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DE518929C - Process for the preparation of aromatic amines - Google Patents

Process for the preparation of aromatic amines

Info

Publication number
DE518929C
DE518929C DEI30357D DEI0030357D DE518929C DE 518929 C DE518929 C DE 518929C DE I30357 D DEI30357 D DE I30357D DE I0030357 D DEI0030357 D DE I0030357D DE 518929 C DE518929 C DE 518929C
Authority
DE
Germany
Prior art keywords
preparation
aromatic amines
iron
solution
reduction
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Expired
Application number
DEI30357D
Other languages
German (de)
Inventor
Dr Julius Laux
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
IG Farbenindustrie AG
Original Assignee
IG Farbenindustrie AG
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by IG Farbenindustrie AG filed Critical IG Farbenindustrie AG
Priority to DEI30357D priority Critical patent/DE518929C/en
Application granted granted Critical
Publication of DE518929C publication Critical patent/DE518929C/en
Expired legal-status Critical Current

Links

Classifications

    • CCHEMISTRY; METALLURGY
    • C09DYES; PAINTS; POLISHES; NATURAL RESINS; ADHESIVES; COMPOSITIONS NOT OTHERWISE PROVIDED FOR; APPLICATIONS OF MATERIALS NOT OTHERWISE PROVIDED FOR
    • C09CTREATMENT OF INORGANIC MATERIALS, OTHER THAN FIBROUS FILLERS, TO ENHANCE THEIR PIGMENTING OR FILLING PROPERTIES ; PREPARATION OF CARBON BLACK  ; PREPARATION OF INORGANIC MATERIALS WHICH ARE NO SINGLE CHEMICAL COMPOUNDS AND WHICH ARE MAINLY USED AS PIGMENTS OR FILLERS
    • C09C1/00Treatment of specific inorganic materials other than fibrous fillers; Preparation of carbon black
    • C09C1/22Compounds of iron
    • C09C1/24Oxides of iron

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)

Description

Verfahren zur Herstellung aromatischer Amine Durch das Hauptpatent 515 758 und das frühere Zusatzpatent 5 16 999 ist ein Verfahren geschützt, welches gestattet, das. bei der Reduktion von aromatischen Nitroverbindungen zu den entsprechendenAminen verwendete Eisen in Form eines technisch zur Herstellung von Pigmentfarben wertvollen Hydroxyds wiederzugewinnen und das darin besteht, die Reduktion in Gegenwart von wäßrigen Lösungen der Salze des Aluminiums oder anderer drei- und vierwertiger Metalle auszuführen.Process for the production of aromatic amines The main patent 515 758 and the earlier additional patent 5 1 6 999 protect a process which allows the iron used in the reduction of aromatic nitro compounds to the corresponding amines to be recovered in the form of a hydroxide which is technically valuable for the production of pigment colors and that consists in carrying out the reduction in the presence of aqueous solutions of the salts of aluminum or of other trivalent and tetravalent metals.

Es wurde weiter gefunden, daß man an Stelle der wäßr igen Lösungen von Salzen auch die fertig gebildeten Hydroxv_ de oder Oxyde oder deren schwerlösliche basische Salze, zweckmäßig in möglichst feiner, bis zu kolloidaler Verteilung in Wasser aufgeschlämtnt, verwenden und dabei im wesentlichen zu den gleichen Ergebnissen gelangen kann.It has also been found that instead of the aqueous solutions of salts also the completely formed hydroxides or oxides or their sparingly soluble basic salts, expediently in the finest possible, up to colloidal distribution in Slurried water, using it, and doing essentially the same results can get.

Beispiel r Aus einer Lösung von .4o kg wasserhalti-g e M Aluminiumsulfat in 3001 Wasser wird mittels der erforderlichen Menge Natriumcarbonatlösung das Aluminium in Form eines hochbasischen unlöslichen Sulfats in feiner Verteilung ausgefällt. Ohne die Lösung vom Niederschlag zu trennen, gibt man sie zu 200 kg Eisen, fügt eine konzentrierte Lösung von 6o kg Anilinhydrochlorid hinzu und läßt in der bei der Reduktion zu Anilin sonst üblichen Weise Zoo kg Nitrobenzol allmählich unter Rühren bei Siedetemperatur zufließen. Man erhält nach Entfernung des Anilins ein bräunlichgelbes Eiseihvdroz-\,c.t, das beim Brennen ein rotes Oxyd ergibt.Example r from a solution of .4o kg wasserhalti- g e M aluminum sulfate in 3001, water is precipitated, the aluminum in the form of a highly basic sulphate insoluble in fine distribution by means of the required amount of sodium carbonate solution. Without separating the solution from the precipitate, it is added to 200 kg of iron, a concentrated solution of 60 kg of aniline hydrochloride is added, and zoo kg of nitrobenzene is gradually added in the usual way for reduction to aniline while stirring at the boiling point. After the aniline has been removed, a brownish-yellow ice cream is obtained, which on firing gives a red oxide.

