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RU2013124424A - Одноконтурное многоступенчатое получение топлива - Google Patents

Одноконтурное многоступенчатое получение топлива Download PDF

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RU2013124424A
RU2013124424A RU2013124424/04A RU2013124424A RU2013124424A RU 2013124424 A RU2013124424 A RU 2013124424A RU 2013124424/04 A RU2013124424/04 A RU 2013124424/04A RU 2013124424 A RU2013124424 A RU 2013124424A RU 2013124424 A RU2013124424 A RU 2013124424A
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reactor
effluent
catalyst
synthesis gas
group
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RU2013124424/04A
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RU2574390C2 (ru
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Говард Л. ФАНЬ
Моше БЕН-РЕВЕН
Ричард Е. БОЙЛ
Роберт М. КОРОС
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Примус Грин Энерджи Инк.
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  • Chemical & Material Sciences (AREA)
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  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Engineering & Computer Science (AREA)
  • General Chemical & Material Sciences (AREA)
  • Crystallography & Structural Chemistry (AREA)
  • Materials Engineering (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
  • Production Of Liquid Hydrocarbon Mixture For Refining Petroleum (AREA)
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Abstract

1. Способ получения топлива из синтез-газа, включающий стадии:а) пропускания синтез-газа через первый реактор с целью конверсии синтез-газа в метанол и воду с образованием первого выходящего потока,б) пропускания первого выходящего потока через второй реактор с целью конверсии метанола в простой диметиловый эфир с образованием второго выходящего потока,в) пропускания второго выходящего потока через третий реактор с целью конверсии метанола и простого диметилового эфира в топливо и тяжелый бензин с образованием третьего выходящего потока,г) пропускания третьего выходящего потока через четвертый реактор с целью конверсии тяжелого бензина в изопарафины, нафтены и ароматические соединения с низкой степенью замещения с образованием четвертого выходящего потока, ид) возвращения непрореагировавшего синтез-газа, содержащегося в четвертом выходящем потоке, в повторный цикл в первый реактор,причем на протяжении способа не осуществляют удаление или отделение первого, второго или третьего выходящих потоков.2. Способ по п.1, в котором первый, второй, третий и четвертый реакторы действуют под давление около 50-100 атмосфер.3. Способ по п.1, в котором топливо содержит по существу C-Cуглеводороды, толуол и ксилол.4. Способ по п.1, в котором тяжелый бензин содержит ароматические соединения ≥C.5. Способ по п.1, в котором температура в первом реакторе составляет около 190-300°C.6. Способ по п.1, в котором в котором температура во втором реакторе составляет около 300-450°C.7. Способ по п.1, в котором в котором температура в третьем реакторе составляет около 300-500°C.8. Способ по п.1, в котором в котором температура в четвертом реакторе составляет окол

Claims (32)

