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US4278522A - Apparatus for treating contaminated water - Google Patents

Apparatus for treating contaminated water Download PDF

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Publication number
US4278522A
US4278522A US06/049,065 US4906579A US4278522A US 4278522 A US4278522 A US 4278522A US 4906579 A US4906579 A US 4906579A US 4278522 A US4278522 A US 4278522A
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United States
Prior art keywords
electrodes
cathode
cathode electrodes
anode
anode electrode
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Expired - Lifetime
Application number
US06/049,065
Inventor
Gernot Jacob
Luciano Pelloni
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BBC Brown Boveri AG Switzerland
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BBC Brown Boveri AG Switzerland
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Assigned to BBC BROWN, BOVERI & COMPANY, LIMITED reassignment BBC BROWN, BOVERI & COMPANY, LIMITED ASSIGNMENT OF ASSIGNORS INTEREST. Assignors: PELLONI LUCIANO, JACOB GERNOT
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    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F1/00Treatment of water, waste water, or sewage
    • C02F1/46Treatment of water, waste water, or sewage by electrochemical methods
    • C02F1/461Treatment of water, waste water, or sewage by electrochemical methods by electrolysis
    • C02F1/465Treatment of water, waste water, or sewage by electrochemical methods by electrolysis by electroflotation
    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F1/00Treatment of water, waste water, or sewage
    • C02F1/46Treatment of water, waste water, or sewage by electrochemical methods
    • C02F1/461Treatment of water, waste water, or sewage by electrochemical methods by electrolysis
    • C02F1/46104Devices therefor; Their operating or servicing
    • C02F1/46109Electrodes
    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F1/00Treatment of water, waste water, or sewage
    • C02F1/46Treatment of water, waste water, or sewage by electrochemical methods
    • C02F1/461Treatment of water, waste water, or sewage by electrochemical methods by electrolysis
    • C02F1/46104Devices therefor; Their operating or servicing
    • C02F1/46109Electrodes
    • C02F2001/46133Electrodes characterised by the material
    • CCHEMISTRY; METALLURGY
    • C02TREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02FTREATMENT OF WATER, WASTE WATER, SEWAGE, OR SLUDGE
    • C02F2201/00Apparatus for treatment of water, waste water or sewage
    • C02F2201/46Apparatus for electrochemical processes
    • C02F2201/461Electrolysis apparatus
    • C02F2201/46105Details relating to the electrolytic devices
    • C02F2201/4612Controlling or monitoring
    • C02F2201/4615Time

