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DE606850C - Process for generating firmly adhering galvanic deposits on aluminum and its alloys - Google Patents

Process for generating firmly adhering galvanic deposits on aluminum and its alloys

Info

Publication number
DE606850C
DE606850C DE1930S0011530 DES0011530A DE606850C DE 606850 C DE606850 C DE 606850C DE 1930S0011530 DE1930S0011530 DE 1930S0011530 DE S0011530 A DES0011530 A DE S0011530A DE 606850 C DE606850 C DE 606850C
Authority
DE
Germany
Prior art keywords
aluminum
alloys
firmly adhering
generating
galvanic
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
DE1930S0011530
Other languages
German (de)
Inventor
Dr Johannes Fischer
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
Siemens Corp
Original Assignee
Siemens Corp
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Siemens Corp filed Critical Siemens Corp
Priority to DE1930S0011530 priority Critical patent/DE606850C/en
Priority to DES99296D priority patent/DE610689C/en
Priority to US572440A priority patent/US1947981A/en
Priority to FR725848D priority patent/FR725848A/en
Priority to GB30791/31A priority patent/GB385067A/en
Priority to DES104429D priority patent/DE611643C/en
Priority to DES108305D priority patent/DE610206C/en
Priority to US665741A priority patent/US1968483A/en
Priority to GB11207/33A priority patent/GB394637A/en
Priority to FR43472D priority patent/FR43472E/en
Priority to NL67186A priority patent/NL36860C/xx
Priority to BE399452D priority patent/BE399452A/xx
Priority to FR44190D priority patent/FR44190E/en
Priority to GB31263/33A priority patent/GB404251A/en
Priority to US709349A priority patent/US2036962A/en
Application granted granted Critical
Publication of DE606850C publication Critical patent/DE606850C/en
Expired legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C25ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25DPROCESSES FOR THE ELECTROLYTIC OR ELECTROPHORETIC PRODUCTION OF COATINGS; ELECTROFORMING; APPARATUS THEREFOR
    • C25D5/00Electroplating characterised by the process; Pretreatment or after-treatment of workpieces
    • C25D5/34Pretreatment of metallic surfaces to be electroplated
    • C25D5/42Pretreatment of metallic surfaces to be electroplated of light metals
    • C25D5/44Aluminium
    • CCHEMISTRY; METALLURGY
    • C25ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25DPROCESSES FOR THE ELECTROLYTIC OR ELECTROPHORETIC PRODUCTION OF COATINGS; ELECTROFORMING; APPARATUS THEREFOR
    • C25D11/00Electrolytic coating by surface reaction, i.e. forming conversion layers
    • C25D11/02Anodisation
    • C25D11/04Anodisation of aluminium or alloys based thereon
    • C25D11/06Anodisation of aluminium or alloys based thereon characterised by the electrolytes used
    • CCHEMISTRY; METALLURGY
    • C25ELECTROLYTIC OR ELECTROPHORETIC PROCESSES; APPARATUS THEREFOR
    • C25DPROCESSES FOR THE ELECTROLYTIC OR ELECTROPHORETIC PRODUCTION OF COATINGS; ELECTROFORMING; APPARATUS THEREFOR
    • C25D11/00Electrolytic coating by surface reaction, i.e. forming conversion layers
    • C25D11/02Anodisation
    • C25D11/04Anodisation of aluminium or alloys based thereon
    • C25D11/06Anodisation of aluminium or alloys based thereon characterised by the electrolytes used
    • C25D11/08Anodisation of aluminium or alloys based thereon characterised by the electrolytes used containing inorganic acids

Landscapes

  • Chemical & Material Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Electrochemistry (AREA)
  • Materials Engineering (AREA)
  • Metallurgy (AREA)
  • Organic Chemistry (AREA)
  • Inorganic Chemistry (AREA)
  • Electroplating Methods And Accessories (AREA)
  • Electroplating And Plating Baths Therefor (AREA)
  • Chemically Coating (AREA)

