DE60316437D1 - Propylen copolymerzusammensetzungen mit guter tieftemperatur-schlagfestigkeit und hoher transparenz - Google Patents
Propylen copolymerzusammensetzungen mit guter tieftemperatur-schlagfestigkeit und hoher transparenzInfo
- Publication number
- DE60316437D1 DE60316437D1 DE60316437T DE60316437T DE60316437D1 DE 60316437 D1 DE60316437 D1 DE 60316437D1 DE 60316437 T DE60316437 T DE 60316437T DE 60316437 T DE60316437 T DE 60316437T DE 60316437 D1 DE60316437 D1 DE 60316437D1
- Authority
- DE
- Germany
- Prior art keywords
- impact strength
- propylene copolymer
- high transparency
- temperature impact
- good temperature
- Prior art date
- Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
- Expired - Lifetime
Links
- 229920001577 copolymer Polymers 0.000 title 1
- 239000000203 mixture Substances 0.000 title 1
- QQONPFPTGQHPMA-UHFFFAOYSA-N propylene Natural products CC=C QQONPFPTGQHPMA-UHFFFAOYSA-N 0.000 title 1
Classifications
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L23/00—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
- C08L23/02—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
- C08L23/10—Homopolymers or copolymers of propene
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F210/00—Copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond
- C08F210/04—Monomers containing three or four carbon atoms
- C08F210/06—Propene
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F4/00—Polymerisation catalysts
- C08F4/42—Metals; Metal hydrides; Metallo-organic compounds; Use thereof as catalyst precursors
- C08F4/44—Metals; Metal hydrides; Metallo-organic compounds; Use thereof as catalyst precursors selected from light metals, zinc, cadmium, mercury, copper, silver, gold, boron, gallium, indium, thallium, rare earths or actinides
- C08F4/60—Metals; Metal hydrides; Metallo-organic compounds; Use thereof as catalyst precursors selected from light metals, zinc, cadmium, mercury, copper, silver, gold, boron, gallium, indium, thallium, rare earths or actinides together with refractory metals, iron group metals, platinum group metals, manganese, rhenium technetium or compounds thereof
- C08F4/62—Refractory metals or compounds thereof
- C08F4/64—Titanium, zirconium, hafnium or compounds thereof
- C08F4/659—Component covered by group C08F4/64 containing a transition metal-carbon bond
- C08F4/65912—Component covered by group C08F4/64 containing a transition metal-carbon bond in combination with an organoaluminium compound
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08F—MACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
- C08F4/00—Polymerisation catalysts
- C08F4/42—Metals; Metal hydrides; Metallo-organic compounds; Use thereof as catalyst precursors
- C08F4/44—Metals; Metal hydrides; Metallo-organic compounds; Use thereof as catalyst precursors selected from light metals, zinc, cadmium, mercury, copper, silver, gold, boron, gallium, indium, thallium, rare earths or actinides
- C08F4/60—Metals; Metal hydrides; Metallo-organic compounds; Use thereof as catalyst precursors selected from light metals, zinc, cadmium, mercury, copper, silver, gold, boron, gallium, indium, thallium, rare earths or actinides together with refractory metals, iron group metals, platinum group metals, manganese, rhenium technetium or compounds thereof
- C08F4/62—Refractory metals or compounds thereof