Definitions

  • the present invention relates to a device for treating contaminated water by means of electroflotation wherein cathode electrodes are arranged above anode electrodes.
  • the present invention also relates to a process for operating a device of this type.
  • the electrodes and in particular the cathode electrodes, must be cleaned approximately every 2 weeks. This is due to the fact that the effluent is almost always calcareous and extensive lime deposits form on the cathode electrodes. As the deposits form, the energy consumption of the device increases steadily since the voltage must be raised continuously in order to ensure constant current through the electrodes. To clean these known flotation cells, the cells must be emptied and the electrodes must be taken out.
  • a pair of cathode electrodes are associated with each anode electrode.
  • the cathodes of each pair are alternately supplied with a negative potential.
  • Each cathode is cleaned by the action of the carbonic acid present in the water during the time period in which no negative potential is applied thereto.
  • each of the anode and cathode electrodes are elongated and cylindrical in shape and are arranged to form a grid-like screen. Every other cathode electrode is connected to a respective conductor bar, to facilitate the application of the negative potential alternately to one electrode in each pair of cathode electrodes.
  • the switching of the negative potential from one cathode electrode to the other in each pair can be carried out by means of a timer which carries out the switching operation at fixed time intervals.
  • the switching can be carried out in response to an increase of the applied voltage over a predetermined value or a decrease in the electrode current below a predetermined value.
  • FIG. 1 diagrammatically illustrates the side view of several anode electrodes and cathode electrodes with the appropriate electrical connections;
  • FIG. 2 is a plan view of a grid-like arrangement of several rod-shaped cathode electrodes.
  • each anode electrode 1 is associated with two cathode electrodes 2, 2'.
  • the mean spacing D between the anode electrodes and the cathode electrodes can be, for example, 10 mm. It should be noted, however, that with increasing spacing D the voltage applied between the anode electrodes and cathode electrodes must also increase in order to maintain the required current density for the electrolysis process, for example 1-1.5 A/dm 2 .
  • the diameter of the electrodes can be advantageously selected such that the surface area of the anode electrodes is at least equal to, and preferably twice the surface area of the cathode electrodes.
  • Anode electrodes, having a diameter of about 8 to 10 mm and a mutual spacing of about 5 to 10 mm, and cathode electrodes having a diameter of about 3 to 4 mm have proven to be particularly suitable.
  • Suitable anode materials can be titanium or stainless steel coated with a layer of lead dioxide. Electrodes of this type have an advantage in that they do not dissolve during the electrolysis process.
  • Every second cathode electrode 2 or 2' is connected to a common conductor bar 3 or 3', respectively, as shown in FIGS. 1 and 2.
  • a negative potential is applied in each case to only one of the two conductor bars of each pair, while the other conductor bar in each case is either at zero potential or has a weak positive potential applied thereto. After a certain interval of time, the potentials on the two conductor bars are interchanged by means of a switch device 4.
  • the switch-over of the cathode potentials can be effected with the aid of a time switch (not shown) operating at fixed intervals.
  • constant current units can be used to control the switching operation, wherein the switch-over is initiated in such a way that after a predetermined rise in voltage (and hence a defined fouling of the cathode electrode), a signal U st is automatically applied to a switch-over relay 5, to carry out the switching operation.
  • a drop in current due to fouling of the cathodes can trigger the switch-over relay 5 in a similar manner.
  • the fouled electrodes which are not connected to the voltage source are cleaned since the deposits on the electrodes are dissolved as bicarbonates by the carbonic acid dissolved in the water (CaCO 3 +H 2 CO 3 ⁇ Ca ++ +2HCO 3 ).
  • Carbonic acid is virtually always present in the water, or it is formed by the decomposition of bicarbonate on the anode during the electrolysis process.
  • Protons generated in the anode zone also have a dissolving action on the precipitate (CaCO 3 +2H + ⁇ Ca ++ +H 2 O+CO 2 ), provided the distance from the idle cathode is not too large.

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  • Chemical & Material Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • General Chemical & Material Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Hydrology & Water Resources (AREA)
  • Engineering & Computer Science (AREA)
  • Environmental & Geological Engineering (AREA)
  • Water Supply & Treatment (AREA)
  • Organic Chemistry (AREA)
  • Water Treatment By Electricity Or Magnetism (AREA)

Abstract

An electroflotation device for treating contaminated water includes cathode electrodes which are self-cleaning with respect to lime deposits. Each anode electrode of the device is associated with a pair of cathode electrodes. During operation of the device, a negative potential is applied to only one of the two electrodes of each cathode pair, while the other electrode has either a zero potential or a weak positive potential applied thereto. The lime deposit formed on the non-negative electrode is dissolved by the action of the carbonic acid which is present in the water, through the formation of bicarbonates.