Description

Die bekannten Vorbehandlungsverfahren für die Galvanisierung von Aluminium lassen sich in zwei Gruppen zusammenfassen:The well-known pretreatment processes for the galvanization of aluminum leave can be summarized in two groups:

1. Verfahren, die die Oberfläche des Aluminiums durch Beizen mit Säuren, Laugen oder beiden nacheinander von den ihr häufig anhaftenden Unreinheiten und Oxyden zu befreien trachten, und < 1. Processes which seek to remove the impurities and oxides that often adhere to the surface of aluminum by pickling with acids, alkalis or both, and <

2. Verfahren, die dieses Ziel durch Ansieden der Gegenstände in schwermetallhaltigen Lösungen erzielen mit dem Nebeneffekt, daß hierbei die Schwermetalle vermutlich durch Lokalelementwirkung niedergeschlagen werden. 2. Processes that achieve this goal by boiling the objects in solutions containing heavy metals, with the side effect that the heavy metals are presumably precipitated by local element effects.

Alle diese Vorbehandlungen sind aber, wie die Praxis zeigt, nur geeignet, um galvanische Niederschläge mit nur sehr beschränkter Haftfähigkeit auf dem Aluminium zu erzielen. However, as practice shows, all of these pretreatments are only suitable for galvanic treatment To achieve deposits with only very limited adhesion to the aluminum.

Bekannt ist ferner auch die — im Gegensatz zu den anderen Verfahren überraschende — Erzeugung einer schwermetallhaltigen Oxydhaut auf dem zu galvanisierenden Aluminiumgegenstand auf rain chemischem Wege als Vorbereitung für die Galvanisierung, wobei auch die Lokalelementwirkung infolge der leitenden Verbindung des Aluminiums mit Kohleelektroden oder Metall im Oxydationsbade bewußt benutzt worden ist. Die notwendige sekundäre Beseitigung der so erzeugten Oxydhaut blieb aber dem nachträglichen galvanischen Prozeß selbst überlassen, weshalb auch den so erzeugten Niederschlagen nur geringe Haftfähigkeit eigen war.The one, which is surprising in contrast to the other methods, is also known - Creation of an oxide skin containing heavy metals on the aluminum object to be galvanized by chemical means as preparation for electroplating, with the local element effect as a result the conductive connection of aluminum with carbon electrodes or metal in the oxidation bath has been used consciously. The necessary secondary elimination of the so generated Oxide skin was left to the subsequent galvanic process itself, which is why the precipitates thus produced only poor adhesiveness was inherent.

Bekannt ist ferner die Vorbehandlung von zu plattierendem Aluminium mittels Ätzung, die entweder eingangs des Verfahrens oder nach einer mittels Wechselstrom in schwach organisch saurem Bade erzielten Voroxydation durchgeführt werden kann. Doch sind die so erzeugten Produkte matt und zeigen eine rauhe Oberfläche. .The pretreatment of aluminum to be plated by means of etching is also known, either at the beginning of the process or after an alternating current in weak Organically acidic bath pre-oxidation achieved can be carried out. But are the products produced in this way are matt and have a rough surface. .

Die Erfindung betrifft ein dreistufiges Verfahren zur Galvanisierung von Aluminium und seinen Legierungen, nämlich:The invention relates to a three-step process for electroplating aluminum and its alloys, namely:

a) Voroxydation mittels Gleichstrom im sauren Bade,a) pre-oxidation by means of direct current in an acid bath,

b) Behandlung und Vorgalvanisierung in einem Entfettungsbade, das gewisse Schwermetallsalze enthält,b) Treatment and pre-electroplating in a degreasing bath, the certain heavy metal salts contains,

c) Galvanisierung in dem für das niederzuschlagende Metall jeweils praktischsten Elektrolyten.c) Electroplating in the most practical way for the metal to be deposited Electrolytes.

