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DE1165379B - Vapor phase inhibitors to protect iron and its alloys against atmospheric corrosion - Google Patents

Vapor phase inhibitors to protect iron and its alloys against atmospheric corrosion

Info

Publication number
DE1165379B
DE1165379B DEM46646A DEM0046646A DE1165379B DE 1165379 B DE1165379 B DE 1165379B DE M46646 A DEM46646 A DE M46646A DE M0046646 A DEM0046646 A DE M0046646A DE 1165379 B DE1165379 B DE 1165379B
Authority
DE
Germany
Prior art keywords
vapor phase
phase inhibitors
atmospheric corrosion
against atmospheric
protect iron
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Pending
Application number
DEM46646A
Other languages
German (de)
Inventor
Heinrich Mueller
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Individual
Original Assignee
Individual
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Individual filed Critical Individual
Priority to DEM46646A priority Critical patent/DE1165379B/en
Publication of DE1165379B publication Critical patent/DE1165379B/en
Pending legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C23COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23FNON-MECHANICAL REMOVAL OF METALLIC MATERIAL FROM SURFACE; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL; MULTI-STEP PROCESSES FOR SURFACE TREATMENT OF METALLIC MATERIAL INVOLVING AT LEAST ONE PROCESS PROVIDED FOR IN CLASS C23 AND AT LEAST ONE PROCESS COVERED BY SUBCLASS C21D OR C22F OR CLASS C25
    • C23F11/00Inhibiting corrosion of metallic material by applying inhibitors to the surface in danger of corrosion or adding them to the corrosive agent
    • C23F11/02Inhibiting corrosion of metallic material by applying inhibitors to the surface in danger of corrosion or adding them to the corrosive agent in air or gases by adding vapour phase inhibitors

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Mechanical Engineering (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Preventing Corrosion Or Incrustation Of Metals (AREA)

Description

Dampfphaseninhibitoren zum Schutz von Eisen und seinen Legierungen gegen atmosphärische Korrosion In der Hauptpatentanmeldung M46156VIb/48d werden flüchtige Ammoniumazide als Dampfphaseninhibitoren vorgeschlagen.Vapor phase inhibitors for the protection of iron and its alloys against atmospheric corrosion In the main patent application M46156VIb / 48d volatile ammonium azides have been proposed as vapor phase inhibitors.

Wie sich nun herausstellte, läßt sich deren Wirksamkeit steigern, wenn man sie zusammen mit flüchtigen Ammoniumnitriten zur Anwendung bringt, wobei eine größere Schutzwirkung erzielt wird,, als wenn man die Substanzen einzeln für sich einsetzt. Die für diesen Zweck geeigneten Ammoniumnitrite müssen unter normalen Bedingungen beständig sein und können auf der Basis sekundärer aliphatischer, alicyclischer oder heterocyclischer Amine aufgebaut werden, wie z. B. Dibutylamin, Dicyclohexylamin, Morpholin usw. Das Mischungsverhältnis des Azids zum Nitrit kann dabei in weiten Grenzen variieren und liegt zwischen 5 und 95,%. Jedoch ist es zweckmäßig, etwa äquivalente Mengen einzusetzen, da in diesem System eventuell auftretende Stickstoffwasserstoffsäure durch die gleichzeitig anwesende salpetrige Säure zerstört wird, wobei indifferente Produkte entstehen, die den Korrosionsablauf nicht mehr beeinflussen. Die Reaktion verläuft nach HN3 -!- HN02 = N20 -t- N2 -!- H20 Es ist auch in diesem Falle zur Erzielung eines einwandfreien Korrosionsschutzes möglich, anstatt der reinen Verbindungen andere Ammoniumsalze, wie z. B. Phosphate, Oxalate und Benzoate, zusammen mit Alkali- bzw. Erdalkaliazid-nitrit-Gemischen zu verwenden. Der pß-Wert dieser Mischungen soll so sein, daß er in wäßriger Lösung zwischen 6 und 12, vorzugsweise jedoch zwischen 7 und 10 liegt.As it now turned out, their effectiveness can be increased, when used together with volatile ammonium nitrites, where a greater protective effect is achieved, than if one were to use the substances individually for gets involved. The ammonium nitrites suitable for this purpose must be below normal Conditions to be stable and can be based on secondary aliphatic, alicyclic or heterocyclic amines are built up, such as. B. dibutylamine, dicyclohexylamine, Morpholine etc. The mixing ratio of the azide to the nitrite can vary widely Limits vary and is between 5 and 95%. However, it is useful about Use equivalent amounts, since hydrazoic acid may occur in this system is destroyed by the simultaneously present nitrous acid, whereby indifferent Products are created that no longer influence the course of corrosion. The reaction runs according to HN3 -! - HN02 = N20 -t- N2 -! - H20 It is also in this case to Achieving perfect corrosion protection possible instead of the pure connections other ammonium salts, e.g. B. phosphates, oxalates and benzoates, together with alkali or alkaline earth azide-nitrite mixtures to be used. The pβ value of these mixtures should be such that he in aqueous solution between 6 and 12, but preferably between 7 and 10 lies.