Description

BACKGROUND OF THE INVENTION
The present invention relates to a device for treating contaminated water by means of electroflotation wherein cathode electrodes are arranged above anode electrodes. The present invention also relates to a process for operating a device of this type.
Devices for treating contaminated water by means of electroflotation are known, for example, from Norwegian Patent Specification No. 92,995. In these known devices, the anode electrodes and cathode electrodes are located on the bottom of a flotation cell. The gas bubbles formed during electrolysis of the water, particularly hydrogen bubbles, attach themselves to the suspended matter present in the water, giving the suspended matter a relative density lower than that of water and carrying it to the surface. The floating materials are then skimmed from the surface of the water.
In these known devices, the electrodes, and in particular the cathode electrodes, must be cleaned approximately every 2 weeks. This is due to the fact that the effluent is almost always calcareous and extensive lime deposits form on the cathode electrodes. As the deposits form, the energy consumption of the device increases steadily since the voltage must be raised continuously in order to ensure constant current through the electrodes. To clean these known flotation cells, the cells must be emptied and the electrodes must be taken out.
OBJECT AND BRIEF SUMMARY OF THE INVENTION
It is therefore an object of the present invention to provide a novel device for treating contaminated water by means of electroflotation wherein the electrodes are self-cleaning, to thereby reduce the need to empty the flotation cell and to remove the electrodes to clean the cathode electrodes.
It is another object of the present invention to provide a novel process for operating a device of this type.
In accordance with the present invention, a pair of cathode electrodes are associated with each anode electrode. The cathodes of each pair are alternately supplied with a negative potential. Each cathode is cleaned by the action of the carbonic acid present in the water during the time period in which no negative potential is applied thereto.
In accordance with a further feature of the present invention, each of the anode and cathode electrodes are elongated and cylindrical in shape and are arranged to form a grid-like screen. Every other cathode electrode is connected to a respective conductor bar, to facilitate the application of the negative potential alternately to one electrode in each pair of cathode electrodes.
The switching of the negative potential from one cathode electrode to the other in each pair can be carried out by means of a timer which carries out the switching operation at fixed time intervals. Alternatively, the switching can be carried out in response to an increase of the applied voltage over a predetermined value or a decrease in the electrode current below a predetermined value.
BRIEF DESCRIPTION OF THE DRAWINGS
Further advantages of the present invention are explained in the following text by reference to illustrative embodiments and in conjunction with accompanying drawings in which:
FIG. 1 diagrammatically illustrates the side view of several anode electrodes and cathode electrodes with the appropriate electrical connections; and
FIG. 2 is a plan view of a grid-like arrangement of several rod-shaped cathode electrodes.
DETAILED DESCRIPTION
The arrangement of the anode electrodes and cathode electrodes of a flotation cell is reproduced diagrammatically in FIG. 1. Each anode electrode 1 is associated with two cathode electrodes 2, 2'. The mean spacing D between the anode electrodes and the cathode electrodes can be, for example, 10 mm. It should be noted, however, that with increasing spacing D the voltage applied between the anode electrodes and cathode electrodes must also increase in order to maintain the required current density for the electrolysis process, for example 1-1.5 A/dm2.
An electrical field distribution which is advantageous for the electrolysis process is obtained when the electrode rods 1, 2, 2' have a cylindrical shape. The diameter of the electrodes can be advantageously selected such that the surface area of the anode electrodes is at least equal to, and preferably twice the surface area of the cathode electrodes. Anode electrodes, having a diameter of about 8 to 10 mm and a mutual spacing of about 5 to 10 mm, and cathode electrodes having a diameter of about 3 to 4 mm have proven to be particularly suitable.
Suitable anode materials can be titanium or stainless steel coated with a layer of lead dioxide. Electrodes of this type have an advantage in that they do not dissolve during the electrolysis process.
Every second cathode electrode 2 or 2' is connected to a common conductor bar 3 or 3', respectively, as shown in FIGS. 1 and 2. A negative potential is applied in each case to only one of the two conductor bars of each pair, while the other conductor bar in each case is either at zero potential or has a weak positive potential applied thereto. After a certain interval of time, the potentials on the two conductor bars are interchanged by means of a switch device 4.
The switch-over of the cathode potentials can be effected with the aid of a time switch (not shown) operating at fixed intervals. Alternatively, constant current units can be used to control the switching operation, wherein the switch-over is initiated in such a way that after a predetermined rise in voltage (and hence a defined fouling of the cathode electrode), a signal Ust is automatically applied to a switch-over relay 5, to carry out the switching operation. In constant voltage units, a drop in current due to fouling of the cathodes can trigger the switch-over relay 5 in a similar manner.
The fouled electrodes which are not connected to the voltage source are cleaned since the deposits on the electrodes are dissolved as bicarbonates by the carbonic acid dissolved in the water (CaCO3 +H2 CO3 →Ca++ +2HCO3). Carbonic acid is virtually always present in the water, or it is formed by the decomposition of bicarbonate on the anode during the electrolysis process. Protons generated in the anode zone also have a dissolving action on the precipitate (CaCO3 +2H+ →Ca++ +H2 O+CO2), provided the distance from the idle cathode is not too large.
In one application of the present invention using a flotation cell having an active cell capacity of 17 liters and using a screen-like cathode grid constructed as shown in FIG. 2, water having a total hardness of 22d and a carbonate hardness of 18d had its carbonate hardness reduced by 17d with a water throughput of 60 liters/hour. Considerable amounts of calcium carbonate flaked off the cathode rods which were potential-free and fell to the bottom. The calcium carbonate was detached substantially more rapidly when current was passing through the other cathode electrode than only in running water alone, i.e. without electrolysis. At a constant voltage of 21.5 V with a current density of 1.2 A/dm2, the current did not fall for a period of about 120 hours. The potentials were switched over between cathodes every 30 minutes. If, however, the unit was operated in the known manner, i.e. the same negative potential was applied to all the cathode rods 2, 2', the current fell after 24 hours from an initial value of 10 A to 6 A.
The present invention may be embodied in other specific forms without departing from the spirit or essential characteristics thereof. The presently disclosed embodiment is therefore considered in all respects as illustrative and not restrictive. The scope of the invention is indicated by the appended claims rather than the foregoing description, and all changes which come within the meaning and range of equivalency of the claims are therefore intended to be embraced therein.