Beispiel e Aus einer Lösung von ro kg Cerchlorid in z So l Wasser wird durch Zusatz von d.o kg Anilin unter Rühren das Cer in Form eines fein verteilten Hydroxyds ausgefällt. Man fügt dann Zoo kg Nitrobenzol hinzu und reduziert in bekannter `'eise durch allmähliche Zugabe von Zoo kg Eisen. Man erhält als Rückstand ein Eisenh_vdrox_vd von braunroter Farbe.Example e From a solution of ro kg cerium chloride in z sol water by adding d.o kg of aniline while stirring the cerium in the form of a finely divided Hydroxyds precipitated. Then zoo kg of nitrobenzene is added and reduced to a known value by the gradual addition of zoo kg of iron. A Eisenh_vdrox_vd is obtained as the residue of brownish red color.

Beispiel 3 Zu einer Lösung von 4o kg Eisenchlorid in i 6o l Wasser fügt man 26 kg gemahlene Kreide und Zoo kg Nitrobenzol, worauf man mittels 22j kg Eisen wie in Beispiel 2 reduziert und aufarbeitet.Example 3 To a solution of 40 kg of iron chloride in 16o l of water add 26 kg of ground Chalk and zoo kg nitrobenzene, what one reduced and worked up using 22j kg of iron as in Example 2.

Claims (1)

PATRNTANSPRUCI3: Abänderung des durch Patent 515 758 und das frühere Zusatzpatent 5 I6 999 geschützten Verfahrens zur Herstellung aromatischer Amine durch Reduktion der entsprechenden Nitroverbindungen mit Eisen, darin bestehend, daß man hier die Reduktion in Gegenwart von wäßri;gen Suspensionen schwerläslicher Oxyde, Hydroxyde oder basischer Salze drei- oder vierwertiger Metalle bewirkt.PATRNTANSPRUCI3: Modification of the process, protected by patent 515 758 and the earlier additional patent 5 16 999 , for the preparation of aromatic amines by reducing the corresponding nitro compounds with iron, consisting in the reduction in the presence of aqueous suspensions of poorly soluble oxides, hydroxides or basic ones Trivalent or tetravalent metal salts.
DEI30357D 1927-02-16 1927-02-16 Process for the preparation of aromatic amines Expired DE518929C (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
DEI30357D DE518929C (en) 1927-02-16 1927-02-16 Process for the preparation of aromatic amines

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
DEI30357D DE518929C (en) 1927-02-16 1927-02-16 Process for the preparation of aromatic amines

Publications (1)

Publication Number Publication Date
DE518929C true DE518929C (en) 1931-02-21

Family

ID=7187599

Family Applications (1)

Application Number Title Priority Date Filing Date
DEI30357D Expired DE518929C (en) 1927-02-16 1927-02-16 Process for the preparation of aromatic amines

Country Status (1)

Country Link
DE (1) DE518929C (en)

Cited By (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE2826941A1 (en) * 1978-06-20 1980-01-10 Bayer Ag METHOD FOR PRODUCING IRON OXIDE RED PIGMENTS
US5665157A (en) * 1995-10-26 1997-09-09 Bayer Ag Clean color shade, yellow-tinged red iron oxide pigments, and a process for their manufacture, and their use
JPH11240724A (en) * 1997-11-19 1999-09-07 Bayer Ag Iron oxide yellow pigment stable to heat
US7235127B2 (en) 2004-12-14 2007-06-26 Lanxess Deutschland Gmbh Reduction- and oxidation-stable iron oxide black pigments having high colour strength for colouring plastics and building materials, their preparation and their use

Cited By (4)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE2826941A1 (en) * 1978-06-20 1980-01-10 Bayer Ag METHOD FOR PRODUCING IRON OXIDE RED PIGMENTS
US5665157A (en) * 1995-10-26 1997-09-09 Bayer Ag Clean color shade, yellow-tinged red iron oxide pigments, and a process for their manufacture, and their use
JPH11240724A (en) * 1997-11-19 1999-09-07 Bayer Ag Iron oxide yellow pigment stable to heat
US7235127B2 (en) 2004-12-14 2007-06-26 Lanxess Deutschland Gmbh Reduction- and oxidation-stable iron oxide black pigments having high colour strength for colouring plastics and building materials, their preparation and their use

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