- C08F4/64—Titanium, zirconium, hafnium or compounds thereof
- C08F4/659—Component covered by group C08F4/64 containing a transition metal-carbon bond
- C08F4/65916—Component covered by group C08F4/64 containing a transition metal-carbon bond supported on a carrier, e.g. silica, MgCl2, polymer
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2205/00—Polymer mixtures characterised by other features
- C08L2205/02—Polymer mixtures characterised by other features containing two or more polymers of the same C08L -group
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2205/00—Polymer mixtures characterised by other features
- C08L2205/04—Polymer mixtures characterised by other features containing interpenetrating networks
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2205/00—Polymer mixtures characterised by other features
- C08L2205/22—Mixtures comprising a continuous polymer matrix in which are dispersed crosslinked particles of another polymer
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L23/00—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers
- C08L23/02—Compositions of homopolymers or copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond; Compositions of derivatives of such polymers not modified by chemical after-treatment
- C08L23/10—Homopolymers or copolymers of propene
- C08L23/14—Copolymers of propene
- C08L23/142—Copolymers of propene at least partially crystalline copolymers of propene with other olefins
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2308/00—Chemical blending or stepwise polymerisation process with the same catalyst
-
- C—CHEMISTRY; METALLURGY
- C08—ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
- C08L—COMPOSITIONS OF MACROMOLECULAR COMPOUNDS
- C08L2314/00—Polymer mixtures characterised by way of preparation
- C08L2314/06—Metallocene or single site catalysts
Landscapes
- Chemical & Material Sciences (AREA)
- Health & Medical Sciences (AREA)
- Chemical Kinetics & Catalysis (AREA)
- Medicinal Chemistry (AREA)
- Polymers & Plastics (AREA)
- Organic Chemistry (AREA)
- Compositions Of Macromolecular Compounds (AREA)
- Transition And Organic Metals Composition Catalysts For Addition Polymerization (AREA)
- Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)
- Manufacture Of Macromolecular Shaped Articles (AREA)
- Graft Or Block Polymers (AREA)
- Laminated Bodies (AREA)
Applications Claiming Priority (5)
| Application Number | Priority Date | Filing Date | Title |
|---|---|---|---|
| DE10226184 | 2002-06-12 | ||
| DE10226184 | 2002-06-12 | ||
| US39461502P | 2002-07-09 | 2002-07-09 | |
| US394615P | 2002-07-09 | ||
| PCT/EP2003/006043 WO2003106553A1 (en) | 2002-06-01 | 2003-06-10 | Propylene copolymer compositions having a good low-temperature impact toughness and a high transparency |
Publications (2)
| Publication Number | Publication Date |
|---|---|
| DE60316437D1 true DE60316437D1 (de) | 2007-10-31 |
| DE60316437T2 DE60316437T2 (de) | 2008-06-26 |
Family
ID=29737599
Family Applications (1)
| Application Number | Title | Priority Date | Filing Date |
|---|---|---|---|
| DE60316437T Expired - Lifetime DE60316437T2 (de) | 2002-06-12 | 2003-06-10 | Propylencopolymerzusammensetzungen mit guter tieftemperatur-schlagfestigkeit und hoher transparenz |
Country Status (13)
| Country | Link |
|---|---|
| US (1) | US20060167185A1 (de) |
| EP (1) | EP1511803B1 (de) |
| JP (1) | JP2005529227A (de) |