Es zeigte sich, daß bei der Durchführung der Behandlung in einem Entfettungsbad, welches Kupfer, Messing oder ein anderes sich galvanisch ähnlich verhaltendes Metall enthält, bei zweckmäßig über 5 Volt Spannung das niedergeschlagene Metall hauchdünn ist, und daß man darauf andere Metalle, goIt was found that when the treatment was carried out in a degreasing bath, which copper, brass or another galvanically similar metal contains, if the voltage is expediently above 5 volts, the deposited metal is extremely thin is, and that you can use other metals, go

*) Von den: Patentsucher ist als der Erfinder angegeben worden:*) From the: Patent seeker has been specified as the inventor:

Dr. Johannes Fischer in Berlin-CharlotLenburg.Dr. Johannes Fischer in Berlin-CharlotLenburg.

wie Cadmium, Nickel, Kupfer, in besonders festhaftender Form galvanisch niederschlagen kann. Die Gegenstände können in normaler Weise ohne besondere Vorsicht geglänzt werden.such as cadmium, nickel, copper, galvanically deposit in a particularly firmly adhering form can. The objects can be polished in the normal way without special care.

Die der Behandlung im schwermetallhaltigen Entfettungsbade voraufgehende oberflächliche Oxydation der Aluminiumteile wird zweckmäßig in an sich bekannter Weise durch ίο anodische Behandlung derselben in einem eine oxydierende, organische oder anorganische Säure, besonders 30- bis 400/oige Chromsäure mit etwas Schwefelsäure, enthaltenden Bade bei 20 bis 60 Volt vorgenommen.The superficial ones preceding the treatment in the heavy metal degreasing bath Oxidation of the aluminum parts is expedient in a manner known per se by ίο anodic treatment of the same in one an oxidizing, organic or inorganic acid, especially 30 to 400% chromic acid made with a little sulfuric acid, containing bath at 20 to 60 volts.

AusführungsbeispielEmbodiment

Ein Gegenstand aus Reinaluminium, der als Anode in einem Chrombad 15 bis 30 Minuten lang oberflächlich oxydiert wurde, wird gut abgespült und in einem der üblichen Entfettungsbäder mit gleichzeitigemNiederschlagen von Messing bei etwa 6 Volt kathodisch behandelt. Nach 2 bis 3 Alinuten ist so viel Metall niedergeschlagen, daß der Gegenstand in einem der üblichen galvanischen Bäder weiterbehandelt werden kann.An object made of pure aluminum that acts as an anode in a chrome bath for 15 to 30 minutes has been superficially oxidized for a long time, it is rinsed well and in one of the usual degreasing baths with simultaneous deposition of brass at about 6 volts cathodically treated. After 2 to 3 minutes, so much metal is deposited that the object can be further treated in one of the usual galvanic baths.

Claims (1)

Patentanspruch:Claim: Verfahren zur Erzeugung festhaftender galvanischer Niederschläge auf Aluminium und dessen Legierungen, wobei zunächst eine Aluminiumoxydschicht auf elektrolytischem Wege erzeugt wird, dadurch gekennzeichnet, daß das durch anodische Oxydation mittels Gleichstrom entstandene Aluminiumoxydhäutchen unter gleichzeitiger Abscheidung von Kupfer. Messing oder einem sich galvanisch gleich verhaltenden Metall in einem Entfettungsbade behandelt und darauf erst der gewünschte galvanische Überzug abgeschieden wird. Process for the production of firmly adhering galvanic deposits on aluminum and its alloys, whereby an aluminum oxide layer is first produced by electrolytic means characterized in that the aluminum oxide membrane formed by anodic oxidation by means of direct current under simultaneous deposition of copper. Brass or electroplated metal with the same behavior is treated in a degreasing bath and only then is the desired galvanic coating deposited.
DE1930S0011530 1930-11-07 1930-11-07 Process for generating firmly adhering galvanic deposits on aluminum and its alloys Expired DE606850C (en)

