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GB851059A - Process for polymerization and the products produced thereby - Google Patents

Process for polymerization and the products produced thereby

Info

Publication number
GB851059A
GB851059A GB10322/57A GB1032257A GB851059A GB 851059 A GB851059 A GB 851059A GB 10322/57 A GB10322/57 A GB 10322/57A GB 1032257 A GB1032257 A GB 1032257A GB 851059 A GB851059 A GB 851059A
Authority
GB
United Kingdom
Prior art keywords
ceric
polymers
grafted
salt
esters
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
GB10322/57A
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Wyeth Holdings LLC
Original Assignee
American Cyanamid Co
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by American Cyanamid Co filed Critical American Cyanamid Co
Publication of GB851059A publication Critical patent/GB851059A/en
Expired legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F36/00Homopolymers and copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds
    • C08F36/02Homopolymers and copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds the radical having only two carbon-to-carbon double bonds
    • C08F36/04Homopolymers and copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds the radical having only two carbon-to-carbon double bonds conjugated
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F291/00Macromolecular compounds obtained by polymerising monomers on to macromolecular compounds according to more than one of the groups C08F251/00 - C08F289/00
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F4/00Polymerisation catalysts
    • C08F4/06Metallic compounds other than hydrides and other than metallo-organic compounds; Boron halide or aluminium halide complexes with organic compounds containing oxygen

Landscapes

  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • Graft Or Block Polymers (AREA)
  • Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)

Abstract

Graft and block polymers are made by polymerizing a compound containing a polymerizable CH2=C < group in an aqueous medium at a pH not greater than 6,0 and at a temperature between -5 DEG C. and 100 DEG C. in the presence of a ceric salt which is soluble in at least one of the components of the reaction system, and a polymeric organic reducing agent capable of being oxidized by the ceric salt and capable of initiating the polymerization, the reducing agent being an aldehyde or an acetal or a compound containing the <FORM:0851059/IV(a)/1> group wherein X is OH, RCO, SH and NHR, wherein R is hydrogen, alkyl, aralkyl or aryl, the open bonds of the <FORM:0851059/IV(a)/2> group being essentially organic residues and/or hydrogen. Monomers specified are styrene and various alkyl and halogen substituted styrenes, acrylic, methacrylic and chloroacrylic acids, anhydrides, amides and nitriles, C1-10 acrylates, acrylic esters of various nitroalkanols, acrylic esters of various polyhydric alcohols, butadiene, isoprene, chloroprene, allyl and methallyl esters of various saturated and unsaturated acids, vinyl acetate, propionate and butyrate, vinyl and vinylidene chlorides, vinyl ethyl, propyl and isobutyl ethers, divinylsulphone, divinylsulphide and vinyl pyridine. Polymeric reducing agents specified are polyvinyl alcohol and its partially formylated, acetylated, sulphated, nitrated and cyanoethylated derivatives, cellulose, regenerated cellulose, the partial acetic, propionic and nitric esters and partial methyl, ethyl, hydroxyethyl ethers of cellulose, starch and its partially cyanoethylated and acetylated derivatives, polymers of beta-hydroxyethyl acrylate and methacrylate, polyvinyl pyrrolidone, polymers of C1-C3 alkyl vinyl ketones, polyamines made by treating acrylamide polymers with sodium hypochlorite, polymers of acrolein, 3-butenal, 3-pentenal and 5-chloro-3-pentenal, various mercaptoalkyl acrylates and methacrylates, polyvinyl formal, acetal and butyral, graft copolymers containing reducing groups, e.g. a graft copolymer of polyacrylamide and polyvinyl alcohol and, for the purpose of forming block polymers, polymers having terminal reducing groups, e.g. polyethylene glycol, polyethylene imines and polymers obtained by polymerizing unsaturated monomers in the presence of trimethylene glycol and 1,4-butanediol. Ceric salts specified are ceric ammonium nitrate, ceric sulphate, ceric dihexyl sulphoccinate and other salts obtained by reacting an inorganic ceric salt with organic sulphur containing acids. When polymerization is carried out in emulsion there is used an emulsifying agent, various alkali metal organic sulphonates and sulphates being specified for this purpose. Polymerisation may be carried in such a way as to graft two monomeric materials, e.g. methyl acrylate and acrylamide, on to the same preformed polymer, e.g. polyvinyl alcohol.ALSO:Oil-soluble ceric salts of organic sulphurcontaining acids are prepared by reacting an inorganic ceric salt, e.g. ceric ammonium nitrate, with an organic sulphur containing monobasic or polybasic acid or an alkali metal salt thereof, e.g. the sulpho derivatives of aliphatic dibasic acids and alkyl esters thereof, monoalkyl esters of sulphuric acid and alkyl benzene and naphthalene sulphonates. Salts specified are ceric dihexyl and dioctyl sulphosuccinates, diheptyl sulphoglutarate, didecyl sulphosuberate, dilaurylsulphosebacate, diamyl sulphomaleate, dimethyl sulphofumarate, dibutyl sulphodimethyl succinate and dilauryl sulphomethylglutarate. The preparation of ceric dihexyl sulphosuccinate is described by a process which involves mixing aqueous solutions of ceric ammonium nitrate and sodium dihexyl sulphosuccinate and filtering off the precipitated ceric salt.ALSO:Textile fabrics made from cellulosic fibres, e.g. those of cotton, viscose rayon and cuprammonium rayon, are treated by graft polymerizing thereon an ethylenically unsaturated compound in an aqueous medium with the aid of a ceric salt (see Group IV(a) ). In examples: (6) acrylonitrile is grafted on to a cotton fabric; (7) acrylonitrile is grafted on to a viscose rayon fabric; (8) acrylamide is grafted on to a cotton fabric; (9) methyl acrylate is grafted on to a cotton fabric; (10) methylene bisacrylamide is grafted on to a viscose rayon fabric; and (11) acrylamide is grafted on to a cotton fabric which is then treated with formaldehyde to give a fabric of improved wrinkle recovery.
GB10322/57A 1956-04-12 1957-03-29 Process for polymerization and the products produced thereby Expired GB851059A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
US851059XA 1956-04-12 1956-04-12

