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WO2002019455A3 - Verfahren zum herstellen einer festkeramischen brennstoffzelle - Google Patents

Verfahren zum herstellen einer festkeramischen brennstoffzelle Download PDF

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Publication number
WO2002019455A3
WO2002019455A3 PCT/EP2001/009760 EP0109760W WO0219455A3 WO 2002019455 A3 WO2002019455 A3 WO 2002019455A3 EP 0109760 W EP0109760 W EP 0109760W WO 0219455 A3 WO0219455 A3 WO 0219455A3
Authority
WO
WIPO (PCT)
Prior art keywords
producing
fuel cell
ceramic fuel
solid ceramic
electrode
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Ceased
Application number
PCT/EP2001/009760
Other languages
English (en)
French (fr)
Other versions
WO2002019455A2 (de
Inventor
Gerard Barbezat
Robert Fleck
Thomas Jansing
Michael Loch
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Oerlikon Metco AG
Siemens AG
Siemens Corp
Original Assignee
Sulzer Metco AG
Siemens AG
Siemens Corp
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Sulzer Metco AG, Siemens AG, Siemens Corp filed Critical Sulzer Metco AG
Priority to EP01960706A priority Critical patent/EP1344272A2/de
Priority to US10/362,831 priority patent/US7141271B2/en
Priority to AU2001282121A priority patent/AU2001282121A1/en
Publication of WO2002019455A2 publication Critical patent/WO2002019455A2/de
Anticipated expiration legal-status Critical
Publication of WO2002019455A3 publication Critical patent/WO2002019455A3/de
Ceased legal-status Critical Current

Links

Classifications

    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/124—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the process of manufacturing or by the material of the electrolyte
    • C—CHEMISTRY; METALLURGY
    • C23—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; CHEMICAL SURFACE TREATMENT; DIFFUSION TREATMENT OF METALLIC MATERIAL; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL; INHIBITING CORROSION OF METALLIC MATERIAL OR INCRUSTATION IN GENERAL
    • C23C—COATING METALLIC MATERIAL; COATING MATERIAL WITH METALLIC MATERIAL; SURFACE TREATMENT OF METALLIC MATERIAL BY DIFFUSION INTO THE SURFACE, BY CHEMICAL CONVERSION OR SUBSTITUTION; COATING BY VACUUM EVAPORATION, BY SPUTTERING, BY ION IMPLANTATION OR BY CHEMICAL VAPOUR DEPOSITION, IN GENERAL
    • C23C4/00—Coating by spraying the coating material in the molten state, e.g. by flame, plasma or electric discharge
    • C23C4/12—Coating by spraying the coating material in the molten state, e.g. by flame, plasma or electric discharge characterised by the method of spraying
    • C23C4/134—Plasma spraying
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M8/1213—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte characterised by the electrode/electrolyte combination or the supporting material
    • H—ELECTRICITY
    • H01—ELECTRIC ELEMENTS
    • H01M—PROCESSES OR MEANS, e.g. BATTERIES, FOR THE DIRECT CONVERSION OF CHEMICAL ENERGY INTO ELECTRICAL ENERGY
    • H01M8/00—Fuel cells; Manufacture thereof
    • H01M8/10—Fuel cells with solid electrolytes
    • H01M8/12—Fuel cells with solid electrolytes operating at high temperature, e.g. with stabilised ZrO2 electrolyte
    • H01M2008/1293—Fuel cells with solid oxide electrolytes
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02E—REDUCTION OF GREENHOUSE GAS [GHG] EMISSIONS, RELATED TO ENERGY GENERATION, TRANSMISSION OR DISTRIBUTION
    • Y02E60/00—Enabling technologies; Technologies with a potential or indirect contribution to GHG emissions mitigation
    • Y02E60/30—Hydrogen technology
    • Y02E60/50—Fuel cells
    • Y—GENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02—TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02P—CLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P70/00—Climate change mitigation technologies in the production process for final industrial or consumer products
    • Y02P70/50—Manufacturing or production processes characterised by the final manufactured product

Landscapes

  • Engineering & Computer Science (AREA)
  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Manufacturing & Machinery (AREA)
  • Sustainable Energy (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Plasma & Fusion (AREA)
  • Sustainable Development (AREA)
  • Physics & Mathematics (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Materials Engineering (AREA)
  • Mechanical Engineering (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Fuel Cell (AREA)

