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US20040040637A1 - Flash-ignitable energetic material - Google Patents

Flash-ignitable energetic material Download PDF

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Publication number
US20040040637A1
US20040040637A1 US10/617,134 US61713403A US2004040637A1 US 20040040637 A1 US20040040637 A1 US 20040040637A1 US 61713403 A US61713403 A US 61713403A US 2004040637 A1 US2004040637 A1 US 2004040637A1
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US
United States
Prior art keywords
weight percent
composition
energetic material
carbon nanotubes
energetic
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Abandoned
Application number
US10/617,134
Inventor
Sylvain Desilets
Patric Brousseau
Nicole Gagnon
Sebastien Cote
Serge Trudel
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Individual
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Individual
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
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Publication date
Application filed by Individual filed Critical Individual
Priority to US10/617,134 priority Critical patent/US20040040637A1/en
Publication of US20040040637A1 publication Critical patent/US20040040637A1/en
Priority to US11/444,464 priority patent/US20070039671A1/en
Priority to US11/798,693 priority patent/US20080066835A1/en
Abandoned legal-status Critical Current

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Classifications

    • CCHEMISTRY; METALLURGY
    • C06EXPLOSIVES; MATCHES
    • C06BEXPLOSIVES OR THERMIC COMPOSITIONS; MANUFACTURE THEREOF; USE OF SINGLE SUBSTANCES AS EXPLOSIVES
    • C06B23/00Compositions characterised by non-explosive or non-thermic constituents
    • C06B23/001Fillers, gelling and thickening agents (e.g. fibres), absorbents for nitroglycerine
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B82NANOTECHNOLOGY
    • B82YSPECIFIC USES OR APPLICATIONS OF NANOSTRUCTURES; MEASUREMENT OR ANALYSIS OF NANOSTRUCTURES; MANUFACTURE OR TREATMENT OF NANOSTRUCTURES
    • B82Y30/00Nanotechnology for materials or surface science, e.g. nanocomposites
    • CCHEMISTRY; METALLURGY
    • C06EXPLOSIVES; MATCHES
    • C06BEXPLOSIVES OR THERMIC COMPOSITIONS; MANUFACTURE THEREOF; USE OF SINGLE SUBSTANCES AS EXPLOSIVES
    • C06B23/00Compositions characterised by non-explosive or non-thermic constituents
    • C06B23/002Sensitisers or density reducing agents, foam stabilisers, crystal habit modifiers
    • CCHEMISTRY; METALLURGY
    • C06EXPLOSIVES; MATCHES
    • C06BEXPLOSIVES OR THERMIC COMPOSITIONS; MANUFACTURE THEREOF; USE OF SINGLE SUBSTANCES AS EXPLOSIVES
    • C06B43/00Compositions characterised by explosive or thermic constituents not provided for in groups C06B25/00 - C06B41/00
    • CCHEMISTRY; METALLURGY
    • C06EXPLOSIVES; MATCHES
    • C06BEXPLOSIVES OR THERMIC COMPOSITIONS; MANUFACTURE THEREOF; USE OF SINGLE SUBSTANCES AS EXPLOSIVES
    • C06B45/00Compositions or products which are defined by structure or arrangement of component of product
    • CCHEMISTRY; METALLURGY
    • C06EXPLOSIVES; MATCHES
    • C06CDETONATING OR PRIMING DEVICES; FUSES; CHEMICAL LIGHTERS; PYROPHORIC COMPOSITIONS
    • C06C9/00Chemical contact igniters; Chemical lighters

