinum group supported on carriers, e.g. powder carriers on carbon or graphite
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1004—Fuel cells with solid electrolytes characterised by membrane-electrode assemblies [MEA]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1027—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having carbon, oxygen and other atoms, e.g. sulfonated polyethersulfones [S-PES]
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/1016—Fuel cells with solid electrolytes characterised by the electrolyte material
    • H01M8/1018—Polymeric electrolyte materials
    • H01M8/102—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer
    • H01M8/1037—Polymeric electrolyte materials characterised by the chemical structure of the main chain of the ion-conducting polymer having silicon, e.g. sulfonated crosslinked polydimethylsiloxanes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M2300/00—Electrolytes
    • H01M2300/0017—Non-aqueous electrolytes
    • H01M2300/0065—Solid electrolytes
    • H01M2300/0082—Organic polymers
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H01M4/8803—Supports for the deposition of the catalytic active composition
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells

Landscapes

  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Electrochemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Manufacturing & Machinery (AREA)
  • Sustainable Energy (AREA)
  • Sustainable Development (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Materials Engineering (AREA)
  • Physics & Mathematics (AREA)
  • Spectroscopy & Molecular Physics (AREA)
  • Fuel Cell (AREA)
  • Inert Electrodes (AREA)
  • Conductive Materials (AREA)

Abstract

ガス透過性に優れると共に、炭化水素系高分子電解質と相互作用を生じ、高分子電解質膜－触媒層間の接合性を確保することが可能な高分子電解質材料及びこれを用いた燃料電池用膜・電極接合体を提供する。 主骨格を形成するＳｉ－Ｏ結合を含む第一の繰り返し単位と、芳香環及びプロトン伝導性基を含む第二の繰り返し単位とを、少なくとも有していることを特徴とする高分子電解質材料、並びに、該高分子電解質材料を含有する高分子電解質膜及び／又は触媒層を備えることを特徴とする、燃料電池用膜・電極接合体。
PCT/JP2008/057509 2007-04-18 2008-04-17 高分子電解質材料及びこれを用いた燃料電池用膜・電極接合体 Ceased WO2008133177A1 (ja)

Priority Applications (4)

Application Number Priority Date Filing Date Title
US12/595,335 US20100151350A1 (en) 2007-04-18 2008-04-17 Polymer electrolyte material and membrane electrode assembly for fuel cell using the same
CA002683876A CA2683876A1 (en) 2007-04-18 2008-04-17 Polymer electrolyte material and membrane electrode assembly for fuel cell using the same
EP08740579A EP2148383A4 (en) 2007-04-18 2008-04-17 POLYMER ELECTROLYTE MATERIAL AND MEMBRANE ELECTROLYTE ASSEMBLY FOR A FUEL CELL THEREFOR
CN200880011904A CN101689645A (zh) 2007-04-18 2008-04-17 高分子电解质材料以及使用该材料的燃料电池用膜电极接合体

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
JP2007-109848 2007-04-18
JP2007109848A JP2008269900A (ja) 2007-04-18 2007-04-18 高分子電解質材料及びこれを用いた燃料電池用膜・電極接合体

Publications (1)

Publication Number Publication Date
WO2008133177A1 true WO2008133177A1 (ja) 2008-11-06

Family

ID=39925633

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/JP2008/057509 Ceased WO2008133177A1 (ja) 2007-04-18 2008-04-17 高分子電解質材料及びこれを用いた燃料電池用膜・電極接合体

Country Status (6)

Country Link
US (1) US20100151350A1 (ja)
EP (1) EP2148383A4 (ja)
JP (1) JP2008269900A (ja)
CN (1) CN101689645A (ja)
CA (1) CA2683876A1 (ja)
WO (1) WO2008133177A1 (ja)

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2009118612A1 (en) * 2008-03-26 2009-10-01 Toyota Jidosha Kabushiki Kaisha Fuel cell electrolyte membrane

Families Citing this family (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US10516182B2 (en) * 2009-08-21 2019-12-24 Iucf-Hyu (Industry-University Cooperation Foundation Hanyang University) Polymer ion exchange membrane and method of preparing same
GB201309806D0 (en) * 2013-05-31 2013-07-17 Itm Power Research Ltd Catalysts and methods of depositing same
DE102020130578A1 (de) 2020-11-19 2022-05-19 Lacom Gmbh Verfahren zur Herstellung einer Membran-Elektroden-Anordnung sowie eine Membran-Elektroden-Anordnung für eine Brennstoffzelle

