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DE1089725B - Process for the simultaneous dyeing and antistatic rendering of textile materials based on polyacrylonitrile - Google Patents

Process for the simultaneous dyeing and antistatic rendering of textile materials based on polyacrylonitrile

Info

Publication number
DE1089725B
DE1089725B DEF25046A DEF0025046A DE1089725B DE 1089725 B DE1089725 B DE 1089725B DE F25046 A DEF25046 A DE F25046A DE F0025046 A DEF0025046 A DE F0025046A DE 1089725 B DE1089725 B DE 1089725B
Authority
DE
Germany
Prior art keywords
antistatic
polyacrylonitrile
dyeing
textile materials
materials based
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Pending
Application number
DEF25046A
Other languages
German (de)
Inventor
Dr Joseph Nuesslein
Dr Adolf Vogt
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Hoechst AG
Original Assignee
Hoechst AG
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Hoechst AG filed Critical Hoechst AG
Priority to DEF25046A priority Critical patent/DE1089725B/en
Priority claimed from DEF25048A external-priority patent/DE1061513B/en
Publication of DE1089725B publication Critical patent/DE1089725B/en
Pending legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G79/00Macromolecular compounds obtained by reactions forming a linkage containing atoms other than silicon, sulfur, nitrogen, oxygen, and carbon with or without the latter elements in the main chain of the macromolecule
    • C08G79/02Macromolecular compounds obtained by reactions forming a linkage containing atoms other than silicon, sulfur, nitrogen, oxygen, and carbon with or without the latter elements in the main chain of the macromolecule a linkage containing phosphorus
    • C08G79/06Phosphorus linked to carbon only
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G12/00Condensation polymers of aldehydes or ketones with only compounds containing hydrogen attached to nitrogen
    • C08G12/02Condensation polymers of aldehydes or ketones with only compounds containing hydrogen attached to nitrogen of aldehydes
    • C08G12/40Chemically modified polycondensates
    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06MTREATMENT, NOT PROVIDED FOR ELSEWHERE IN CLASS D06, OF FIBRES, THREADS, YARNS, FABRICS, FEATHERS OR FIBROUS GOODS MADE FROM SUCH MATERIALS
    • D06M15/00Treating fibres, threads, yarns, fabrics, or fibrous goods made from such materials, with macromolecular compounds; Such treatment combined with mechanical treatment
    • D06M15/19Treating fibres, threads, yarns, fabrics, or fibrous goods made from such materials, with macromolecular compounds; Such treatment combined with mechanical treatment with synthetic macromolecular compounds
    • D06M15/37Macromolecular compounds obtained otherwise than by reactions only involving carbon-to-carbon unsaturated bonds
    • D06M15/39Aldehyde resins; Ketone resins; Polyacetals
    • D06M15/423Amino-aldehyde resins
    • D06M15/43Amino-aldehyde resins modified by phosphorus compounds
    • D06M15/431Amino-aldehyde resins modified by phosphorus compounds by phosphines or phosphine oxides; by oxides or salts of the phosphonium radical
    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06PDYEING OR PRINTING TEXTILES; DYEING LEATHER, FURS OR SOLID MACROMOLECULAR SUBSTANCES IN ANY FORM
    • D06P1/00General processes of dyeing or printing textiles, or general processes of dyeing leather, furs, or solid macromolecular substances in any form, classified according to the dyes, pigments, or auxiliary substances employed
    • D06P1/44General processes of dyeing or printing textiles, or general processes of dyeing leather, furs, or solid macromolecular substances in any form, classified according to the dyes, pigments, or auxiliary substances employed using insoluble pigments or auxiliary substances, e.g. binders
    • D06P1/60General processes of dyeing or printing textiles, or general processes of dyeing leather, furs, or solid macromolecular substances in any form, classified according to the dyes, pigments, or auxiliary substances employed using insoluble pigments or auxiliary substances, e.g. binders using compositions containing polyethers
    • D06P1/607Nitrogen-containing polyethers or their quaternary derivatives
    • D06P1/6076Nitrogen-containing polyethers or their quaternary derivatives addition products of amines and alkylene oxides or oxiranes
    • DTEXTILES; PAPER
    • D06TREATMENT OF TEXTILES OR THE LIKE; LAUNDERING; FLEXIBLE MATERIALS NOT OTHERWISE PROVIDED FOR
    • D06PDYEING OR PRINTING TEXTILES; DYEING LEATHER, FURS OR SOLID MACROMOLECULAR SUBSTANCES IN ANY FORM
    • D06P3/00Special processes of dyeing or printing textiles, or dyeing leather, furs, or solid macromolecular substances in any form, classified according to the material treated
    • D06P3/70Material containing nitrile groups
    • D06P3/76Material containing nitrile groups using basic dyes