Definitions

  • This invention relates to a light ignitable, energetic materials. More specifically, the invention relates to light ignitable, energetic materials containing carbon nanotubes or activated carbon containing a metal.
  • a carbon nanotube is a hollow nanostructure consisting essentially of a graphitic plane rolled into a thin tube, both ends of which can be closed by a fullerene-type dome structure.
  • CNT carbon nanotube
  • SWNT single walled nanotubes
  • MWNT multiwalled nanotubes
  • the object of the present invention is to exploit the above described property of carbon nanotubes and activated carbon containing a metal to produce a light ignitable, energetic material.
  • a variety of energetic materials can be used in the method of the present invention.
  • Such energetic materials include carbon black powder, ammonium perchlorate (AP), hexogen (RDX), octogen (HMX), pentaerythritol tetranitrate, (PETN), trinitrotoluene (TNT), nitroglycerine, nitrocellulose, ammonium nitrate, lead azide, lead styphnate, nitro plasticizers and picric acid.
  • AP ammonium perchlorate
  • RDX hexogen
  • HMX octogen
  • PETN pentaerythritol tetranitrate
  • PET pentaerythritol tetranitrate
  • TNT trinitrotoluene
  • nitroglycerine nitrocellulose
  • ammonium nitrate lead azide
  • lead styphnate nitro plasticizers and picric acid.
  • the carbon nanotubes can be
  • the invention takes advantage of the photoacoustic effect of carbon nanotubes when subjected to a burst of light, e.g. a camera flash to ignite an energetic material.
  • a burst of light e.g. a camera flash
  • different carbon nanotubes were used, the most common one being a SWNT commercial available from Carbon Nanotechnologies, Inc., Houston, Tex.
  • Different percentages of carbon nanotubes (1-90 weight percent) were manually mixed (gently) with carbon black powder.
  • the most efficient composition contained 5 weight percent SWNT mixed with 95 weight percent Grade 7 carbon black powder.
  • the composition exploded instantaneously after being subjected to a camera flash. It was found that carbon black powder with the smallest particle size was the most effective.
  • activated carbon containing a metal e.g. palladium was mixed with carbon black powder, and the resulting mixture was exposed to a camera flash.
  • Example 1 The procedure of Example 1 was repeated using 3%, 5%, 10% and 20% carbon nanotubes. At a concentration in excess of 20% nanotubes, the ignition phenomenon was less efficient, i.e. the combustion process (explosion) appears to be incomplete.
  • Example 1 The method of Example 1 was repeated using 5 weight percent activated carbon containing palladium (97% carbon and 3% palladium) with 95 weight percent ground ammonium perchlorate. The mixture was homogenized using the same ball milling equipment as in Example 1. The composition was ignited using a flash; however, the process was less efficient than when using carbon nanotubes.
  • the ignition effect was observed for a variety of mixtures of activated carbon containing 3-30% palladium catalyst and a variety of energetic materials. The ignition effect was similar to that observed when using carbon nanotubes, but seemed to be less efficient after 3 to 5 days. It is believed that the activated carbon was absorbing water which reduced the efficiency of the ignition phenomenon.
  • compositions in accordance with the present invention can be used for light ignited pyrotechnic effects and as light ignited triggers for detonators, gas generators and air bags.

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Nanotechnology (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Physics & Mathematics (AREA)
  • Condensed Matter Physics & Semiconductors (AREA)
  • General Physics & Mathematics (AREA)
  • Materials Engineering (AREA)
  • Composite Materials (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Carbon And Carbon Compounds (AREA)
  • Medicinal Preparation (AREA)

Abstract

Carbon nanotubes and activated carbon containing a metal such as palladium release a photoacoustic effect when subjected to a flash of light. A light ignitable, energetic composition is produced by mixing one of them with an energetic material such as carbon black powder or ammonium perchlorate.