| CN (1) | CN1290917C (de) |
| AR (1) | AR040187A1 (de) |
| AT (1) | ATE373692T1 (de) |
| AU (1) | AU2003245926B2 (de) |
| BR (1) | BR0311863B1 (de) |
| CA (1) | CA2483206A1 (de) |
| DE (1) | DE60316437T2 (de) |
| ES (1) | ES2291651T3 (de) |
| RU (1) | RU2337114C2 (de) |
| WO (1) | WO2003106553A1 (de) |
Families Citing this family (42)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| WO2003106523A1 (en) * | 2002-06-01 | 2003-12-24 | Basell Polyolefine Gmbh | Flexible propylene copolymer compositions having a high transparency |
| JP5309377B2 (ja) * | 2003-05-08 | 2013-10-09 | ノボレン テクノロジー ホールディングス シー・ブイ | ポリプロピレン樹脂組成物 |
| PT1781737E (pt) * | 2004-07-30 | 2009-01-21 | Saudi Basic Ind Corp | Composições de co-polímero de propileno com elevada transparência |
| JP5116210B2 (ja) * | 2004-11-26 | 2013-01-09 | 三井化学株式会社 | レトルトフィルム用シーラントフィルム |
| JP2008523231A (ja) * | 2004-12-13 | 2008-07-03 | バーゼル・ポリオレフィン・イタリア・ソチエタ・ア・レスポンサビリタ・リミタータ | ポリオレフィン繊維 |
| CN101115796B (zh) | 2005-02-03 | 2010-11-17 | 巴塞尔聚烯烃股份有限公司 | 制造热成形制品的方法 |
| US7799880B2 (en) * | 2005-03-23 | 2010-09-21 | Basell Polyolefine Gmbh | Process for the polymerization of olefins |
| EP1871832B1 (de) * | 2005-04-21 | 2012-06-13 | Basell Poliolefine Italia S.r.l. | Biaxial orientierte propylenpolymerfolien |
| RU2398794C2 (ru) * | 2005-04-28 | 2010-09-10 | Базелль Полиолефин Италия С.Р.Л. | Композиция пропиленовых полимеров для горячего формования |
| KR101183747B1 (ko) * | 2005-05-10 | 2012-09-17 | 에스케이종합화학 주식회사 | 우수한 내충격성, 굴곡탄성율 및 투명성을 갖는폴리프로필렌 조성물 및 이의 제품 |
| ATE458601T1 (de) * | 2005-08-19 | 2010-03-15 | Solvay | Verfahren zur herstellung einer zellularen struktur auf kunststoffbasis und verfahren zur umsetzung dieses verfahrens |
| CN101410426B (zh) | 2006-03-29 | 2012-05-09 | 三井化学株式会社 | 丙烯类无规嵌段共聚物、含有该共聚物的树脂组合物和由其形成的成型体 |
| PL2137257T3 (pl) * | 2007-01-12 | 2011-03-31 | Dow Global Technologies Inc | Kompozycja odpowiednia do wyrobów cienkościennych formowanych wtryskowo |
| WO2008124040A1 (en) * | 2007-04-09 | 2008-10-16 | Exxonmobil Chemical Patents Inc. | Soft heterogeneous isotactic polyroplene compositions |
| ES2378290T3 (es) | 2008-10-29 | 2012-04-10 | Borealis Ag | Composición tenaz para aplicaciones alimentarias |
| US8076429B2 (en) | 2009-03-11 | 2011-12-13 | Lummus Novolen Technology Gmbh | Supertransparent high impact strength random block copolymer |
| DE102009049122B4 (de) | 2009-10-12 | 2023-10-19 | Sihl Gmbh | Kratzfeste Polypropylenfolie |
| KR100977665B1 (ko) * | 2009-12-18 | 2010-08-24 | 에스케이에너지 주식회사 | 충격강도, 표면특성 및 유동성이 우수한 에틸렌-프로필렌 블록공중합체계 폴리프로필렌 수지 조성물 |
| SG182828A1 (en) * | 2010-02-19 | 2012-09-27 | Exxonmobil Chem Patents Inc | Elastomeric polymer blends and processes for their production |
| EP2655506B1 (de) | 2010-12-21 | 2016-06-15 | Basell Polyolefine GmbH | Polypropylenzusammensetzung mit hoher elastizität und transparenz |
| CN102757614A (zh) * | 2011-04-28 | 2012-10-31 | 北京化工大学 | 一种化妆品用耐低温高抗冲透明聚丙烯材料及其制备方法 |
| CN103649209B (zh) | 2011-07-08 | 2016-05-04 | 博瑞立斯有限公司 | 多相共聚物 |
| ES2569733T3 (es) | 2013-07-12 | 2016-05-12 | Borealis Ag | Copolímero heterofásico |
| KR101501835B1 (ko) * | 2013-08-13 | 2015-03-12 | 삼성토탈 주식회사 | 내백화성 및 내충격성이 우수한 폴리프로필렌 수지 조성물 |
| CN104558811A (zh) * | 2013-10-10 | 2015-04-29 | 中国石油化工股份有限公司 | 一种聚丙烯组合物及其制备方法和应用 |
| EP3083819B1 (de) | 2013-12-20 | 2019-01-30 | Saudi Basic Industries Corporation | Polyolefinzusammensetzung |