Landscapes

  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Textile Engineering (AREA)
  • Health & Medical Sciences (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Coloring (AREA)

Description

DEUTSCHESGERMAN

Vollsynthetische Fasermaterialien, wie Flocke, Kammzug oder endlose Fäden, laden sich durch Reibung bei der Verarbeitung sehr leicht elektrostatisch auf, wodurch erhebliche Verarbeitungsschwierigkeiten hervorgerufen werden. Zur Verhinderung der elektrostatischen Aufladung derartiger Materialien hat man diese bisher mit Mitteln behandelt, die eine Erhöhung des elektrischen Leitvermögens bewirken. Als antistatische Mittel hat man anorganische Salze wie auch anionische, kationische und nichtionogene Verbindungen eingesetzt, die man auf das ungefärbte Material oder nach dem Färben aufgetragen hat. Diese Behandlung erfolgt z. B. beim Kammzug vorzugsweise auf der Lisseuse, wobei im letzten Spülbad das Präparationsmittel eingesetzt wird. Eine weitere Naßbehandlung erfolgt dann nicht mehr vor dem Spinnprozeß, um ein Ausspulen des wirksamen Präparationsmittels zu vermeiden. Soweit ungefärbtes Material erst nach dem Spinnen und Weben gefärbt wurde, hat man die Präparation vor dem Färbebad ausgespült, um eine Beeinträchtigung der Färbung zu vermeiden.Fully synthetic fiber materials such as flake, sliver or endless threads, are very easily charged electrostatically due to friction during processing, which means that considerable processing difficulties are caused. To prevent electrostatic charge Such materials have hitherto been treated with agents that increase the electrical conductivity cause. As antistatic agents, there are inorganic salts as well as anionic, cationic and non-ionic compounds used, which are applied to the uncolored material or after dyeing Has. This treatment is carried out e.g. B. preferably on the Lisseuse in the ridge draw, with the last rinsing bath the preparation agent is used. No further wet treatment takes place before the spinning process, to avoid rinsing out the effective spin finish. As far as uncolored material first after the spinning and weaving was dyed, the preparation was rinsed out before the dyebath to avoid a To avoid deterioration of the coloring.

Als antistatische Mittel hat man auch bereits Oxäthylierungsprodukte von primären oder sekundären Aminen empfohlen. Hierbei hat man jedoch Produkte verwendet, die bis zu 50 Mol Äthylenoxyd enthalten.Ethylation products are also already available as antistatic agents recommended by primary or secondary amines. Here, however, products have been used which contain up to 50 moles of ethylene oxide.

Es wurde nun gefunden, daß ein geringer Zusatz niedrig oxäthylierter Fettamine sich beim Färben von Polyacrylnitrilfasern mit basischen Farbstoffen nicht störend auswirkt und auch nach dem Spülprozeß noch einen guten antistatischen Effekt bewirkt, so daß man vollsynthetisches Fasermaterial auf Basis Polyacrylnitril gleichzeitig mit basischen Farbstoffen färben und antistatisch ausrüsten kann, wenn man dem Färbebad Verbindungen der allgemeinen FormelIt has now been found that a small addition of low oxyethylated fatty amines is useful when dyeing Polyacrylonitrile fibers with basic dyes do not have a disruptive effect and even after the rinsing process causes a good antistatic effect, so that one fully synthetic fiber material based on polyacrylonitrile at the same time dyeing with basic dyes and antistatic finish if you put the dye bath Compounds of the general formula

Verfahren zum gleichzeitigen FärbenSimultaneous dyeing method

und Antistatischmachenand antistatic

von Textilmaterialien auf Basisof textile materials based

PolyacrylnitrilPolyacrylonitrile

Anmelder:Applicant:

