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WO2004098773A3 - Catalyst layer containing an acidic ion exchanger and specific base polymers, suitable catalyst paste, and method for the production thereof - Google Patents

Catalyst layer containing an acidic ion exchanger and specific base polymers, suitable catalyst paste, and method for the production thereof Download PDF

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Publication number
WO2004098773A3
WO2004098773A3 PCT/DE2004/000896 DE2004000896W WO2004098773A3 WO 2004098773 A3 WO2004098773 A3 WO 2004098773A3 DE 2004000896 W DE2004000896 W DE 2004000896W WO 2004098773 A3 WO2004098773 A3 WO 2004098773A3
Authority
WO
WIPO (PCT)
Prior art keywords
catalyst
production
ion exchanger
specific base
acidic ion
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Ceased
Application number
PCT/DE2004/000896
Other languages
German (de)
French (fr)
Other versions
WO2004098773A2 (en
Inventor
Kai Jakoby
Morten Schonert
Andreas Gluesen
Carola Schlumbohm
Detlef Stolten
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Forschungszentrum Juelich GmbH
Original Assignee
Forschungszentrum Juelich GmbH
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Forschungszentrum Juelich GmbH filed Critical Forschungszentrum Juelich GmbH
Priority to EP04730194A priority Critical patent/EP1624966A2/en
Publication of WO2004098773A2 publication Critical patent/WO2004098773A2/en
Publication of WO2004098773A3 publication Critical patent/WO2004098773A3/en
Anticipated expiration legal-status Critical
Ceased legal-status Critical Current

Links

Classifications

    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8663—Selection of inactive substances as ingredients for catalytic active masses, e.g. binders, fillers
    • H01M4/8668—Binders
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J23/00—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00
    • B01J23/38—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of noble metals
    • B01J23/40—Catalysts comprising metals or metal oxides or hydroxides, not provided for in group B01J21/00 of noble metals of the platinum group metals
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J31/00—Catalysts comprising hydrides, coordination complexes or organic compounds
    • B01J31/02—Catalysts comprising hydrides, coordination complexes or organic compounds containing organic compounds or metal hydrides
    • B01J31/06—Catalysts comprising hydrides, coordination complexes or organic compounds containing organic compounds or metal hydrides containing polymers
    • B01J31/08—Ion-exchange resins
    • B—PERFORMING OPERATIONS; TRANSPORTING
    • B01—PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01J—CHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J37/00—Processes, in general, for preparing catalysts; Processes, in general, for activation of catalysts
    • B01J37/02—Impregnation, coating or precipitation
    • B01J37/0215—Coating
    • B01J37/0219—Coating the coating containing organic compounds
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/8605—Porous electrodes
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M4/00—Electrodes
    • H01M4/86—Inert electrodes with catalytic activity, e.g. for fuel cells
    • H01M4/88—Processes of manufacture
    • H01M4/8825—Methods for deposition of the catalytic active composition
    • H01M4/8828—Coating with slurry or ink
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells

Landscapes

  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • Organic Chemistry (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Materials Engineering (AREA)
  • Manufacturing & Machinery (AREA)
  • Catalysts (AREA)

Abstract

Known prior art catalyst pastes are, as a rule, to liquid for coating by means of silk-screen printing or colour ductors. The invention relates to a method for the production of a catalyst paste, containing an acidic ion exchanger and specific base polymers, which is especially suitable for coating methods such as silk-screen printing and colour ductors due to the viscosity thereof. A catalyst layer produced with said inventive catalyst paste does not regularly display any loss in performance compared to catalyst layers produced by prior art standard catalyst pastes. Even improved performance properties are partially obtained.
PCT/DE2004/000896 2003-05-06 2004-04-29 Catalyst layer containing an acidic ion exchanger and specific base polymers, suitable catalyst paste, and method for the production thereof Ceased WO2004098773A2 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
EP04730194A EP1624966A2 (en) 2003-05-06 2004-04-29 Catalyst layer, suitable catalyst paste, and method for the production thereof

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
DE10320320A DE10320320B4 (en) 2003-05-06 2003-05-06 Catalyst layer, suitable catalyst paste, as well as production process thereof
DE10320320.6 2003-05-06

Publications (2)

Publication Number Publication Date
WO2004098773A2 WO2004098773A2 (en) 2004-11-18
WO2004098773A3 true WO2004098773A3 (en) 2005-02-10

Family

ID=33426688

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/DE2004/000896 Ceased WO2004098773A2 (en) 2003-05-06 2004-04-29 Catalyst layer containing an acidic ion exchanger and specific base polymers, suitable catalyst paste, and method for the production thereof

Country Status (3)

Country Link
EP (1) EP1624966A2 (en)
DE (1) DE10320320B4 (en)
WO (1) WO2004098773A2 (en)

Families Citing this family (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE102004024845A1 (en) * 2004-05-13 2005-12-08 Volkswagen Ag Catalyst layer`s manufacture for high-temperature fuel cells, involves applying electrode paste on substrate under blade pressure to form catalyst layers, drying layers above room temperature and soaking dried layers in acid
DE102005054149A1 (en) * 2005-11-14 2007-05-16 Basf Ag Amine-containing catalyst ink for fuel cells