| US10696829B2 (en) | 2013-12-20 | 2020-06-30 | Saudi Basic Industries Corporation | Heterophasic propylene copolymer |
| PL2891667T3 (pl) | 2014-01-07 | 2017-07-31 | Borealis Ag | Heterofazowy polimer polipropylenu |
| CN103923392A (zh) * | 2014-04-29 | 2014-07-16 | 广东溢达纺织有限公司 | 耐低温聚丙烯服装包装薄膜及其制备方法 |
| WO2016038211A1 (en) | 2014-09-12 | 2016-03-17 | Borealis Ag | Process for the preparation of copolymers of propylene |
| EP2995629B1 (de) | 2014-09-12 | 2018-03-07 | Borealis AG | Verfahren zur Herstellung von Propylencopolymeren in Gasphase |
| PL3212713T5 (pl) | 2014-10-27 | 2022-10-10 | Borealis Ag | Heterofazowy polipropylen o poprawionej równowadze udarność/sztywność, poprawionej sypkości proszku, zmniejszonych emisjach i niskim skurczu |
| EP3015503A1 (de) | 2014-10-27 | 2016-05-04 | Borealis AG | Heterophasisches Polypropylen mit verbesserter Steifheit/Schlagfestigkeitsbilanz |
| EP3015504A1 (de) | 2014-10-27 | 2016-05-04 | Borealis AG | Heterophasisches Polypropylen mit verbessertem Punktions- bzw. Schlagzähigkeits-/Steifigkeitsgleichgewicht |
| ES2974283T3 (es) | 2017-10-25 | 2024-06-26 | Borealis Ag | Composición de polipropileno cargado con propiedades termo-mecánicas mejoradas |
| CN107903499A (zh) * | 2017-12-04 | 2018-04-13 | 天津科技大学 | 一种透明增韧改性聚丙烯塑料及其制备 |
| JP7376500B2 (ja) * | 2018-04-18 | 2023-11-08 | ダブリュー・アール・グレース・アンド・カンパニー-コーン | 耐衝撃性を有する透明ポリプロピレンコポリマー組成物 |
| JP7153464B2 (ja) | 2018-04-27 | 2022-10-14 | サンアロマー株式会社 | ポリプロピレン組成物および成形体 |
| WO2020106172A1 (en) * | 2018-11-21 | 2020-05-28 | Public Joint Stock Company "Sibur Holding" | Transparent, tasily flow able high-impact polypropylene composition |
| JP2021066825A (ja) | 2019-10-24 | 2021-04-30 | サンアロマー株式会社 | ポリプロピレン組成物および成形体 |
| CN116829605B (zh) * | 2021-01-22 | 2025-10-24 | 博里利斯股份公司 | 纤维增强聚丙烯组合物 |
| CN118843645A (zh) * | 2022-03-21 | 2024-10-25 | 北欧化工公司 | 玻璃纤维增强聚丙烯组合物 |
Family Cites Families (22)
| Publication number | Priority date | Publication date | Assignee | Title |
|---|---|---|---|---|
| US5280074A (en) * | 1989-12-21 | 1994-01-18 | Hoechst Ag | Process for the preparation of a polypropylene molding composition |
| DE3942365A1 (de) * | 1989-12-21 | 1991-06-27 | Hoechst Ag | Verfahren zur herstellung einer polypropylen-formmasse |
| DE4317655A1 (de) * | 1993-05-27 | 1994-12-01 | Basf Ag | Mehrphasige Blockcopolymerisate des Propylens |
| DE4330667A1 (de) * | 1993-09-10 | 1995-03-16 | Basf Ag | Verfahren zur Herstellung von mehrphasigen Homo- oder Copolymerisaten von C¶2¶-C¶1¶¶0¶-Alk-1-enen in einer Reaktionszone |
| IT1275404B1 (it) * | 1994-02-07 | 1997-08-05 | Spherilene Srl | Composizioni poliolefiniche utilizzabili per la preparazione di articoli per uso biomedicale |
| US5773516A (en) * | 1995-12-06 | 1998-06-30 | Basf Aktiengesellschaft | Propylene polymers |
| US6583227B2 (en) * | 1996-09-04 | 2003-06-24 | Exxonmobil Chemical Patents Inc. | Propylene polymers for films |
| DE69713343T2 (de) * | 1996-09-04 | 2002-10-10 | Exxonmobil Chemical Patents Inc., Baytown | Verbesserte propylenpolymere für orientierte filme |
| DE19653079A1 (de) * | 1996-12-19 | 1998-06-25 | Basf Ag | Verfahren zur Gasphasenpolymerisation von C¶2¶-C¶8¶-Alk-1-enen mittels Ziegler -Natta- oder Metallocen-Katalysatorsystemen |
| TW400341B (en) * | 1997-05-22 | 2000-08-01 | Chisso Corp | Propyene polymer blends, processes of producing the same, and polypropylene resin compositions |