Farbwerke Hoechst AktiengesellschaftFarbwerke Hoechst Aktiengesellschaft

vormals Meister Lucius & Brüning,formerly Master Lucius & Brüning,

Frankfurt/M., Brüningstr. 45Frankfurt / M., Brüningstr. 45

Dr. Joseph Nüsslein, Frankfurt/M.,Dr. Joseph Nüsslein, Frankfurt / M.,

und Dr. Adolf Vogt, Bad Soden (Taunus),and Dr. Adolf Vogt, Bad Soden (Taunus),

sind als Erfinder genannt wordenhave been named as inventors

R—n:R — n:

zusetzt, worin R einen Kohlenwasserstoffrest mit mindestens 10 Kohlenstoffatomen, vorzugsweise 16 bis 20 Kohlenstoffatomen, X und Y einen Äthylenglykol- oder Polyäthylenglykolrest mit insgesamt 2 bis 6, vorzugsweise 2 bis 3 Äthylenglykolgruppen bedeuten.
Als Verbindungen der allgemeinen Formel
added, wherein R is a hydrocarbon radical with at least 10 carbon atoms, preferably 16 to 20 carbon atoms, X and Y an ethylene glycol or polyethylene glycol radical with a total of 2 to 6, preferably 2 to 3 ethylene glycol groups.
As compounds of the general formula

X
R — N,
X
R - N,

kommen Umsetzungsprodukte von Fettaminen mit mindestens 10 Kohlenstoffatomen, beispielsweise Decylamin, Lauryl-, Palmityl-, Oleyl-, Stearylamin, Palmkernfettalkylamin, Talgfettalkylamin, Cocosfettalkylamin, Äthyllauryl-amin, Methyl-pahnityl-amin u. ä. mit insgesamt 2 bis 6 Mol Äthylenoxyd in Betracht. An Stelle einheitlicher Umsetzungsprodukte können auch Mischungen der genannten Verbindungen oder Oxäthylierungsprodukte technischer Gemische von Aminen, wie sie aus natürlichen Fettsäuren und Gemischen derselben gewonnen werden, verwendet werden.there are reaction products of fatty amines with at least 10 carbon atoms, for example decylamine, Lauryl, palmityl, oleyl, stearylamine, palm kernel fatty alkylamine, Tallow fatty alkylamine, coconut fatty alkylamine, ethyl lauryl amine, Methyl-pahnityl-amine and the like with a total of 2 to 6 moles of ethylene oxide into consideration. Instead of uniform reaction products, mixtures of the compounds mentioned or Oxäthylierungsprodukte technical mixtures of amines, such as those from natural Fatty acids and mixtures thereof are obtained, can be used.

Die Konzentration der gemäß dem Verfahren der vorliegenden Erfindung dem Färbebad zuzusetzenden Produkte kann in gewissen Grenzen schwanken. Üblicherweise wird man etwa 0,15 bis 0,3 g/l wirksame Substanz der Produkte verwenden. Eine zu hohe Konzentration des Zusatzes bewirkt eine deutlich in Erscheinung tretende Zurückhaltung des Farbstoffes.The concentration of those to be added to the dye bath according to the method of the present invention Products can fluctuate within certain limits. Usually about 0.15 to 0.3 g / l of active substance will be used of the products. Too high a concentration of the additive causes a clear appearance increasing reluctance of the dye.

Das Verfahren der vorliegenden Erfindung gestattet es, das Färben von Polyacrylnitril-Fasermaterialien mit basischen Farbstoffen, wie Triphenyl- oder Diphenylmethanfarbstoffen, Xanthenfarbstoffen, Azin- oder Thiazinfarbstoffen, gleichzeitig mit der antistatischen Ausrüstung vor dem Spinnen und Weben vorzunehmen, so daß ein Präparieren im Anschluß an das Färbebad entfällt. Die vorliegende Arbeitsweise gestattet also, Färben und Präparieren in einem Bad und in einem Arbeitsgang vorzunehmen.The method of the present invention allows the dyeing of polyacrylonitrile fiber materials with basic dyes, such as triphenyl or diphenylmethane dyes, xanthene dyes, azine or Thiazine dyes, to be carried out simultaneously with the antistatic finish before spinning and weaving, so that preparation after the dyebath is not necessary. The present way of working thus allows Dyeing and preparation in one bath and in one operation.

