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GB1020728A - Process for the allylation of organic compounds - Google Patents

Process for the allylation of organic compounds

Info

Publication number
GB1020728A
GB1020728A GB32812/63A GB3281263A GB1020728A GB 1020728 A GB1020728 A GB 1020728A GB 32812/63 A GB32812/63 A GB 32812/63A GB 3281263 A GB3281263 A GB 3281263A GB 1020728 A GB1020728 A GB 1020728A
Authority
GB
United Kingdom
Prior art keywords
group
allyl
hydrogen atom
methylene
catalyst
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
GB32812/63A
Inventor
Robert James Stephenson
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Monsanto Chemicals Ltd
Original Assignee
Monsanto Chemicals Ltd
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Monsanto Chemicals Ltd filed Critical Monsanto Chemicals Ltd
Priority to GB32812/63A priority Critical patent/GB1020728A/en
Publication of GB1020728A publication Critical patent/GB1020728A/en
Expired legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C49/00Ketones; Ketenes; Dimeric ketenes; Ketonic chelates
    • C07C49/20Unsaturated compounds containing keto groups bound to acyclic carbon atoms
    • C07C49/203Unsaturated compounds containing keto groups bound to acyclic carbon atoms with only carbon-to-carbon double bonds as unsaturation
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07CACYCLIC OR CARBOCYCLIC COMPOUNDS
    • C07C45/00Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds
    • C07C45/61Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups
    • C07C45/67Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton
    • C07C45/68Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton by increase in the number of carbon atoms
    • C07C45/70Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton by increase in the number of carbon atoms by reaction with functional groups containing oxygen only in singly bound form
    • C07C45/71Preparation of compounds having >C = O groups bound only to carbon or hydrogen atoms; Preparation of chelates of such compounds by reactions not involving the formation of >C = O groups by isomerisation; by change of size of the carbon skeleton by increase in the number of carbon atoms by reaction with functional groups containing oxygen only in singly bound form being hydroxy groups
    • YGENERAL TAGGING OF NEW TECHNOLOGICAL DEVELOPMENTS; GENERAL TAGGING OF CROSS-SECTIONAL TECHNOLOGIES SPANNING OVER SEVERAL SECTIONS OF THE IPC; TECHNICAL SUBJECTS COVERED BY FORMER USPC CROSS-REFERENCE ART COLLECTIONS [XRACs] AND DIGESTS
    • Y02TECHNOLOGIES OR APPLICATIONS FOR MITIGATION OR ADAPTATION AGAINST CLIMATE CHANGE
    • Y02PCLIMATE CHANGE MITIGATION TECHNOLOGIES IN THE PRODUCTION OR PROCESSING OF GOODS
    • Y02P20/00Technologies relating to chemical industry
    • Y02P20/50Improvements relating to the production of bulk chemicals
    • Y02P20/582Recycling of unreacted starting or intermediate materials

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Abstract

The alkylation of organic compounds containing an active methylene or an active methine group in which the methylene or methine group is attached to two activating groups of the kind exemplified by cyano and carbonyl is effected by reaction of said organic compound w4th an allyl alcohol or an allyl ether. If an activating group is a carbonyl group it may be ketonic or aldehydic or form part of a carboxyl, ester or amide group. Other specified activating groups are the nitro group and, in certain cases, an aromatic ring. Preferred allyl alcohols are those of the general formula R1-CH = CH-CHR2-OH wherein R1 is a hydrogen atom or a substituted or unsubstituted hydrocarbon group and R2 is a hydrogen atom or an alkyl group or R1 and R2 together with the -CH = CH(OH)-CH- radical form an alicyclic ring, and preferred ethers are those derived from said alcohols. The reaction, which is usually effected by heating the reactants, may be performed in the presence of a catalyst which can be an acid, including Lewis acids and acidic ion exchange resins, but is preferably an acid together with a salt of a metal that is capable of forming a complex compound with an olefin. The products of the allylation are compounds wherein a hydrogen atom of the active methylene or methine group has been replaced by an allyl group of the allyl alcohol or ether. In the only Example 3 allyl pentan-2-4-diol is prepared from acetyl acetone and diallylether in the presence of a sulphonated cross-linked polystyrene resin and cuprous chloride as catalyst.
GB32812/63A 1963-08-20 1963-08-20 Process for the allylation of organic compounds Expired GB1020728A (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
GB32812/63A GB1020728A (en) 1963-08-20 1963-08-20 Process for the allylation of organic compounds

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
GB32812/63A GB1020728A (en) 1963-08-20 1963-08-20 Process for the allylation of organic compounds

Publications (1)

Publication Number Publication Date
GB1020728A true GB1020728A (en) 1966-02-23

Family

ID=10344377

Family Applications (1)

Application Number Title Priority Date Filing Date
GB32812/63A Expired GB1020728A (en) 1963-08-20 1963-08-20 Process for the allylation of organic compounds

Country Status (1)

Country Link
GB (1) GB1020728A (en)

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3965193A (en) 1971-11-17 1976-06-22 Badische Anilin- & Soda-Fabrik Aktiengesellschaft Production of high molecular weight α,β-unsaturated aldehydes
US4021411A (en) * 1971-11-17 1977-05-03 Badische Anilin- & Soda-Fabrik Aktiengesellschaft Production of high molecular weight α,β-unsaturated aldehydes

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US3965193A (en) 1971-11-17 1976-06-22 Badische Anilin- & Soda-Fabrik Aktiengesellschaft Production of high molecular weight α,β-unsaturated aldehydes
US4021411A (en) * 1971-11-17 1977-05-03 Badische Anilin- & Soda-Fabrik Aktiengesellschaft Production of high molecular weight α,β-unsaturated aldehydes

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