Claims (5)

What is claimed is:
1. Apparatus for treating contaminated water by means of electroflotation; comprising:
a multiplicity of positively biased anode electrodes each having a cylindrical shape;
a pair of cylindrically shaped cathode electrodes respectively associated with each anode electrode said cathode and anode electrodes forming a grid-like screen, further wherein every second cathode electrode in said screen is connected to a common conductor bar; and
means for alternately applying a negative potential to only one of the cathode electrodes in each pair of cathode electrodes while maintaining the other of said cathode electrodes at a non-negative potential.
2. Apparatus according to claim 1, wherein the anode electrode consists of titanium provided with a coating of lead dioxide.
3. Apparatus according to claim 1, wherein the anode electrode consists of stainless steel provided with a coating of lead dioxide.
4. Apparatus according to claim 1, wherein the surface area of the anode electrode is at least equal to the surface area of each of the cathode electrodes.
5. Apparatus according to claim 4, wherein the surface area of the anode electrode is twice the surface area of each of the cathode electrodes.
US06/049,065 1978-08-23 1979-06-18 Apparatus for treating contaminated water Expired - Lifetime US4278522A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CH891378A CH631951A5 (en) 1978-08-23 1978-08-23 DEVICE FOR TREATING POLLUTED WATER AND METHOD FOR OPERATING SUCH A DEVICE.
CH8913/78 1978-08-23

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US4278522A true US4278522A (en) 1981-07-14

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US (1) US4278522A (en)
BE (1) BE878346A (en)
CH (1) CH631951A5 (en)
DE (1) DE2838502A1 (en)
GB (1) GB2028298B (en)
NL (1) NL7906328A (en)

Cited By (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4772369A (en) * 1984-08-24 1988-09-20 Dominique Mercier Electromagnetic treatment of water
CN103408111A (en) * 2013-07-05 2013-11-27 北京仁创科技集团有限公司 Pervious electrode plate with sterilization effect and preparation method thereof
US9540257B2 (en) 2014-11-17 2017-01-10 Drexel University Plasma spark discharge reactor and durable electrode
US10167209B2 (en) 2014-12-01 2019-01-01 Drexel Univerisity System and method for disinfection and fouling prevention in the treatment of water

Families Citing this family (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE3808393A1 (en) * 1988-03-12 1989-09-21 Westfael Elekt Werke METHOD FOR THE ELECTROCHEMICAL TREATMENT OF WATER
DE3837628A1 (en) * 1988-11-05 1990-05-10 Broesamle Peter METHOD AND DEVICE FOR TREATING ORGANIC SLUDGE
CN103408109B (en) * 2013-06-27 2014-08-13 北京仁创科技集团有限公司 Water permeable battery lead plate and preparation method thereof
CN111855754B (en) * 2019-04-29 2021-12-03 深圳安吉尔饮水产业集团有限公司 Water hardness detection probe, sensor, detection method and water softener