| DE19726796A1 (de) * | 1997-06-24 | 1999-01-07 | Basf Ag | Propylenpolymerisate |
| DE19733017A1 (de) * | 1997-07-31 | 1999-02-04 | Hoechst Ag | Chemische Verbindung |
| US6635715B1 (en) * | 1997-08-12 | 2003-10-21 | Sudhin Datta | Thermoplastic polymer blends of isotactic polypropylene and alpha-olefin/propylene copolymers |
| DE19812229A1 (de) * | 1998-03-20 | 1999-09-23 | Basf Ag | Polymere des Propens |
| CA2299390A1 (en) * | 1998-06-05 | 1999-12-16 | Japan Polychem Corporation | Propylene block copolymer and propylene resin composition |
| WO2000011079A1 (en) * | 1998-08-21 | 2000-03-02 | Chisso Corporation | Polypropylene film abd multilayered polypropylene film |
| JP4346182B2 (ja) * | 1999-12-14 | 2009-10-21 | 株式会社プライムポリマー | 二軸延伸フィルム |
| AU1863201A (en) * | 1999-12-21 | 2001-07-03 | Basell Polyolefine Gmbh | Partly crystalline propylene polymerisate composition for production of biaxial-stretched polypropylene films |
| DE19962130A1 (de) * | 1999-12-21 | 2001-07-05 | Basell Polypropylen Gmbh | Teilkristalline Propylenpolymerisat-Zusammensetzungen mit guter Eignung zur Herstellung von biaxial orientierten Folien |
| WO2001048034A2 (de) * | 1999-12-23 | 2001-07-05 | Basell Polyolefine Gmbh | Übergangsmetallverbindung, ligandensystem, katalysatorsystem und seine verwendung zur polymerisation und copolymerisation von olefinen |
| US6586528B1 (en) * | 2000-11-15 | 2003-07-01 | Polypropylene Belgium (Naamlose Vennootshap) | Composition based on propylene polymers and process for obtaining same |
| WO2003106523A1 (en) * | 2002-06-01 | 2003-12-24 | Basell Polyolefine Gmbh | Flexible propylene copolymer compositions having a high transparency |
-
2003
- 2003-06-10 ES ES03738009T patent/ES2291651T3/es not_active Expired - Lifetime
- 2003-06-10 BR BRPI0311863-0B1A patent/BR0311863B1/pt active IP Right Grant
- 2003-06-10 CN CN03813426.8A patent/CN1290917C/zh not_active Expired - Lifetime
- 2003-06-10 DE DE60316437T patent/DE60316437T2/de not_active Expired - Lifetime
- 2003-06-10 JP JP2004513375A patent/JP2005529227A/ja active Pending
- 2003-06-10 US US10/517,580 patent/US20060167185A1/en not_active Abandoned
- 2003-06-10 RU RU2005100045/04A patent/RU2337114C2/ru not_active IP Right Cessation
- 2003-06-10 EP EP03738009A patent/EP1511803B1/de not_active Revoked
- 2003-06-10 CA CA002483206A patent/CA2483206A1/en not_active Abandoned
- 2003-06-10 AT AT03738009T patent/ATE373692T1/de not_active IP Right Cessation
- 2003-06-10 WO PCT/EP2003/006043 patent/WO2003106553A1/en not_active Ceased
- 2003-06-10 AU AU2003245926A patent/AU2003245926B2/en not_active Ceased
- 2003-06-11 AR ARP030102077A patent/AR040187A1/es unknown
Also Published As
| Publication number | Publication date |
|---|---|
| DE60316437T2 (de) | 2008-06-26 |
| EP1511803A1 (de) | 2005-03-09 |
| CN1290917C (zh) | 2006-12-20 |
| ATE373692T1 (de) | 2007-10-15 |
| US20060167185A1 (en) | 2006-07-27 |
| CA2483206A1 (en) | 2003-12-24 |
| RU2337114C2 (ru) | 2008-10-27 |
| CN1659224A (zh) | 2005-08-24 |
| AR040187A1 (es) | 2005-03-16 |
| ES2291651T3 (es) | 2008-03-01 |
| RU2005100045A (ru) | 2005-06-27 |
| EP1511803B1 (de) | 2007-09-19 |
| BR0311863B1 (pt) | 2013-11-26 |
| AU2003245926B2 (en) | 2007-11-29 |
| BR0311863A (pt) | 2005-03-15 |
| WO2003106553A1 (en) | 2003-12-24 |
| AU2003245926A1 (en) | 2003-12-31 |
| JP2005529227A (ja) | 2005-09-29 |
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