Abstract

Bei dem Verfahren festkeramischen Brennstoffzelle wird innerhalb einer Beschichtungskammer (10) eine Festelektrolytschicht (8) auf eine Elektrode (4) mittels eines Plasmaspritzverfahrens gasdicht aufgebracht, wobei in der Beschichtungskammer (10) ein Druck von kleiner etwa 15 mbar eingestellt wird. Im Plasmastrahl (20) ist ein pulverförmiges Beschichtungsmaterial, vorzugsweise mit einem Partikelmesser von deutlich unter 10 νm, derart dünn verteilt, dass die einzelnen Partikel isoliert voneinander auf der Elektrode (4) auftreffen. Dadurch lässt sich eine sehr homogene und dichte Festelektrolytschicht (8) aufbringen.
PCT/EP2001/009760 2000-08-30 2001-08-23 Verfahren zum herstellen einer festkeramischen brennstoffzelle Ceased WO2002019455A2 (de)

Priority Applications (3)

Application Number Priority Date Filing Date Title
EP01960706A EP1344272A2 (de) 2000-08-30 2001-08-23 Verfahren zum herstellen einer festkeramischen brennstoffzelle
US10/362,831 US7141271B2 (en) 2000-08-30 2001-08-23 Method for producing a solid ceramic fuel cell
AU2001282121A AU2001282121A1 (en) 2000-08-30 2001-08-23 Method for producing a solid ceramic fuel cell

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
EP00118769 2000-08-30
EP00118769.9 2000-08-30

Publications (2)

Publication Number Publication Date
WO2002019455A2 WO2002019455A2 (de) 2002-03-07
WO2002019455A3 true WO2002019455A3 (de) 2003-06-05

Family

ID=8169695

Family Applications (1)

Application Number Title Priority Date Filing Date
PCT/EP2001/009760 Ceased WO2002019455A2 (de) 2000-08-30 2001-08-23 Verfahren zum herstellen einer festkeramischen brennstoffzelle

Country Status (4)

Country Link
US (1) US7141271B2 (de)
EP (1) EP1344272A2 (de)
AU (1) AU2001282121A1 (de)
WO (1) WO2002019455A2 (de)

Families Citing this family (16)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE10222855A1 (de) * 2002-05-23 2003-12-11 Siemens Ag Verfahren zur Herstellung beschichteter Rohre und damit aufgebaute Brennstoffzellenanlage
EP1479788B1 (de) * 2003-05-23 2007-11-28 Sulzer Metco AG Hybrides Verfahren zum Beschichten eines Substrats durch ein thermisches Aufbringen der Beschichtung
CA2460296C (en) 2003-05-23 2012-02-14 Sulzer Metco Ag A hybrid method for the coating of a substrate by a thermal application of the coating
DE102004004477A1 (de) * 2004-01-28 2005-08-18 Siemens Ag Verfahren und Vorrichtung zum Herstellen einer festkeramischen Brennstoffzelle
DE102004044597B3 (de) * 2004-09-13 2006-02-02 Forschungszentrum Jülich GmbH Verfahren zur Herstellung dünner, dichter Keramikschichten
CA2582312C (en) 2006-05-05 2014-05-13 Sulzer Metco Ag A method for the manufacture of a coating
DE102006062378A1 (de) * 2006-12-22 2008-06-26 Deutsches Zentrum für Luft- und Raumfahrt e.V. Verfahren zur Herstellung einer elektrochemischen Funktionsstruktur und Funktionsstruktur
DE102007026233A1 (de) * 2007-05-31 2008-12-04 Deutsches Zentrum für Luft- und Raumfahrt e.V. Verfahren zur Herstellung einer gasdichten Festelektrolytschicht und Festelektrolytschicht
US8029870B2 (en) * 2008-03-24 2011-10-04 GM Global Technology Operations LLC Method of coating fuel cell components for water removal
TWI373880B (en) 2008-10-16 2012-10-01 Iner Aec Executive Yuan Solid oxide fuel cell and manufacture method thereof
CN109475885B (zh) * 2016-05-27 2022-03-08 欧瑞康美科股份公司，沃伦 覆层方法、热覆层以及具有热覆层的缸
US11611097B2 (en) 2018-11-06 2023-03-21 Utility Global, Inc. Method of making an electrochemical reactor via sintering inorganic dry particles
US11539053B2 (en) 2018-11-12 2022-12-27 Utility Global, Inc. Method of making copper electrode
US11603324B2 (en) 2018-11-06 2023-03-14 Utility Global, Inc. Channeled electrodes and method of making
US11761100B2 (en) 2018-11-06 2023-09-19 Utility Global, Inc. Electrochemical device and method of making
US20200176803A1 (en) 2018-11-06 2020-06-04 Utility Global, Inc. Method of Making Fuel Cells and a Fuel Cell Stack