Priority Applications (15)

Application Number Priority Date Filing Date Title
DE1930S0011530 DE606850C (en) 1930-11-07 1930-11-07 Process for generating firmly adhering galvanic deposits on aluminum and its alloys
DES99296D DE610689C (en) 1930-11-07 1931-06-21 Process for achieving firmly adhering galvanic deposits on aluminum and its alloys
US572440A US1947981A (en) 1930-11-07 1931-10-31 Plating aluminum
FR725848D FR725848A (en) 1930-11-07 1931-11-06 Production process, on aluminum and its alloys, of strongly adhering galvanic deposits
GB30791/31A GB385067A (en) 1930-11-07 1931-11-06 An improved method of producing firmly adherent galvanic deposits on aluminium and its alloys
DES104429D DE611643C (en) 1930-11-07 1932-05-01 Process for generating galvanic deposits on aluminum and its alloys
DES108305D DE610206C (en) 1930-11-07 1933-02-16 Process for the production of firmly adhering galvanic deposits on aluminum and its alloys
US665741A US1968483A (en) 1930-11-07 1933-04-12 Plating aluminium and its alloys
GB11207/33A GB394637A (en) 1930-11-07 1933-04-13 Method of producing galvanic deposits on aluminium and its alloys
FR43472D FR43472E (en) 1930-11-07 1933-04-18 Production process, on aluminum and its alloys, of strongly adhering galvanic deposits
NL67186A NL36860C (en) 1930-11-07 1933-10-27
BE399452D BE399452A (en) 1930-11-07 1933-11-02
FR44190D FR44190E (en) 1930-11-07 1933-11-03 Production process, on aluminum and its alloys, of strongly adhering galvanic deposits
GB31263/33A GB404251A (en) 1930-11-07 1933-11-09 Method of producing firmly adherent galvanic deposits on aluminium and its alloys
US709349A US2036962A (en) 1930-11-07 1934-02-01 Method for production of firmly adhering galvanic coatings on aluminum and aluminum alloys

Applications Claiming Priority (3)

Application Number Priority Date Filing Date Title
DE1930S0011530 DE606850C (en) 1930-11-07 1930-11-07 Process for generating firmly adhering galvanic deposits on aluminum and its alloys
DES104429D DE611643C (en) 1930-11-07 1932-05-01 Process for generating galvanic deposits on aluminum and its alloys
DES108305D DE610206C (en) 1930-11-07 1933-02-16 Process for the production of firmly adhering galvanic deposits on aluminum and its alloys

Publications (1)

Publication Number Publication Date
DE606850C true DE606850C (en) 1934-12-12

Family

ID=40626731

Family Applications (4)

Application Number Title Priority Date Filing Date
DE1930S0011530 Expired DE606850C (en) 1930-11-07 1930-11-07 Process for generating firmly adhering galvanic deposits on aluminum and its alloys
DES99296D Expired DE610689C (en) 1930-11-07 1931-06-21 Process for achieving firmly adhering galvanic deposits on aluminum and its alloys
DES104429D Expired DE611643C (en) 1930-11-07 1932-05-01 Process for generating galvanic deposits on aluminum and its alloys
DES108305D Expired DE610206C (en) 1930-11-07 1933-02-16 Process for the production of firmly adhering galvanic deposits on aluminum and its alloys

Family Applications After (3)

Application Number Title Priority Date Filing Date
DES99296D Expired DE610689C (en) 1930-11-07 1931-06-21 Process for achieving firmly adhering galvanic deposits on aluminum and its alloys
DES104429D Expired DE611643C (en) 1930-11-07 1932-05-01 Process for generating galvanic deposits on aluminum and its alloys
DES108305D Expired DE610206C (en) 1930-11-07 1933-02-16 Process for the production of firmly adhering galvanic deposits on aluminum and its alloys

Country Status (6)

