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GB804097A - A process for the production of organosilicon compounds - Google Patents

A process for the production of organosilicon compounds

Info

Publication number
GB804097A
GB804097A GB24867/56A GB2486756A GB804097A GB 804097 A GB804097 A GB 804097A GB 24867/56 A GB24867/56 A GB 24867/56A GB 2486756 A GB2486756 A GB 2486756A GB 804097 A GB804097 A GB 804097A
Authority
GB
United Kingdom
Prior art keywords
copolymer
silicon
compounds
compound
ch3cl2si
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
GB24867/56A
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Midland Silicones Ltd
Original Assignee
Midland Silicones Ltd
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Midland Silicones Ltd filed Critical Midland Silicones Ltd
Publication of GB804097A publication Critical patent/GB804097A/en
Expired legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G77/00Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
    • C08G77/60Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule in which all the silicon atoms are connected by linkages other than oxygen atoms
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07FACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
    • C07F7/00Compounds containing elements of Groups 4 or 14 of the Periodic Table
    • C07F7/02Silicon compounds
    • C07F7/08Compounds having one or more C—Si linkages
    • C07F7/0801General processes
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08GMACROMOLECULAR COMPOUNDS OBTAINED OTHERWISE THAN BY REACTIONS ONLY INVOLVING UNSATURATED CARBON-TO-CARBON BONDS
    • C08G77/00Macromolecular compounds obtained by reactions forming a linkage containing silicon with or without sulfur, nitrogen, oxygen or carbon in the main chain of the macromolecule
    • C08G77/04Polysiloxanes
    • C08G77/38Polysiloxanes modified by chemical after-treatment

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • General Chemical & Material Sciences (AREA)
  • Compositions Of Macromolecular Compounds (AREA)
  • Silicon Polymers (AREA)

Abstract

Chloroplatinic acid is used as catalyst in the reaction between silicon compounds containing silicon-bonded hydrogen and compounds containing aliphatic unsaturation. The catalyst is preferably used in the form of its hexahydrate and may be in solution, e.g. in water, alcohols and various glycols, and esters. The silicon compound, which may be inorganic or organic, monomeric or polymeric, must not contain more than two hydrogen atoms attached to one silicon atom. The examples of polymers include polysiloxanes, polysilanes, polysilcarbanes and polysilazanes. The unsaturated compound may have ethylenic or acetylenic unsaturation and may be heterocyclic, an organo-metallic compound, e.g. an organo-silicon compound, a titanate or zirconate, or it may be an organic salt or ester of an inorganic acid. Other suitable compounds are natural and synthetic polymers which contain residual unsaturation. The presence of aldehyde groups is undesirable as it leads to a rearrangement in the form of polymeric groups such as ­Si(CH2)3OSi­. If the unsaturated compound is an organo-silicon compound containing silicon-bonded hydrogen, it can react with itself. The Specification contains numerous examples of specific reactants. The following are used in the examples illustrating the invention:-Hydrosilicon compounds: MeHSiCl2, [(CH3)HSiO]4, SiHCl3, PhSiHCl2, [CH3)HSiO]6, (Me2HSi)2O, triacetoxysilane, methyldiethoxysilane, MeH2SiCl, BuHSiCl2, (MeHSiO)x, and a copolymer prepared from PhMeSiCl2, HSiCl3 and MeHSiCl2. Unsaturated compounds: pentene-1 and -2, cyclohexene, ethyl crotonate, methyl cis-bicyclo-(2,2,1)-hept-5-ene-2-carboxylate, 3-butenyl acetate, allyl methacrylate, <FORM:0804097/IV (a)/1> styrene, divinyl benzene, diallyl phthalate, triallyl cyanurate, ethylene, allyl acetate, dichloro-styrene, propylene, a copolymer of PhMeSiO and PhViSiO, allyl cyanide, methyl acrylate and methacrylate, acetylene, vinyl chloride, butadiene, methyl oleate, isobutylene, butyne, vinyl acetate, a copolymer of Me2SiO and MeViSiO, natural rubber, butadiene-styrene copolymer, and a copolymer of PhEtSiO, Me3SiO0.5, SiO2, Cl2C6H3SiO1.5, cyclohexylsiloxane, benzylmethylsiloxane, ViSiO1.5, Me2ViSiO0.5 and cyclohexenylmethylsiloxane. Among the products identified are: amylmethyldichlorosilane, cyclohexylmethyldichlorosilane, amyltrichlorosilane, CH3Cl2Si(CH2)4 OOCCH3, CH3Cl2Si (CH2)3OOC(CH3)C=CH2, a foamed resin prepared from (CH3HSiO)4 and diallyl phthalate at 150 DEG C. or triallyl cyanurate at 50 DEG C., ethyl trichloro- and tribromo-silanes, MeCOOCH2CH2 CH2SiPhCl2, (dichlorostyryl)dimethylchlorosilane, n-propyltrichlorosilane, CH3Cl2Si(CH2)3 CN, Me2HSiOSiMe2(CH2)4OAc, O[SiMe2(CH2)4 OAc]2, MeCl2SiCHCH3COOMe, MeCl2SiCH2CH2 COOMe, vinyltriacetoxysilane, methylethyldiethoxysilane, methyldiethylchlorosilane, ethylbutyldichlorosilane, MeCl2SiCH2CHMeCOOMe and MeCl2SiC2H4OAc. In an example, Hervea braziliensis in the form of smoked sheet is heated with trichlorosilane (1 mol. of silane per double bond) in benzene with the catalyst to give a trichlorosilyl substituted rubber.
GB24867/56A 1955-12-05 1956-08-14 A process for the production of organosilicon compounds Expired GB804097A (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
US804097XA 1955-12-05 1955-12-05