Citations (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPH1021943A (ja) * 1996-06-28 1998-01-23 Sumitomo Chem Co Ltd 燃料電池用高分子電解質及び燃料電池
JP2002309016A (ja) * 2001-04-13 2002-10-23 National Institute Of Advanced Industrial & Technology 可撓性に富んだプロトン伝導性膜、その製造方法及びそれを用いた燃料電池
JP2003277506A (ja) * 2001-11-15 2003-10-02 Korea Inst Of Chemical Technology 新規架橋剤とそれを含有する架橋型固体高分子電解質
JP2004346316A (ja) 2003-04-30 2004-12-09 Mitsubishi Chemicals Corp スルホン酸基含有シロキサン類、プロトン伝導材料およびそれを用いた燃料電池
JP2005190813A (ja) 2003-12-25 2005-07-14 Toyota Motor Corp 燃料電池電極用電解質材
JP2005276721A (ja) 2004-03-26 2005-10-06 Corona Corp 燃料電池及び電解質膜
JP2005350673A (ja) * 2004-06-07 2005-12-22 Korea Inst Of Chemical Technology ポリシロキサン系化合物及びそれを用いた固体高分子電解質組成物
JP2006134765A (ja) 2004-11-08 2006-05-25 Toyota Motor Corp 触媒電極層用電解質材料、それを用いた膜電極複合体、および固体高分子電解質型燃料電池
JP2006269414A (ja) * 2005-02-28 2006-10-05 Shin Etsu Chem Co Ltd 電解質膜用硬化性樹脂組成物、電解質膜の製造方法及び電解質膜・電極接合体の製造方法

Family Cites Families (11)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JP4043135B2 (ja) * 1999-03-29 2008-02-06 株式会社東芝 機能素子および多成分多相系高分子成形体
DE10163518A1 (de) * 2001-12-21 2003-07-10 Fraunhofer Ges Forschung Protonenleitfähige Membranen/Schichten und Verfahren zu deren Herstellung
DE10258175A1 (de) * 2002-12-12 2004-07-08 General Motors Corp., Detroit Ein Blockcopolymer zur Verwendung als fester Polymerelektrolyt, eine ionenleitfähige Membran, die aus einem Blockcopolymer gemacht ist, und Verfahren zur Herstellung eines Blockcopolymers
JP4769577B2 (ja) * 2003-04-25 2011-09-07 積水化学工業株式会社 プロトン伝導性膜、その製造方法およびそのプロトン伝導性膜を用いた燃料電池
CN100446312C (zh) * 2003-06-25 2008-12-24 东丽株式会社 高分子电解质、以及使用了该高分子电解质的高分子电解质膜、膜电极复合体和高分子电解质型燃料电池
US7208243B2 (en) * 2004-12-01 2007-04-24 Toyota Technical Center Usa, Inc. Proton exchange membranes using cycloaddition reaction between azide and alkyne containing components
US7459505B2 (en) * 2005-05-03 2008-12-02 General Motors Corporation Block copolymers with acidic groups
KR101193164B1 (ko) * 2006-02-21 2012-10-19 삼성에스디아이 주식회사 술폰산기 함유 유기 고분자 실록산 화합물 및 이를포함하는 연료전지
EP2009723A1 (en) * 2006-03-27 2008-12-31 Toyota Jidosha Kabushiki Kaisha Composite electrolyte membrane comprising imide network polymer crosslinked with strongly acidic group, method for manufacturing the composite electrolyte membrane, and fuel cell
US20100119908A1 (en) * 2007-03-02 2010-05-13 Sekisui Chemical Co., Ltd. Proton conducting membrane, membrane-electrode assembly, and polymer electrolyte fuel cell
US7897650B2 (en) * 2007-08-31 2011-03-01 Sayre Jay R Ionically conductive polymers for use in fuel cells

Patent Citations (9)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPH1021943A (ja) * 1996-06-28 1998-01-23 Sumitomo Chem Co Ltd 燃料電池用高分子電解質及び燃料電池
JP2002309016A (ja) * 2001-04-13 2002-10-23 National Institute Of Advanced Industrial & Technology 可撓性に富んだプロトン伝導性膜、その製造方法及びそれを用いた燃料電池
JP2003277506A (ja) * 2001-11-15 2003-10-02 Korea Inst Of Chemical Technology 新規架橋剤とそれを含有する架橋型固体高分子電解質
JP2004346316A (ja) 2003-04-30 2004-12-09 Mitsubishi Chemicals Corp スルホン酸基含有シロキサン類、プロトン伝導材料およびそれを用いた燃料電池
JP2005190813A (ja) 2003-12-25 2005-07-14 Toyota Motor Corp 燃料電池電極用電解質材
JP2005276721A (ja) 2004-03-26 2005-10-06 Corona Corp 燃料電池及び電解質膜
JP2005350673A (ja) * 2004-06-07 2005-12-22 Korea Inst Of Chemical Technology ポリシロキサン系化合物及びそれを用いた固体高分子電解質組成物
JP2006134765A (ja) 2004-11-08 2006-05-25 Toyota Motor Corp 触媒電極層用電解質材料、それを用いた膜電極複合体、および固体高分子電解質型燃料電池
JP2006269414A (ja) * 2005-02-28 2006-10-05 Shin Etsu Chem Co Ltd 電解質膜用硬化性樹脂組成物、電解質膜の製造方法及び電解質膜・電極接合体の製造方法