Citations (7)

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Publication number Priority date Publication date Assignee Title
JPS63450A (ja) * 1986-06-20 1988-01-05 Mitsubishi Heavy Ind Ltd 固体電解質の形成方法
EP0588597A1 (de) * 1992-09-18 1994-03-23 Ngk Insulators, Ltd. Festoxid-Brennstoffzellen und Verfahren zur Herstellung
FR2729400A1 (fr) * 1995-01-18 1996-07-19 Univ Paris Curie Procede et dispositif pour deposer une couche mince d'oxyde metallique, materiau ainsi obtenu, et element de pile a combustible incluant ce materiau
JPH08293310A (ja) * 1995-04-20 1996-11-05 Tokyo Gas Co Ltd 固体電解質膜の製造方法
JPH10255825A (ja) * 1997-03-07 1998-09-25 Tokyo Gas Co Ltd 固体電解質薄膜とその製造方法
JPH10294115A (ja) * 1997-04-21 1998-11-04 Tokyo Gas Co Ltd 固体電解質薄膜とその製造方法
US5853815A (en) * 1994-08-18 1998-12-29 Sulzer Metco Ag Method of forming uniform thin coatings on large substrates

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JPS61198570A (ja) * 1985-02-28 1986-09-02 Mitsubishi Heavy Ind Ltd 固体電解質燃料電池の製造方法
US4629537A (en) * 1985-05-17 1986-12-16 Hsu Michael S Compact, light-weight, solid-oxide electrochemical converter
JP2572883B2 (ja) * 1990-09-04 1997-01-16 日本碍子株式会社 固体電解質膜及びこれを有する固体電解質型燃料電池、並びにこれらの製造方法
JPH04118861A (ja) * 1990-09-10 1992-04-20 Fuji Electric Co Ltd 固体電解質型燃料電池およびその製造方法
JPH053037A (ja) * 1990-10-03 1993-01-08 Fuji Electric Co Ltd 固体電解質型燃料電池
US5342703A (en) * 1991-07-19 1994-08-30 Ngk Insulators, Ltd. Solid electrolyte type fuel cell and method for producing the same
JPH0693404A (ja) * 1991-12-04 1994-04-05 Ngk Insulators Ltd ランタンクロマイト膜の製造方法およびランタンクロマイト膜
US5527633A (en) * 1992-09-17 1996-06-18 Ngk Insulators, Ltd. Solid oxide fuel cells, a process for producing solid electrolyte films and a process for producing solid oxide fuel cells
US5391440A (en) * 1994-02-14 1995-02-21 Westinghouse Electric Corporation Method of forming a leak proof plasma sprayed interconnection layer on an electrode of an electrochemical cell
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DE19609418C2 (de) 1996-03-11 1998-08-13 Forschungszentrum Juelich Gmbh Beschichtung von porösen Elektroden mit dünnen Elektrolytschichten
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Patent Citations (7)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPS63450A (ja) * 1986-06-20 1988-01-05 Mitsubishi Heavy Ind Ltd 固体電解質の形成方法
EP0588597A1 (de) * 1992-09-18 1994-03-23 Ngk Insulators, Ltd. Festoxid-Brennstoffzellen und Verfahren zur Herstellung
US5853815A (en) * 1994-08-18 1998-12-29 Sulzer Metco Ag Method of forming uniform thin coatings on large substrates
FR2729400A1 (fr) * 1995-01-18 1996-07-19 Univ Paris Curie Procede et dispositif pour deposer une couche mince d'oxyde metallique, materiau ainsi obtenu, et element de pile a combustible incluant ce materiau
JPH08293310A (ja) * 1995-04-20 1996-11-05 Tokyo Gas Co Ltd 固体電解質膜の製造方法
JPH10255825A (ja) * 1997-03-07 1998-09-25 Tokyo Gas Co Ltd 固体電解質薄膜とその製造方法
JPH10294115A (ja) * 1997-04-21 1998-11-04 Tokyo Gas Co Ltd 固体電解質薄膜とその製造方法

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Also Published As

Publication number Publication date
AU2001282121A1 (en) 2002-03-13
US20040076866A1 (en) 2004-04-22
US7141271B2 (en) 2006-11-28
EP1344272A2 (de) 2003-09-17
WO2002019455A2 (de) 2002-03-07

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