Publications (1)

Publication Number Publication Date
GB804097A true GB804097A (en) 1958-11-05

Family

ID=22157173

Family Applications (1)

Application Number Title Priority Date Filing Date
GB24867/56A Expired GB804097A (en) 1955-12-05 1956-08-14 A process for the production of organosilicon compounds

Country Status (3)

Country Link
DE (1) DE1069148B (en)
FR (1) FR1163492A (en)
GB (1) GB804097A (en)

Cited By (5)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE1126619B (en) * 1959-08-14 1962-03-29 Wacker Chemie Gmbh Process for the production of high molecular weight silicon-containing polymers
US3419593A (en) * 1965-05-17 1968-12-31 Dow Corning Catalysts for the reaction of = sih with organic compounds containing aliphatic unsaturation
WO1985002854A1 (en) * 1983-12-28 1985-07-04 Union Carbide Corporation Organosiloxane polymers and compositions containing same curable upon exposure to gaseous oxygen
JPS62501717A (en) * 1984-12-11 1987-07-09 エアゾ−ブ・プロプライアトリ−・リミテッド Protective helmets and securing devices
EP0251678A3 (en) * 1986-06-30 1988-07-20 Dow Corning Corporation Ceramic materials from polycarbosilanes

Families Citing this family (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
GB923710A (en) * 1960-11-07 1963-04-18 Ici Ltd Production of organosilicon compounds
DE1283529B (en) * 1966-10-28 1968-11-21 Bayer Ag Casting compounds convertible into transparent organosiloxane elastomers
US3678126A (en) * 1970-08-25 1972-07-18 Dow Corning Siloxane containing thermoplastic elastomers
DE4023960A1 (en) * 1990-07-27 1992-01-30 Fraunhofer Ges Forschung Polymers contg. poly:organo-siloxane] units - prepd. by reacting polymer contg. terminal or lateral olefinic gps. with poly:hydrogen-organo-polysiloxane and transition metal catalyst

Cited By (6)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE1126619B (en) * 1959-08-14 1962-03-29 Wacker Chemie Gmbh Process for the production of high molecular weight silicon-containing polymers
US3419593A (en) * 1965-05-17 1968-12-31 Dow Corning Catalysts for the reaction of = sih with organic compounds containing aliphatic unsaturation
WO1985002854A1 (en) * 1983-12-28 1985-07-04 Union Carbide Corporation Organosiloxane polymers and compositions containing same curable upon exposure to gaseous oxygen
EP0152630A3 (en) * 1983-12-28 1985-09-25 Union Carbide Corporation Organosiloxane polymers and compositions containing same curable upon exposure to gaseous oxygen
JPS62501717A (en) * 1984-12-11 1987-07-09 エアゾ−ブ・プロプライアトリ−・リミテッド Protective helmets and securing devices
EP0251678A3 (en) * 1986-06-30 1988-07-20 Dow Corning Corporation Ceramic materials from polycarbosilanes

Also Published As

Publication number Publication date
FR1163492A (en) 1958-09-26
DE1069148B (en) 1959-11-19

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