Country Link
US (3) US1947981A (en)
BE (1) BE399452A (en)
DE (4) DE606850C (en)
FR (3) FR725848A (en)
GB (3) GB385067A (en)
NL (1) NL36860C (en)

Families Citing this family (23)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2430468A (en) * 1943-11-08 1947-11-11 Bell Telephone Labor Inc Electroplating silver on aluminum and its alloys
US2422903A (en) * 1944-04-21 1947-06-24 Western Electric Co Process for electrolytically treating stainless steel articles
US2473163A (en) * 1945-06-25 1949-06-14 Ewald H Mccoy Plating nickel on aluminum
US2541083A (en) * 1945-08-25 1951-02-13 Sperry Corp Electroplating on aluminum
US2496845A (en) * 1946-06-10 1950-02-07 Chrysler Corp Bath for brass immersion coating on aluminum and aluminum alloy
US2495941A (en) * 1946-12-18 1950-01-31 Reynolds Metals Co Electroplating copper on aluminum
US2721835A (en) * 1951-07-07 1955-10-25 Shwayder Bros Inc Surface treatment of aluminum articles
US2798037A (en) * 1953-05-13 1957-07-02 Sprague Electric Co Aluminum oxide films
BE559886A (en) * 1956-08-08
DE1546005B1 (en) * 1964-02-27 1971-01-21 Schmidt Gmbh Karl Treatment of sliding surfaces with chemically or galvanically coated surfaces
US3531379A (en) * 1965-07-28 1970-09-29 Micral Ind Inc Process of coating aluminum with other metals
US3929594A (en) * 1973-05-18 1975-12-30 Fromson H A Electroplated anodized aluminum articles
US4085012A (en) * 1974-02-07 1978-04-18 The Boeing Company Method for providing environmentally stable aluminum surfaces for adhesive bonding and product produced
US4021592A (en) * 1974-03-07 1977-05-03 Fromson H A Process of making electroplated anodized aluminum articles and electroless plating
US4159229A (en) * 1977-06-03 1979-06-26 Ford Motor Company Method of plating light weight metal to enhance lateral corrosion resistance
US4157941A (en) * 1977-06-03 1979-06-12 Ford Motor Company Method of adherency of electrodeposits on light weight metals
US4914081A (en) * 1988-01-15 1990-04-03 American Telephone And Telegraph Company, At&T Bell Laboratories Process for making metallized structure and article comprising structure
US5466360A (en) * 1994-10-13 1995-11-14 Robert Z. Reath Method for preparing aluminum for subsequent electroplating
JP4194143B2 (en) * 1998-10-09 2008-12-10 株式会社神戸製鋼所 Aluminum alloy material with excellent gas and plasma corrosion resistance
US20040072011A1 (en) * 2002-10-10 2004-04-15 Centro De Investigaciq Materiales Avanzados, S.C. Electroless brass plating method and product-by-process
US20060254922A1 (en) * 2005-03-21 2006-11-16 Science & Technology Corporation @ Unm Method of depositing films on aluminum alloys and films made by the method
DE102016113641A1 (en) 2016-07-25 2018-01-25 Christian-Albrechts-Universität Zu Kiel Aluminum-copper connector having a heterostructure and method of making the heterostructure
US11261533B2 (en) 2017-02-10 2022-03-01 Applied Materials, Inc. Aluminum plating at low temperature with high efficiency

Also Published As

Publication number Publication date
US2036962A (en) 1936-04-07
GB394637A (en) 1933-06-29
GB385067A (en) 1932-12-22
BE399452A (en) 1933-12-30
US1968483A (en) 1934-07-31
DE610206C (en) 1935-03-06
US1947981A (en) 1934-02-20
GB404251A (en) 1934-01-11
FR725848A (en) 1932-05-18
NL36860C (en) 1935-11-15
DE610689C (en) 1935-03-14
FR43472E (en) 1934-06-07
DE611643C (en) 1935-04-02
FR44190E (en) 1934-11-20

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