Citations (12)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US5415888A (en) * 1993-04-26 1995-05-16 E. I. Du Pont De Nemours And Company Method of imprinting catalytically active particles on membrane
EP0731520A1 (en) * 1995-03-09 1996-09-11 Johnson Matthey Public Limited Company Materials for use in catalytic electrode manufacture
DE19817376A1 (en) * 1998-04-18 1999-10-21 Univ Stuttgart Lehrstuhl Und I Ion exchange membranes and polymer blends, useful for fuel cells, gas separation, pervaporation and reverse osmosis
DE19817374A1 (en) * 1998-04-18 1999-10-21 Univ Stuttgart Lehrstuhl Und I Acid base polymer blends and membranes useful as polymer electrolyte membranes in fuel cells, pervaporation and reverse osmosis
DE19836514A1 (en) * 1998-08-12 2000-02-17 Univ Stuttgart Modification of engineering polymers with N-basic groups and ion exchange groups in the side chain gives membranes of good thermal and mechanical stability useful for fuel cells, diffusion dialysis, electrodialysis, and reverse osmosis
WO2001071840A2 (en) * 2000-03-20 2001-09-27 Stichting Energieonderzoek Centrum Nederland Production of low-temperature fuel cell electrodes
DE10021106A1 (en) * 2000-05-02 2001-11-08 Univ Stuttgart Polymeric membranes
EP1176652A2 (en) * 2000-07-29 2002-01-30 OMG AG & Co. KG Ink for manufacturing membrane electrode units for PEM fuel cells
DE10201886A1 (en) * 2001-01-19 2002-08-01 Honda Motor Co Ltd Polymer electrolyte membrane and solid polymer electrolyte fuel cell using them
US20030008199A1 (en) * 1999-08-20 2003-01-09 Medis El Ltd. Class of electrocatalysts and a gas diffusion electrode based thereon
WO2003014201A2 (en) * 2001-07-07 2003-02-20 Haering Thomas Membranes for ion transport
WO2003078492A2 (en) * 2002-02-28 2003-09-25 Haering Thomas Layered structures and method for producing the same

Family Cites Families (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US6221523B1 (en) * 1998-02-10 2001-04-24 California Institute Of Technology Direct deposit of catalyst on the membrane of direct feed fuel cells
KR100407793B1 (en) * 2001-09-04 2003-12-01 한국과학기술연구원 proton exchange composite membranes and composite solutions having selectivity, its preparation and fuel cell comprising the same
AU2002357324A1 (en) * 2001-12-19 2003-07-09 Polyfuel, Inc. Printing of catalyst on the membrane of fuel cells

Patent Citations (12)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US5415888A (en) * 1993-04-26 1995-05-16 E. I. Du Pont De Nemours And Company Method of imprinting catalytically active particles on membrane
EP0731520A1 (en) * 1995-03-09 1996-09-11 Johnson Matthey Public Limited Company Materials for use in catalytic electrode manufacture
DE19817376A1 (en) * 1998-04-18 1999-10-21 Univ Stuttgart Lehrstuhl Und I Ion exchange membranes and polymer blends, useful for fuel cells, gas separation, pervaporation and reverse osmosis
DE19817374A1 (en) * 1998-04-18 1999-10-21 Univ Stuttgart Lehrstuhl Und I Acid base polymer blends and membranes useful as polymer electrolyte membranes in fuel cells, pervaporation and reverse osmosis
DE19836514A1 (en) * 1998-08-12 2000-02-17 Univ Stuttgart Modification of engineering polymers with N-basic groups and ion exchange groups in the side chain gives membranes of good thermal and mechanical stability useful for fuel cells, diffusion dialysis, electrodialysis, and reverse osmosis
US20030008199A1 (en) * 1999-08-20 2003-01-09 Medis El Ltd. Class of electrocatalysts and a gas diffusion electrode based thereon
WO2001071840A2 (en) * 2000-03-20 2001-09-27 Stichting Energieonderzoek Centrum Nederland Production of low-temperature fuel cell electrodes
DE10021106A1 (en) * 2000-05-02 2001-11-08 Univ Stuttgart Polymeric membranes
EP1176652A2 (en) * 2000-07-29 2002-01-30 OMG AG & Co. KG Ink for manufacturing membrane electrode units for PEM fuel cells
DE10201886A1 (en) * 2001-01-19 2002-08-01 Honda Motor Co Ltd Polymer electrolyte membrane and solid polymer electrolyte fuel cell using them
WO2003014201A2 (en) * 2001-07-07 2003-02-20 Haering Thomas Membranes for ion transport
WO2003078492A2 (en) * 2002-02-28 2003-09-25 Haering Thomas Layered structures and method for producing the same

Non-Patent Citations (3)

* Cited by examiner, † Cited by third party
Title
KERRES J ET AL: "Synthesis and characterization of polyaryl blend membranes having different composition, different covalent and/or ionical cross-linking density, and their application to DMFC", DESALINATION, ELSEVIER SCIENTIFIC PUBLISHING CO, AMSTERDAM, NL, vol. 147, no. 1-3, 10 September 2002 (2002-09-10), pages 173 - 178, XP004386428, ISSN: 0011-9164 *
KERRES J ET AL: "Synthesis of novel engineering polymers containing basic side groups and their application in acid-base polymer blend membranes", SEPARATION AND PURIFICATION TECHNOLOGY, vol. 22-23, 1 March 2001 (2001-03-01), pages 1 - 15, XP002307986 *
MAKOTO UCHIDA ET AL: "NEW PREPARATION METHOD FOR POLYMER-ELECTROLYTE FUEL CELLS", JOURNAL OF THE ELECTROCHEMICAL SOCIETY, ELECTROCHEMICAL SOCIETY. MANCHESTER, NEW HAMPSHIRE, US, vol. 142, no. 2, February 1995 (1995-02-01), pages 463 - 468, XP002155036, ISSN: 0013-4651 *

Also Published As

Publication number Publication date
DE10320320B4 (en) 2007-08-16
WO2004098773A2 (en) 2004-11-18
DE10320320A1 (en) 2004-12-16
EP1624966A2 (en) 2006-02-15

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