Publications (1)

Publication Number Publication Date
GB851059A true GB851059A (en) 1960-10-12

Family

ID=22189501

Family Applications (2)

Application Number Title Priority Date Filing Date
GB10322/57A Expired GB851059A (en) 1956-04-12 1957-03-29 Process for polymerization and the products produced thereby
GB10538/57A Expired GB855235A (en) 1956-04-12 1957-04-01 Process for polymerization and the products produced thereby

Family Applications After (1)

Application Number Title Priority Date Filing Date
GB10538/57A Expired GB855235A (en) 1956-04-12 1957-04-01 Process for polymerization and the products produced thereby

Country Status (5)

Country Link
BE (2) BE556515A (en)
DE (2) DE1082409B (en)
FR (2) FR1173524A (en)
GB (2) GB851059A (en)
NL (4) NL216299A (en)

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP1264868A3 (en) * 2001-05-25 2003-12-10 Hewlett-Packard Company Ink additive
CN112921443A (en) * 2021-01-31 2021-06-08 福建沃凯丝化纤有限公司 Preparation method of special low-melting-point fiber polymerization auxiliary agent

Families Citing this family (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
NL120957C (en) * 1958-10-04
NL268017A (en) * 1960-08-08
CN113072791A (en) * 2021-04-01 2021-07-06 吴达华 Degradable plastic taking corn starch as raw material and preparation method thereof
CN113549188B (en) * 2021-09-01 2022-12-16 苏州胜蓝夫密封材料有限公司 A kind of hydrophilic halamine antibacterial agent modified polyurethane foam and preparation method thereof

Family Cites Families (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2485535A (en) * 1946-12-12 1949-10-18 Monsanto Chemicals Ceric sulfate catalyzed emulsion polymerization of styrene

Cited By (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
EP1264868A3 (en) * 2001-05-25 2003-12-10 Hewlett-Packard Company Ink additive
US7115675B2 (en) 2001-05-25 2006-10-03 Hewlett-Packard Development Company, L.P. Under-/overprinting fluid component for enhancing ink stability in printing
CN112921443A (en) * 2021-01-31 2021-06-08 福建沃凯丝化纤有限公司 Preparation method of special low-melting-point fiber polymerization auxiliary agent

Also Published As

Publication number Publication date
BE556633A (en)
BE556515A (en)
NL92194C (en)
FR1173524A (en) 1959-02-26
NL216298A (en)
DE1082409B (en) 1960-05-25
DE1082408B (en) 1960-05-25
NL216299A (en)
GB855235A (en) 1960-11-30
FR1174149A (en) 1959-03-06
NL97977C (en)

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