Description

    BACKGROUND OF THE INVENTION
  • 1. Field of the Invention [0001]
  • This invention relates to a light ignitable, energetic materials. More specifically, the invention relates to light ignitable, energetic materials containing carbon nanotubes or activated carbon containing a metal. [0002]
  • 2. Discussion of the Prior Art [0003]
  • A carbon nanotube (CNT) is a hollow nanostructure consisting essentially of a graphitic plane rolled into a thin tube, both ends of which can be closed by a fullerene-type dome structure. The existence of CNT's was originally discovered by S. Iijima [see Nature 354, 56 (1991)]. The material exhibits various interesting mechanical and electrical properties. There exists two forms of carbon nanotubes, namely single walled nanotubes (SWNT) and multiwalled nanotubes (MWNT). [0004]
  • It has recently been reported by P. M. Ajayan et al in Science, Vol. 296, 705 (2002) that carbon nanotubes release a large photoacoustic effect when sujected to a flash of light caused by the absorption of the light. It seems that the phenomenon is predominantly present in SWNT's and that the temperature of the process can reach 1500° C. The inventors have also determined that activated carbon containing a metal such as palladium also possesses the property of releasing a photoacoustic effect when subjected to a flash of light. [0005]
  • GENERAL DESCRIPTION OF THE INVENTION
  • The object of the present invention is to exploit the above described property of carbon nanotubes and activated carbon containing a metal to produce a light ignitable, energetic material. [0006]
  • Accordingly, the present invention relates to a light ignitable, energetic composition comprising an intimate mixture of an energetic material and one of carbon nanotubes and activated carbon containing a metal selected from the group consisting of palladium, iron, nickel, cobalt, aluminum, copper, zinc, potassium, sodium and titanium. [0007]
  • The invention also relates to a method of preparing a light ignitable, energetic composition comprising intimately mixing an energetic material and one of carbon nanotubes and activated carbon containing a metal selected from the group consisting of palladium, iron, nickel, cobalt, aluminum, copper, zinc, potassium, sodium and titanium. [0008]
  • A variety of energetic materials can be used in the method of the present invention. Such energetic materials include carbon black powder, ammonium perchlorate (AP), hexogen (RDX), octogen (HMX), pentaerythritol tetranitrate, (PETN), trinitrotoluene (TNT), nitroglycerine, nitrocellulose, ammonium nitrate, lead azide, lead styphnate, nitro plasticizers and picric acid. While the carbon nanotubes can be SWNT or MWNT, the single walled nanotubes are preferred. [0009]
  • DESCRIPTION OF THE PREFERRED EMBODIMENT
  • In general terms, the invention takes advantage of the photoacoustic effect of carbon nanotubes when subjected to a burst of light, e.g. a camera flash to ignite an energetic material. In order to test the theory, different carbon nanotubes were used, the most common one being a SWNT commercial available from Carbon Nanotechnologies, Inc., Houston, Tex. Different percentages of carbon nanotubes (1-90 weight percent) were manually mixed (gently) with carbon black powder. Initially, the most efficient composition contained 5 weight percent SWNT mixed with 95 weight percent Grade 7 carbon black powder. The composition exploded instantaneously after being subjected to a camera flash. It was found that carbon black powder with the smallest particle size was the most effective. The same effect was observed when activated carbon containing a metal, e.g. palladium was mixed with carbon black powder, and the resulting mixture was exposed to a camera flash. [0010]
  • The invention will be better understood from the following examples.[0011]
  • EXAMPLE 1
  • 3 weight percent of crude carbon nanotubes were mixed with 97 weight percent ground ammonium perchlorate. The mixture was homogenized using ball milling equipment for 15 minutes. The balls used in the mill were made of glass. The resulting composition was then exposed to an intense flash using a commercially available Vivitar (trademark) flash. The power of the flash was 200W/cm[0012] 2 at a distance of 4.5 cm.
  • EXAMPLE 2
  • The procedure of Example 1 was repeated using 3%, 5%, 10% and 20% carbon nanotubes. At a concentration in excess of 20% nanotubes, the ignition phenomenon was less efficient, i.e. the combustion process (explosion) appears to be incomplete. [0013]
  • EXAMPLE 3
  • Energetic formulations containing carbon nanotubes and RDX, TNT, black powder or AP were ignited at distances from 3 to 7 cm using the Vivitar flash. In a few cases, ignition was possible from a distance as great as 14 cm. [0014]
  • EXAMPLE 4
  • The method of Example 1 was repeated using 5 weight percent activated carbon containing palladium (97% carbon and 3% palladium) with 95 weight percent ground ammonium perchlorate. The mixture was homogenized using the same ball milling equipment as in Example 1. The composition was ignited using a flash; however, the process was less efficient than when using carbon nanotubes. [0015]
  • EXAMPLE 5
  • The ignition effect was observed for a variety of mixtures of activated carbon containing 3-30% palladium catalyst and a variety of energetic materials. The ignition effect was similar to that observed when using carbon nanotubes, but seemed to be less efficient after 3 to 5 days. It is believed that the activated carbon was absorbing water which reduced the efficiency of the ignition phenomenon. [0016]
  • Compositions in accordance with the present invention can be used for light ignited pyrotechnic effects and as light ignited triggers for detonators, gas generators and air bags. [0017]
  • Various modifications may be made to the described embodiments without departing from the spirit and scope of the invention as defined in the appended claims. [0018]

Claims (15)