1. Способ получения топлива из синтез-газа, включающий стадии:
а) пропускания синтез-газа через первый реактор с целью конверсии синтез-газа в метанол и воду с образованием первого выходящего потока,
б) пропускания первого выходящего потока через второй реактор с целью конверсии метанола в простой диметиловый эфир с образованием второго выходящего потока,
в) пропускания второго выходящего потока через третий реактор с целью конверсии метанола и простого диметилового эфира в топливо и тяжелый бензин с образованием третьего выходящего потока,
г) пропускания третьего выходящего потока через четвертый реактор с целью конверсии тяжелого бензина в изопарафины, нафтены и ароматические соединения с низкой степенью замещения с образованием четвертого выходящего потока, и
д) возвращения непрореагировавшего синтез-газа, содержащегося в четвертом выходящем потоке, в повторный цикл в первый реактор,
причем на протяжении способа не осуществляют удаление или отделение первого, второго или третьего выходящих потоков.
2. Способ по п.1, в котором первый, второй, третий и четвертый реакторы действуют под давление около 50-100 атмосфер.
3. Способ по п.1, в котором топливо содержит по существу C4-C8 углеводороды, толуол и ксилол.
4. Способ по п.1, в котором тяжелый бензин содержит ароматические соединения ≥C8.
5. Способ по п.1, в котором температура в первом реакторе составляет около 190-300°C.
6. Способ по п.1, в котором в котором температура во втором реакторе составляет около 300-450°C.
7. Способ по п.1, в котором в котором температура в третьем реакторе составляет около 300-500°C.
8. Способ по п.1, в котором в котором температура в четвертом реакторе составляет около 100-220°C.
9. Способ по п.1, в котором первый реактор содержит катализаторы CuO/ZnO/Al2O3.
10. Способ по п.1, в котором второй реактор содержит катализаторы на основе гамма-оксида алюминия.
11. Способ по п.1, в котором третий реактор содержит катализаторы ZSM-5.
12. Способ по п.1, в котором четвертый реактор содержит катализатор на основе оксида металла Группы IX или X на алюминийоксидном носителе, восстановленный в присутствии водорода и окиси углерода и в отсутствие серы.
13. Способ по п.12, в котором оксидом металла Группы IX или X является оксид никеля.
14. Способ по п.1, в котором четвертый реактор содержит катализатор на основе оксида металла Группы IX или X в сочетании с катализатором на основе оксида металла Группы VI на алюминийоксидном носителе, восстановленный в присутствии водорода и окиси углерода и в отсутствие серы.
15. Способ по п.14, в котором оксидом металла Группы IX или X является оксид кобальта, а оксидом металла Группы VI является оксид молибдена, образующий молибдат кобальта.
16. Способ по п.1, в котором до осуществления стадии д) четвертый выходящий поток разделяют на первый поток, содержащий воду, второй поток, содержащий непрореагировавший синтез-газ, и третий поток, содержащий топливо.
17. Способ по п.1, в котором нагревают или охлаждают первый, второй и третий выходящие потоки до их подачи во второй, третий и четвертый реакторы, соответственно.
18. Способ по п.1, в котором тяжелый бензин содержит триметилбензол, тетраметилбензол и дурол.
19. Способ по п.1, в котором менее замещенными ароматическими соединениями являются толуол и ксилол.
20. Способ по п.1, в котором температура замерзания третьего выходящего потока составляет от около 30 до около 50°C.
21. Способ по п.1, в котором температура замерзания топлива составляет менее около -5°C.
22. Способ по п.1, в котором выход составляет более около 25% по весу синтез-газа.
23. Способ по п.1, в котором синтез-газ изначально подают непосредственно в третий реактор.
24. Способ по п.23, в котором синтез-газ содержит молекулы алифатических углеводородов и/или олефинов с двумя или более атомами углерода и/или более крупные молекулы циклических и ароматических соединений
25. Система получения готового топлива, содержащая:
а) первый реактор, содержащий первый катализатор для конверсии синтез-газа в метанол и воду,
б) второй реактор, содержащий второй катализатор для конверсии метанола в простой диметиловый эфир,
в) третий реактор, содержащий третий катализатор для конверсии метанола и простого диметилового эфира в топливо и тяжелый бензин,
г) четвертый реактор, содержащий четвертый катализатор для конверсии тяжелого бензина в изопарафины, нафтены и ароматические соединения с низкой степенью замещения,
д) сепаратор для разделения продукта, выходящего из четвертого реактора, на первый поток, содержащий готовое топливо, второй поток, содержащий воду, и третий поток, содержащий непрореагировавший синтез-газ, и
е) поток, возвращаемый в повторный цикл, с целью возврата части третьего потока в повторный цикл в первый реактор.
26. Система по п.25, в которой первым катализатором является CuO/ZnO/Al2O3.
27. Система по п.25, в которой вторым катализатором является гамма-оксид алюминия.
28. Система по п.25, в которой третьим катализатором является ZSM-5.
29. Система по п.25, в которой четвертым катализатором является катализатор на основе оксида металла Группы IX или X на алюминийоксидном носителе, восстановленный в присутствии водорода и окиси углерода и в отсутствие серы.
30. Система по п.29, в которой оксидом металла Группы IX или X является оксид никеля.
31. Система по п.25, в которой четвертый реактор содержит катализатор на основе оксида металла Группы IX или X в сочетании с катализатором на основе оксида металла Группы VI на алюминийоксидном носителе, восстановленный в присутствии водорода и окиси углерода и в отсутствие серы.
32. Система по п.31, в которой оксидом металла Группы IX или X является оксид кобальта, а оксидом металла Группы VI является оксид молибдена, образующий молибдат кобальта.
RU2013124424/04A 2010-11-09 2011-11-09 Одноконтурное многоступенчатое получение топлива RU2574390C2 (ru)

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US12/942,680 US8686206B2 (en) 2010-11-09 2010-11-09 Single loop multistage fuel production
PCT/US2011/059975 WO2012064844A2 (en) 2010-11-09 2011-11-09 Single loop multistage fuel production

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