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IE34082L - 3-oxo-19-nor- delta4-steroids - Google Patents

3-oxo-19-nor- delta4-steroids

Info

Publication number
IE34082L
IE34082L IE700412A IE41270A IE34082L IE 34082 L IE34082 L IE 34082L IE 700412 A IE700412 A IE 700412A IE 41270 A IE41270 A IE 41270A IE 34082 L IE34082 L IE 34082L
Authority
IE
Ireland
Prior art keywords
acid
alkyl
compounds
reaction
formula
Prior art date
Application number
IE700412A
Other versions
IE34082B1 (en
Original Assignee
Hoffmann La Roche
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Hoffmann La Roche filed Critical Hoffmann La Roche
Publication of IE34082L publication Critical patent/IE34082L/en
Publication of IE34082B1 publication Critical patent/IE34082B1/en

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07JSTEROIDS
    • C07J1/00Normal steroids containing carbon, hydrogen, halogen or oxygen, not substituted in position 17 beta by a carbon atom, e.g. estrane, androstane
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07JSTEROIDS
    • C07J73/00Steroids in which the cyclopenta[a]hydrophenanthrene skeleton has been modified by substitution of one or two carbon atoms by hetero atoms
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C2603/00Systems containing at least three condensed rings
    • C07C2603/02Ortho- or ortho- and peri-condensed systems
    • C07C2603/04Ortho- or ortho- and peri-condensed systems containing three rings
    • C07C2603/06Ortho- or ortho- and peri-condensed systems containing three rings containing at least one ring with less than six ring members
    • C07C2603/10Ortho- or ortho- and peri-condensed systems containing three rings containing at least one ring with less than six ring members containing five-membered rings
    • C07C2603/12Ortho- or ortho- and peri-condensed systems containing three rings containing at least one ring with less than six ring members containing five-membered rings only one five-membered ring
    • C07C2603/16Benz[e]indenes; Hydrogenated benz[e]indenes

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • General Health & Medical Sciences (AREA)
  • Steroid Compounds (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
  • Pharmaceuticals Containing Other Organic And Inorganic Compounds (AREA)

Abstract

1309651 Steroid synthesis; 4,5-secosteroids F HOFFMANN-LA ROCHE & CO AG 2 April 1970 [4 April 1969] 15632/70 Headings C2C and C2U The invention comprises compounds of Formul VI and VII and a process for preparing compounds of Formula I from compounds of Formula II by reaction sequence ABCDE or ABCDFG in the reaction scheme in which all compounds are d, l or dl, M is the remainder of the D ring of the steroid; R is OH, C 1-7 alkoxy or -NXY where X and Y are each C 1-7 alkyl; R<SP>1</SP> is primary C 1-5 alkyl, R<SP>2</SP>, R<SP>3</SP> and R<SP>5</SP> are each H or C 1-7 alkyl; and R<SP>6</SP> is H, monocyclic aryl- C 1-7 -alkyl, acyl or -CR<SP>7</SP>R<SP>8</SP>R<SP>9</SP> where R<SP>7</SP>, R<SP>8</SP> and R<SP>9</SP> are each C 1-7 alkyl. Reaction sequence A<SP>1</SP>B<SP>1</SP> is alternative to AB but does not form part of the invention and is not exemplified. The reaction steps are effected as follows: (A) heat and/or acid; (A<SP>1</SP>) and (B) hydrogenation with a noble metal catalyst in the presence of a base; (B<SP>1</SP>) heat and acid; (C) reaction with R-NH 2 or a salt thereof; (D) selective oxidation, e.g. with CrO 3 /acetone, metal alkoxide, silver carbonate, or CrO 3 /H 2 SO 4 /N,N-dialkylalkanamide; (E) aqueous acid in an inert watermiscible organic solvent; (F) reaction with a reactive carbonyl compound; e.g. acetone, pyruvic acid or levulinic acid; (G) cyclization which may be acid- or base-catalysed. A 17 oxo group (steroid numbering) in a compound of Formula III may be converted to an =NR group during step (C) and regenerated during step (E) or (G). Alternatively said 17- oxo group may be reduced to a 17#-hydroxy group or converted to a 17α-alkynyl-17#- hydroxy group immediately prior to step C. A 17-hydroxy group in a compound of Formula VI may be converted to an oxo group during step (D). Compounds of Formul III and IV comprise the subject-matter of Specification 1,309,652. Reference has been directed by the Comptroller to Specification 1,207,048. [GB1309651A]
IE412/70A 1969-04-04 1970-04-02 A process for the preparation of 3-oxo-19-nor-delta4-steroids via novel nitrogenous 4,5-secosteroids IE34082B1 (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
US81369369A 1969-04-04 1969-04-04

Publications (2)

Publication Number Publication Date
IE34082L true IE34082L (en) 1970-10-04
IE34082B1 IE34082B1 (en) 1975-01-22

Family

ID=25213104

Family Applications (1)

Application Number Title Priority Date Filing Date
IE412/70A IE34082B1 (en) 1969-04-04 1970-04-02 A process for the preparation of 3-oxo-19-nor-delta4-steroids via novel nitrogenous 4,5-secosteroids

Country Status (13)

Country Link
JP (2) JPS5028952B1 (en)
BE (1) BE748356A (en)
CH (1) CH568336A5 (en)
DE (1) DE2015800C3 (en)
FR (1) FR2068452B1 (en)
GB (2) GB1309652A (en)
HU (1) HU163408B (en)
IE (1) IE34082B1 (en)
IL (1) IL34184A (en)
NL (1) NL7004801A (en)
PL (1) PL80640B1 (en)
SE (1) SE362421B (en)
SU (1) SU439089A3 (en)

Families Citing this family (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
JPS53146139U (en) * 1977-04-22 1978-11-17
GB2514589B (en) 2013-05-30 2020-01-29 Nat Oilwell Varco Lp Centrifuge for separating solids from solids laden drilling fluid

Family Cites Families (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CH503050A (en) * 1967-11-02 1971-02-15 Hoffmann La Roche Process for the preparation of polycyclic compounds

Also Published As

Publication number Publication date
GB1309652A (en) 1973-03-14
IE34082B1 (en) 1975-01-22
GB1309651A (en) 1973-03-14
CH568336A5 (en) 1975-10-31
HU163408B (en) 1973-08-28
NL7004801A (en) 1970-10-06
FR2068452B1 (en) 1973-07-13
IL34184A0 (en) 1970-05-21
SU439089A3 (en) 1974-08-05
PL80640B1 (en) 1975-08-30
JPS5028952B1 (en) 1975-09-19
DE2015800C3 (en) 1979-06-13
DE2015800B2 (en) 1978-10-19
SE362421B (en) 1973-12-10
IL34184A (en) 1973-08-29
BE748356A (en) 1970-10-02
JPS4935626B1 (en) 1974-09-25
FR2068452A1 (en) 1971-08-27
DE2015800A1 (en) 1970-10-22

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