Die Wirksamkeit der hier beschriebenen Azid-Nitrit-Gemische mag an folgendem Beispiel erläutert werden. Die Versuche wurden unter den in der Hauptpatentanmeldung angegebenen Bedingungen und Voraussetzungen durchgeführt. Beispiel Ge- Ns- N02- wichts- Inhibitor Konzen- Konzen- zu- Aussehen tration tration rahme (mg) DicYclohexyl- ammonium- azid ....... O,Oln 2,5 schwach gerostet Ge- Ns- N02- wichts- Inhibitor Konzen- Konzen- zu- Aussehen tration tration rahme (mg) DicycloheXyl- ammonium- nitxlt ....... 0,01n 11,5 gerostet Dicyclohexyl- ammonium- azid und Di- cyclohexyl- ammonium- nitrit ....... 0,01n 0,01n 0,0 blank und urgerostet The effectiveness of the azide-nitrite mixtures described here can be illustrated using the following example. The tests were carried out under the conditions and requirements specified in the main patent application. example Ge Ns- N02- weight- Inhibitor Concentrate Concentrate to Appearance tration tration frame (mg) Dicyclohexyl ammonium- acidic ....... O, Oln 2.5 weak roasted Ge Ns- N02- weight- Inhibitor Concentrate Concentrate to Appearance tration tration frame (mg) Dicyclohexyl ammonium- nitxlt ....... 0.01n 11.5 rusted Dicyclohexyl ammonium- acidic and di- cyclohexyl ammonium- nitrite ....... 0.01n 0.01n 0.0 blank and rusted

Claims (1)

Patentanspruch: Verwendung von flüchtigen Ammoniumnitriten auf der Grundlage eines sekundären aliphatischen, alicychschen oder heterocyclischen Amins zusammen mit anorganischen oder organischen Ammoniumaziden gemäß Hauptpatentanmeldung M 46156 VI b/48 d als Dampfphaseninhibitoren zum Schutz von Gegenständen aus Eisen und seinen Legierungen vor Korrosion. In Betracht gezogene Druckschriften: Österreichische Patentschrift Nr. 185190.Claim: Use of volatile ammonium nitrites on the Based on a secondary aliphatic, alicychic or heterocyclic amine together with inorganic or organic ammonium azides according to the main patent application M 46156 VI b / 48 d as vapor phase inhibitors to protect iron objects and its alloys from corrosion. Publications considered: Österreichische Patent No. 185190.
DEM46646A 1960-09-23 1960-09-23 Vapor phase inhibitors to protect iron and its alloys against atmospheric corrosion Pending DE1165379B (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
DEM46646A DE1165379B (en) 1960-09-23 1960-09-23 Vapor phase inhibitors to protect iron and its alloys against atmospheric corrosion

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
DEM46646A DE1165379B (en) 1960-09-23 1960-09-23 Vapor phase inhibitors to protect iron and its alloys against atmospheric corrosion

Publications (1)

Publication Number Publication Date
DE1165379B true DE1165379B (en) 1964-03-12

Family

ID=7305662

Family Applications (1)

Application Number Title Priority Date Filing Date
DEM46646A Pending DE1165379B (en) 1960-09-23 1960-09-23 Vapor phase inhibitors to protect iron and its alloys against atmospheric corrosion

Country Status (1)

Country Link
DE (1) DE1165379B (en)

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3383328A (en) * 1966-04-04 1968-05-14 Navy Usa Water displacing and rust preventive compositions

Citations (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
AT185190B (en) * 1944-10-05 1956-04-10 Bataafsche Petroleum Process for protecting metal surfaces against corrosion and packaging material that protects against corrosion

Patent Citations (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
AT185190B (en) * 1944-10-05 1956-04-10 Bataafsche Petroleum Process for protecting metal surfaces against corrosion and packaging material that protects against corrosion

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3383328A (en) * 1966-04-04 1968-05-14 Navy Usa Water displacing and rust preventive compositions

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