Beispielexample

100 g reine Polyacrylnitrilfasern werden im Flottenveihältnis 1:50 in einem Bad gefärbt, das 2°/0 Methylenblau BB extra stark (Schultz Farbstofftabellen, 7. Auflage, Nr. 1038), 1% Essigsäure (30°/0ig) und 0,5 g/l des Anlagerungsproduktes von 2 Mol Äthylenoxyd an 1 Mol Stearylamin (33% aktive Substanz) enthält. Man geht100 g of pure polyacrylonitrile fibers are dyed in a bath in a liquor ratio of 1:50, the 2 % / 0 methylene blue BB extra strong (Schultz dye tables, 7th edition, No. 1038), 1% acetic acid (30% / 0 ig) and 0, Contains 5 g / l of the adduct of 2 moles of ethylene oxide with 1 mole of stearylamine (33% active substance). One goes

009 609/363009 609/363

bei 6O0C mit der Ware ein, erhöht die Temperatur innerhalb von 45 Minuten zum Kochen und färbt I1Z2 Stunden in kochender Flotte. Anschließend wird die gefärbte Ware gespült, bis das Spülbad klar ist.at 6O 0 C with the goods, increases the temperature within 45 minutes to boiling and dyes I 1 Z 2 hours in boiling liquor. The dyed goods are then rinsed until the rinsing bath is clear.

Nach dem Trocknen ist das gefärbte Fasermaterial gleichzeitig antistatisch ausgerüstet und läuft einwandfrei über die Krempel. Während ein Material, das ohne den Zusatz des Oxäthylierungsproduktes gefärbt wurde, einen Megohmwert von 180000 zeigt, liegt der Megohmwert der wie vorstehend beschrieben behandelten Faser bei 730 Megohm.After drying, the dyed fiber material is antistatic at the same time and runs perfectly over the clutter. While a material which has been colored without the addition of the oxethylation product, shows a megohm value of 180,000, the megohm value of the fiber treated as described above is at 730 megohms.

Claims (2)

PATENTANSPRÜCHE:PATENT CLAIMS: 1. Verfahren zum gleichzeitigen Färben und Antistatischmachen von Textilmaterialien auf Basis Polyacrylnitril vor dem Spinnen oder Weben, dadurch gekennzeichnet, daß man in einem Färbebad färbt, das basische Farbstoffe und Verbindungen der allgemeinen Formel1. A process for the simultaneous dyeing and antistatic treatment of textile materials based on polyacrylonitrile before spinning or weaving, characterized in that dyeing in a dye bath, the basic dyes and compounds of the general formula X
R — N,
X
R - N,
enthält, in der R einen Kohlenwasserstoffrest mit mindestens 10 Kohlenstoffatomen, X und Y Äthylenglykol- oder Polyäthylenglykolreste mit insgesamt 2 bis 6 Äthylenglykolgruppen bedeuten.contains, in which R is a hydrocarbon radical with at least 10 carbon atoms, X and Y ethylene glycol or mean polyethylene glycol residues with a total of 2 to 6 ethylene glycol groups.
2. Verfahren nach Anspruch 1, dadurch gekennzeichnet, daß R einen Kohlenwasserstoffrest mit 16 bis 20 Kohlenstoffatomen und X und Y Äthylenglykol- oder Polyäthylenglykolreste mit insgesamt 2 bis 3 Äthylenglykolgruppen bedeuten.2. The method according to claim 1, characterized in that R is a hydrocarbon radical with 16 to 20 carbon atoms and X and Y ethylene glycol or polyethylene glycol residues with a total of 2 to 3 ethylene glycol groups mean. © 009 609/363 9.60© 009 609/363 9.60
DEF25046A 1958-02-14 1958-02-14 Process for the simultaneous dyeing and antistatic rendering of textile materials based on polyacrylonitrile Pending DE1089725B (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
DEF25046A DE1089725B (en) 1958-02-14 1958-02-14 Process for the simultaneous dyeing and antistatic rendering of textile materials based on polyacrylonitrile

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
DEF25046A DE1089725B (en) 1958-02-14 1958-02-14 Process for the simultaneous dyeing and antistatic rendering of textile materials based on polyacrylonitrile
DEF25048A DE1061513B (en) 1958-02-14 1958-02-14 Process for the production of incombustible, phosphorus-containing condensation resins

Publications (1)

Publication Number Publication Date
DE1089725B true DE1089725B (en) 1960-09-29

Family

ID=25974107

Family Applications (1)

Application Number Title Priority Date Filing Date
DEF25046A Pending DE1089725B (en) 1958-02-14 1958-02-14 Process for the simultaneous dyeing and antistatic rendering of textile materials based on polyacrylonitrile

Country Status (1)

Country Link
DE (1) DE1089725B (en)

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