1. A light ignitable, energetic composition comprising an intimate mixture of an energetic material and one of carbon nanotubes and activated carbon containing a metal selected from the group consisting of palladium, iron, nickel, cobalt, aluminum, copper, zinc, potassium, sodium and titanium.
2. The composition of claim 1, wherein the energetic material is selected from the group consisting of carbon black powder, ammonium perchlorate, hexogen, octogen, pentaerythritol tetranitrate, trinitrotolune, nitroglycerine, nitrocellulose, ammonium nitrate, lead azide, lead styphnate, nitro plasticizers and picric acid.
3. The composition of claim 2, wherein the mixture contains an energetic material and single walled carbon nanotubes.
4. The composition of claim 3, wherein the mixture contains 1 to 20 weight percent carbon nanotubes, the remainder being the energetic material.
5. The composition of claim 3, wherein the mixture contains 95 weight percent of the energetic material and 5 weight percent carbon nanotubes.
6. The composition of claim 4, wherein the mixture contains 95 weight percent carbon black powder and 5 weight percent carbon nanotubes.
7. The composition of claim 3, wherein the energetic material is ammonium perchlorate.
8. The composition of claim 7, wherein the mixture contains 97 weight percent ammonium perchlorate and 3 weight percent carbon nanotubes.
9. The composition of claim 7, wherein the mixture contains 95 weight percent of ground ammonium perchlorate and 5 weight percent of activated carbon containing 97 weight percent carbon and 3 weight percent palladium.
10. A method of preparing a light ignitable, energetic composition comprising intimately mixing an energetic material and one of carbon nanotubes and activated carbon containing a metal selected from the group consisting of palladium, iron nickel, cobalt, aluminum, copper, zinc, potassium, sodium and titanium.
11. The method of claim 10, wherein the energetic material is selected from the group consisting of carbon black powder, ammonium perchlorate, hexogen, octogen, pentaerythritol tetranitrate, trinitrotolune, nitroglycerine, nitrocellulose, ammonium nitrate, lead azide, lead styphnate, nitro plasticizers and picric acid.
12. The method of claim 11, wherein single walled carbon nanotubes are mixed with the energetic material.
13. The method of claim 12, wherein the energetic material is ammonium perchlorate.
14. The method of claim 12, wherein the energetic material is carbon black powder.
15. The method of claim 11, wherein ground ammonium perchlorate is mixed with activated carbon containing palladium.
US10/617,134 2002-07-11 2003-07-11 Flash-ignitable energetic material Abandoned US20040040637A1 (en)

Priority Applications (3)

Application Number Priority Date Filing Date Title
US10/617,134 US20040040637A1 (en) 2002-07-11 2003-07-11 Flash-ignitable energetic material
US11/444,464 US20070039671A1 (en) 2002-07-11 2006-06-01 Flash-ignitable energetic material
US11/798,693 US20080066835A1 (en) 2002-07-11 2007-05-16 Flash-ignitable energetic material

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US39487102P 2002-07-11 2002-07-11
US10/617,134 US20040040637A1 (en) 2002-07-11 2003-07-11 Flash-ignitable energetic material

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US11/798,693 Abandoned US20080066835A1 (en) 2002-07-11 2007-05-16 Flash-ignitable energetic material

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Cited By (15)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US20060011083A1 (en) * 2004-06-30 2006-01-19 Perry William L Microwave heating of energetic materials
US7025840B1 (en) * 2003-07-15 2006-04-11 Lockheed Martin Corporation Explosive/energetic fullerenes
US20080233402A1 (en) * 2006-06-08 2008-09-25 Sid Richardson Carbon & Gasoline Co. Carbon black with attached carbon nanotubes and method of manufacture
US7517215B1 (en) * 2004-07-09 2009-04-14 Erc Incorporated Method for distributed ignition of fuels by light sources
US7833366B1 (en) 2007-10-31 2010-11-16 The United States Of America As Represented By The Secretary Of The Navy Method for making single walled carbon nanotubes by activation with hydrazoic acid
US7879166B1 (en) * 2007-10-31 2011-02-01 The United States Of America As Represented By The Secretary Of The Navy Single walled carbon nanotubes activated with hydrazoic acid
US7896990B1 (en) * 2004-02-20 2011-03-01 The United States Of America As Represented By The Secretary Of The Navy Burn rate nanotube modifiers
US20120291931A1 (en) * 2006-10-16 2012-11-22 Mcdermott Will & Emery Composite compound including explosive and modifier for explosive and method of manufacture thereof
US20140216288A1 (en) * 2013-02-06 2014-08-07 U.S. Army Research Laboratory Attn: Rdrl-Loc-I Carbon nanotube and porous substrate integrated energetic device
KR101471998B1 (en) * 2013-08-09 2014-12-15 부산대학교 산학협력단 Nano Energetic Materials Composite with Explosion in Air and Water via Optical Ignition and Method for Manufacturing the same
WO2015156528A1 (en) * 2014-04-07 2015-10-15 부산대학교 산학협력단 Nano-energetic material composite having remote ignition characteristics by high-power pulse type laser beam and method for preparing same
US9550875B2 (en) 2014-06-18 2017-01-24 Sid Richardson Carbon, Ltd. Nanospike hybrid carbon black
CN111875454A (en) * 2020-07-17 2020-11-03 西安近代化学研究所 Ammonium perchlorate catalyst, preparation method and application
RU2756556C1 (en) * 2020-10-08 2021-10-01 Акционерное общество "Новосибирский механический завод "Искра" Lead trinitroresorcinate modified with carbon nanotubes and method for production thereof
RU2777333C1 (en) * 2021-02-16 2022-08-02 Акционерное общество "Новосибирский механический завод "Искра" Pentaerythritol tetranitrate modified with carbon nanotubes and method for its preparation