Non-Patent Citations (1)

* Cited by examiner, † Cited by third party
Title
See also references of EP2148383A4 *

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
WO2009118612A1 (en) * 2008-03-26 2009-10-01 Toyota Jidosha Kabushiki Kaisha Fuel cell electrolyte membrane

Also Published As

Publication number Publication date
EP2148383A4 (en) 2010-07-14
JP2008269900A (ja) 2008-11-06
US20100151350A1 (en) 2010-06-17
CA2683876A1 (en) 2008-11-06
CN101689645A (zh) 2010-03-31
EP2148383A1 (en) 2010-01-27

Similar Documents

Publication Publication Date Title
WO2008111570A1 (ja) 膜－電極接合体およびこれを用いた燃料電池
WO2008096598A1 (ja) 触媒層及びその製法並びに該触媒層を使用した膜－電極接合体及び固体高分子型燃料電池
WO2005006473A3 (de) Membran-elektroden-einheit für elektrochemische vorrichtungen
TW200640067A (en) Gasketed membrane-electrode-assembly and fuel cell system employing the same
WO2008114567A1 (ja) 膜電極接合体
WO2008090774A1 (ja) 高分子電解質膜及びその製法、並びに膜－電極接合体及び固体高分子型燃料電池
WO2010022963A3 (en) Proton exchange membrane for use in proton exchange membrane fuel cells
MX2010000759A (es) Celdas de combustible de oxido solido de reformacion interna.
WO2007142364A8 (en) Process for producing membrane/electrode assembly for polymer electrolyte fuel cells
WO2009054334A1 (ja) 双極型電池の製造方法、および双極型電池
WO2008114688A1 (ja) 電極バインダ、電極、膜－電極接合体及び固体高分子形燃料電池
EP2190047A4 (en) REINFORCED FESTPOLYMER ELECTROLYTE COMPOUND MEMBRANE, MEMBRANE ELECTRODE ASSEMBLY FOR A FESTPOLYMER FUEL CELL AND FESTPOLYMER FUEL CELL
WO2009017147A1 (ja) 燃料電池スタックおよび燃料電池システム
EP1742282A4 (en) MEMBRANE ELECTRODE ASSEMBLY FOR A FUEL CELL AND FUEL CELL THEREFOR
EP1705737B8 (en) Membrane catalyst layer assembly, membrane electrode assembly, and polymer electrolyte fuel cell
ATE465525T1 (de) Laminierungsprozess zur herstellung von integrierten membran-elektroden-baugruppen
EP2131431A4 (en) MEMBRANE ELECTRODE CONTAINER, PROTON-CONDUCTIVE MEMBRANE WITH BONUS LAYER, MEMBRANE ELECTRODE ASSEMBLY, FETTOLYMER FUEL CELL AND METHOD FOR PRODUCING A MEMBRANE ELECTRODE ASSEMBLY
EP2061110B8 (en) Reinforced electrolyte membrane for fuel cell, method for production thereof, membrane-electrode assembly for fuel cell, and solid polymer-type fuel cell having the assembly
WO2008093795A1 (ja) 固体高分子形燃料電池用膜電極接合体、固体高分子形燃料電池およびそれらの製造方法
WO2012173352A3 (ko) 연료전지용 고분자 전해질 막, 이를 포함하는 막 전극 접합체 및 연료전지
WO2009004958A1 (ja) 膜電極接合体及び膜電極接合体の製造方法、固体高分子形燃料電池
WO2008079529A3 (en) Passive recovery of liquid water produced by fuel cells
WO2007124011A3 (en) Methods of making components for electrochemical cells
WO2008133177A1 (ja) 高分子電解質材料及びこれを用いた燃料電池用膜・電極接合体
FR2971628B1 (fr) Pile a combustible a membrane d'echange de protons presentant des performances accrues

Legal Events

Date Code Title Description
WWE Wipo information: entry into national phase

Ref document number: 200880011904.7

Country of ref document: CN

121 Ep: the epo has been informed by wipo that ep was designated in this application

Ref document number: 08740579

Country of ref document: EP

Kind code of ref document: A1

DPE1 Request for preliminary examination filed after expiration of 19th month from priority date (pct application filed from 20040101)
WWE Wipo information: entry into national phase

Ref document number: 2008740579

Country of ref document: EP

WWE Wipo information: entry into national phase

Ref document number: 2683876

Country of ref document: CA

NENP Non-entry into the national phase

Ref country code: DE

WWE Wipo information: entry into national phase

Ref document number: 12595335

Country of ref document: US