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DE932374C - Process for the preparation of thiol compounds - Google Patents

Process for the preparation of thiol compounds

Info

Publication number
DE932374C
DE932374C DEB22575A DEB0022575A DE932374C DE 932374 C DE932374 C DE 932374C DE B22575 A DEB22575 A DE B22575A DE B0022575 A DEB0022575 A DE B0022575A DE 932374 C DE932374 C DE 932374C
Authority
DE
Germany
Prior art keywords
preparation
thiol compounds
compounds
hydrogen sulfide
parts
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
DEB22575A
Other languages
German (de)
Inventor
Richard Dr Kuhn
Guenter Dr Quadbeck
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
BASF SE
Original Assignee
BASF SE
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by BASF SE filed Critical BASF SE
Priority to DEB22575A priority Critical patent/DE932374C/en
Application granted granted Critical
Publication of DE932374C publication Critical patent/DE932374C/en
Expired legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C233/00Carboxylic acid amides
    • C07C233/01Carboxylic acid amides having carbon atoms of carboxamide groups bound to hydrogen atoms or to acyclic carbon atoms
    • C07C233/16Carboxylic acid amides having carbon atoms of carboxamide groups bound to hydrogen atoms or to acyclic carbon atoms having the nitrogen atom of at least one of the carboxamide groups bound to a carbon atom of a hydrocarbon radical substituted by singly-bound oxygen atoms

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Description

Verfahren zur Herstellung von Thiolverbindungen Gegenstand des Patents 893 795 ist ein Verfahren zur Herstellung von Thiolverbindungen, das darin besteht, daß man Äthylenimin mit Thiocarbonsäuren umsetzt.Process for the preparation of thiol compounds Subject matter of the patent 893 795 is a process for the preparation of thiol compounds, which consists in that ethyleneimine is reacted with thiocarboxylic acids.

Es wurde nun gefunden, daß man derartige Verbindungen ebenfalls in sehr vorteilhafter Weise gewinnen kann, wenn man N-Acylverbindungen des Äthylenimins mit Schwefelwasserstoff oder diesen liefernden Substanzen umsetzt. Die Reaktion verläuft bereits in der Kälte sehr glatt; oftmals ist sogar Kühlung notwendig. Zweckmäßig wird in Gegenwart von Lösungs- oder Verdünnungsmitteln gearbeitet. Als geeignete Ausgangsstoffe seien beispielsweise das N-Acetyl-, N-Propionyl-, N-Capryl-und N-Benzoyl-äthylenimin genannt. Die in der beschriebenen Weise erhältlichen Produkte können als Zwischenprodukte für die Gewinnung von Heilmitteln, Kosmetika undTextilhilfsmitteln dienen.It has now been found that such compounds can also be found in can win very advantageously if you use N-acyl compounds of ethylenimine with hydrogen sulfide or these supplying substances. The reaction runs very smoothly even in the cold; often cooling is even necessary. Appropriate is carried out in the presence of solvents or diluents. As suitable Starting materials are, for example, N-acetyl-, N-propionyl-, N-capryl- and N-benzoylethyleneimine called. The products obtainable in the manner described can be used as intermediates are used for the production of remedies, cosmetics and textile auxiliaries.

Beispiel i In ein Gemisch aus i Volumteil N-Acetyläthylenimin (erhältlich nach der Patentschrift 735 008) und a Volumteilen Methanol wird unter Kühlung Schwefelwasserstoff eingeleitet. Das Reaktionsgemisch wird sodann der fraktionierten Destillation im Vakuum unterworfen. Unter 7 mm Druck geht bei 138 bis 1401 N-Acetylcysteamin als farbloses Öl über. Die Ausbeute beträgt mehr als 8o % der Theorie. Beispiel 2 In eine Füllkörpersäule (z. B. von i6o X 8 cm) wird von unten Schwefelwasserstoff eingeleitet, während von oben 5o Gewichtsteile N-Acetyläthylenimin, die mit ioo Gewichtsteilen Methanol verdünnt sind, zütropfen. Die Zutropfgeschwindigkeit wird so reguliert, daß die Hauptreaktionswärme etwa in der Mitte der Säule auftritt. Die weitere Aufarbeitung erfolgt in der in Beispiel i beschriebenen Weise.Example i In a mixture of i part by volume of N-acetylethyleneimine (available according to patent specification 735 008) and a parts by volume of methanol becomes hydrogen sulfide with cooling initiated. The reaction mixture is then the fractional distillation in Subject to vacuum. Under 7 mm pressure, 138 to 1401 N-acetylcysteamine goes as colorless oil over. The yield is more than 80% of theory. example 2 Hydrogen sulphide is poured into a packed column (e.g. 160 X 8 cm) from below initiated, while from above 5o parts by weight of N-acetylethyleneimine, which with ioo Parts by weight of methanol are diluted, add dropwise. The dropping speed becomes regulated so that the main heat of reaction occurs approximately in the middle of the column. The further work-up takes place in the manner described in Example i.

Claims (1)

PATENTANSPRUCH: Weiterbildung des Verfahrens des Patents 893 795 zur Herstellung von Thiolverbindungen, dadurch gekennzeichnet, daß man N-Acylverbindungen des Äth3#lenimin@s mit Schwefelwasserstoff oder diesen liefernden Stoffen. umsetzt.PATENT CLAIM: Further development of the process of the patent 893 795 for Production of thiol compounds, characterized in that N-acyl compounds des Äth3 # lenimin @ s with hydrogen sulfide or substances that supply them. implements.
DEB22575A 1952-10-24 1952-10-24 Process for the preparation of thiol compounds Expired DE932374C (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
DEB22575A DE932374C (en) 1952-10-24 1952-10-24 Process for the preparation of thiol compounds

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
DEB22575A DE932374C (en) 1952-10-24 1952-10-24 Process for the preparation of thiol compounds

Publications (1)

Publication Number Publication Date
DE932374C true DE932374C (en) 1955-08-29

Family

ID=6960942

Family Applications (1)

Application Number Title Priority Date Filing Date
DEB22575A Expired DE932374C (en) 1952-10-24 1952-10-24 Process for the preparation of thiol compounds

Country Status (1)

Country Link
DE (1) DE932374C (en)

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