Citations (15)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US1183753A (en) * 1915-07-08 1916-05-16 Walter E Fuller Water-purifier.
US2773025A (en) * 1953-09-10 1956-12-04 Westinghouse Electric Corp Destroying cyanides in aqueous cyanide solutions
US2872405A (en) * 1955-12-14 1959-02-03 Pennsalt Chemicals Corp Lead dioxide electrode
US3207679A (en) * 1960-05-03 1965-09-21 American Potash & Chem Corp Method for electroplating on titanium
US3249520A (en) * 1961-02-17 1966-05-03 Coussinets Ste Indle Process of providing an electrolytic deposit on a face of a workpiece
US3463707A (en) * 1965-06-16 1969-08-26 Pacific Eng & Production Co Electrodeposition of lead dioxide
US3632498A (en) * 1967-02-10 1972-01-04 Chemnor Ag Electrode and coating therefor
US3793173A (en) * 1969-02-03 1974-02-19 K Price Wastewater treatment using electrolysis with activated carbon cathode
US3800286A (en) * 1972-08-24 1974-03-26 Honeywell Inf Systems Address development technique utilizing a content addressable memory
US3813321A (en) * 1973-06-28 1974-05-28 S Bastacky Process for treating industrial wastes
US3969216A (en) * 1974-12-27 1976-07-13 Doreen Veronica Barrett Flotation separation
US4000056A (en) * 1973-10-01 1976-12-28 Electrolyte Services Ltd. Apparatus for electrolytic metal recovery
US4036716A (en) * 1974-04-05 1977-07-19 Goteborgs Analyslaboratorium Ab Method to prevent the formation of incrustations on working electrodes in electrode steam generators or the like and a means for performing the method
US4038170A (en) * 1976-03-01 1977-07-26 Rhees Raymond C Anode containing lead dioxide deposit and process of production
US4064035A (en) * 1975-08-07 1977-12-20 Agency Of Industrial Science & Technology Lead dioxide electrode

Patent Citations (15)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US1183753A (en) * 1915-07-08 1916-05-16 Walter E Fuller Water-purifier.
US2773025A (en) * 1953-09-10 1956-12-04 Westinghouse Electric Corp Destroying cyanides in aqueous cyanide solutions
US2872405A (en) * 1955-12-14 1959-02-03 Pennsalt Chemicals Corp Lead dioxide electrode
US3207679A (en) * 1960-05-03 1965-09-21 American Potash & Chem Corp Method for electroplating on titanium
US3249520A (en) * 1961-02-17 1966-05-03 Coussinets Ste Indle Process of providing an electrolytic deposit on a face of a workpiece
US3463707A (en) * 1965-06-16 1969-08-26 Pacific Eng & Production Co Electrodeposition of lead dioxide
US3632498A (en) * 1967-02-10 1972-01-04 Chemnor Ag Electrode and coating therefor
US3793173A (en) * 1969-02-03 1974-02-19 K Price Wastewater treatment using electrolysis with activated carbon cathode
US3800286A (en) * 1972-08-24 1974-03-26 Honeywell Inf Systems Address development technique utilizing a content addressable memory
US3813321A (en) * 1973-06-28 1974-05-28 S Bastacky Process for treating industrial wastes
US4000056A (en) * 1973-10-01 1976-12-28 Electrolyte Services Ltd. Apparatus for electrolytic metal recovery
US4036716A (en) * 1974-04-05 1977-07-19 Goteborgs Analyslaboratorium Ab Method to prevent the formation of incrustations on working electrodes in electrode steam generators or the like and a means for performing the method
US3969216A (en) * 1974-12-27 1976-07-13 Doreen Veronica Barrett Flotation separation
US4064035A (en) * 1975-08-07 1977-12-20 Agency Of Industrial Science & Technology Lead dioxide electrode
US4038170A (en) * 1976-03-01 1977-07-26 Rhees Raymond C Anode containing lead dioxide deposit and process of production

Cited By (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US4772369A (en) * 1984-08-24 1988-09-20 Dominique Mercier Electromagnetic treatment of water
CN103408111A (en) * 2013-07-05 2013-11-27 北京仁创科技集团有限公司 Pervious electrode plate with sterilization effect and preparation method thereof
US9540257B2 (en) 2014-11-17 2017-01-10 Drexel University Plasma spark discharge reactor and durable electrode
US10167209B2 (en) 2014-12-01 2019-01-01 Drexel Univerisity System and method for disinfection and fouling prevention in the treatment of water

Also Published As

Publication number Publication date
GB2028298A (en) 1980-03-05
GB2028298B (en) 1982-11-03
BE878346A (en) 1979-12-17
NL7906328A (en) 1980-02-26
DE2838502A1 (en) 1980-03-06
CH631951A5 (en) 1982-09-15

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Owner name: BBC BROWN ,BOVERI & COMPANY, LIMITED, BADEN, SWIT

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