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Publication number Priority date Publication date Assignee Title
CA2434859A1 (en) * 2002-07-11 2004-01-11 Her Majesty The Queen In Right Of Canada As Represented By The Minister Of National Defence Of Her Majesty's Canadian Government Flash-ignitable energetic material
US7874250B2 (en) * 2005-02-09 2011-01-25 Schlumberger Technology Corporation Nano-based devices for use in a wellbore
CN105836729B (en) * 2016-04-11 2017-12-05 大连理工大学 The method that Gaseous Detonation method synthesizes iron content CNT

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JP4337254B2 (en) * 2000-09-22 2009-09-30 日油株式会社 Gas generating agent
US6787122B2 (en) * 2001-06-18 2004-09-07 The University Of North Carolina At Chapel Hill Method of making nanotube-based material with enhanced electron field emission properties
CA2434859A1 (en) * 2002-07-11 2004-01-11 Her Majesty The Queen In Right Of Canada As Represented By The Minister Of National Defence Of Her Majesty's Canadian Government Flash-ignitable energetic material

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US3734020A (en) * 1971-10-01 1973-05-22 Us Army Igniter for propelling charges
US20030183504A1 (en) * 2002-02-19 2003-10-02 Rensselaer Polytechnic Institute Method of transforming carbon nanotubes

Cited By (18)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US7025840B1 (en) * 2003-07-15 2006-04-11 Lockheed Martin Corporation Explosive/energetic fullerenes
US7896990B1 (en) * 2004-02-20 2011-03-01 The United States Of America As Represented By The Secretary Of The Navy Burn rate nanotube modifiers
US20060011083A1 (en) * 2004-06-30 2006-01-19 Perry William L Microwave heating of energetic materials
WO2006085956A3 (en) * 2004-06-30 2007-04-12 Univ California Microwave heating of energetic materials
US7517215B1 (en) * 2004-07-09 2009-04-14 Erc Incorporated Method for distributed ignition of fuels by light sources
US7665985B1 (en) * 2004-07-09 2010-02-23 Erc Incorporated Apparatus for distributed ignition of fuels by light sources
US20080233402A1 (en) * 2006-06-08 2008-09-25 Sid Richardson Carbon & Gasoline Co. Carbon black with attached carbon nanotubes and method of manufacture
US20120291931A1 (en) * 2006-10-16 2012-11-22 Mcdermott Will & Emery Composite compound including explosive and modifier for explosive and method of manufacture thereof
US7833366B1 (en) 2007-10-31 2010-11-16 The United States Of America As Represented By The Secretary Of The Navy Method for making single walled carbon nanotubes by activation with hydrazoic acid
US7879166B1 (en) * 2007-10-31 2011-02-01 The United States Of America As Represented By The Secretary Of The Navy Single walled carbon nanotubes activated with hydrazoic acid
US20140216288A1 (en) * 2013-02-06 2014-08-07 U.S. Army Research Laboratory Attn: Rdrl-Loc-I Carbon nanotube and porous substrate integrated energetic device
KR101471998B1 (en) * 2013-08-09 2014-12-15 부산대학교 산학협력단 Nano Energetic Materials Composite with Explosion in Air and Water via Optical Ignition and Method for Manufacturing the same
WO2015156528A1 (en) * 2014-04-07 2015-10-15 부산대학교 산학협력단 Nano-energetic material composite having remote ignition characteristics by high-power pulse type laser beam and method for preparing same
US10252953B2 (en) 2014-04-07 2019-04-09 Pusan National University Industry—University Cooperation Foundation Nanoenergetic material composite having remote ignition characteristic
US9550875B2 (en) 2014-06-18 2017-01-24 Sid Richardson Carbon, Ltd. Nanospike hybrid carbon black
CN111875454A (en) * 2020-07-17 2020-11-03 西安近代化学研究所 Ammonium perchlorate catalyst, preparation method and application
RU2756556C1 (en) * 2020-10-08 2021-10-01 Акционерное общество "Новосибирский механический завод "Искра" Lead trinitroresorcinate modified with carbon nanotubes and method for production thereof
RU2777333C1 (en) * 2021-02-16 2022-08-02 Акционерное общество "Новосибирский механический завод "Искра" Pentaerythritol tetranitrate modified with carbon nanotubes and method for its preparation

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US20070039671A1 (en) 2007-02-22
CA2434859A1 (en) 2004-01-11
US20080066835A1 (en) 2008-03-20

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