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DE10137564A1 - Screening for drugs in a human or animal, comprises taking the condensation from exhaled breath, to be prepared for quantitative and qualitative analysis on site or to give a sample for a laboratory - Google Patents

Screening for drugs in a human or animal, comprises taking the condensation from exhaled breath, to be prepared for quantitative and qualitative analysis on site or to give a sample for a laboratory

Info

Publication number
DE10137564A1
DE10137564A1 DE2001137564 DE10137564A DE10137564A1 DE 10137564 A1 DE10137564 A1 DE 10137564A1 DE 2001137564 DE2001137564 DE 2001137564 DE 10137564 A DE10137564 A DE 10137564A DE 10137564 A1 DE10137564 A1 DE 10137564A1
Authority
DE
Germany
Prior art keywords
drugs
analysis
condensation
human
animal
Prior art date
Legal status (The legal status is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the status listed.)
Ceased
Application number
DE2001137564
Other languages
German (de)
Inventor
Michael Rothe
Gunther Becher
Current Assignee (The listed assignees may be inaccurate. Google has not performed a legal analysis and makes no representation or warranty as to the accuracy of the list.)
FILT LUNGEN und THORAXDIAGNOST
FILT LUNGEN und THORAXDIAGNOSTIK GmbH
Original Assignee
FILT LUNGEN und THORAXDIAGNOST
FILT LUNGEN und THORAXDIAGNOSTIK GmbH
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by FILT LUNGEN und THORAXDIAGNOST, FILT LUNGEN und THORAXDIAGNOSTIK GmbH filed Critical FILT LUNGEN und THORAXDIAGNOST
Priority to DE2001137564 priority Critical patent/DE10137564A1/en
Publication of DE10137564A1 publication Critical patent/DE10137564A1/en
Ceased legal-status Critical Current

Links

Classifications

    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N33/00Investigating or analysing materials by specific methods not covered by groups G01N1/00 - G01N31/00
    • G01N33/48Biological material, e.g. blood, urine; Haemocytometers
    • G01N33/483Physical analysis of biological material
    • G01N33/497Physical analysis of biological material of gaseous biological material, e.g. breath
    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N1/00Sampling; Preparing specimens for investigation
    • G01N1/02Devices for withdrawing samples
    • G01N1/22Devices for withdrawing samples in the gaseous state
    • G01N2001/2282Devices for withdrawing samples in the gaseous state with cooling means
    • GPHYSICS
    • G01MEASURING; TESTING
    • G01NINVESTIGATING OR ANALYSING MATERIALS BY DETERMINING THEIR CHEMICAL OR PHYSICAL PROPERTIES
    • G01N1/00Sampling; Preparing specimens for investigation
    • G01N1/28Preparing specimens for investigation including physical details of (bio-)chemical methods covered elsewhere, e.g. G01N33/50, C12Q
    • G01N1/40Concentrating samples
    • G01N1/4022Concentrating samples by thermal techniques; Phase changes
    • G01N2001/4033Concentrating samples by thermal techniques; Phase changes sample concentrated on a cold spot, e.g. condensation or distillation

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  • Health & Medical Sciences (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Engineering & Computer Science (AREA)
  • Molecular Biology (AREA)
  • Physics & Mathematics (AREA)
  • Biomedical Technology (AREA)
  • Chemical & Material Sciences (AREA)
  • Urology & Nephrology (AREA)
  • Hematology (AREA)
  • Biophysics (AREA)
  • Food Science & Technology (AREA)
  • Medicinal Chemistry (AREA)
  • Analytical Chemistry (AREA)
  • Biochemistry (AREA)
  • General Health & Medical Sciences (AREA)
  • General Physics & Mathematics (AREA)
  • Immunology (AREA)
  • Pathology (AREA)
  • Investigating Or Analysing Biological Materials (AREA)

Abstract

Establishing the qualitative and quantitative presence of pharmaceuticals or drugs, in a human or animal body, comprising recovering condensation from exhaled breath and analyzing it, is new. To establish the qualitative and quantitative presence of pharmaceuticals or drugs, in a human or animal body, the condensation is recovered from exhaled breath and taken for analysis. Before analysis, the condensation is filtered through a filter material with a surface which has been modified or not. Before analysis, the condensation passes through an extraction process using an organic solvent, supercritical fluids or modified solid phases, and volatile components are removed by evaporation. Before analysis, protein bonds are separated, and sulfuric acid or gluconic acid esters are separated by a hydrolysis reaction. The residue is analyzed using chromatography, and colorimetry with detectors or biosensors.

Description

Gegenwärtig ist für eine genaue Bestimmung und damit etwa der Feststellung einer Beeinträchtigung der Fahrtauglichkeit infolge des Vorhandenseins von Arzneimitteln oder Drogen oder eines Verstoßes gegen das Betäubungsmittelgesetz die Blutentnahme oder die Gewinnung von Urin erforderlich. Für die Blutentnahme muss in der Regel eine Klink aufgesucht werden, die Uringewinnung ist durch den Patienten relativ leicht manipulierbar. Dies sind wesentliche Nachteile. At present there is one for an exact determination and thus about the determination Impairment of roadworthiness due to the presence of drugs or Drugs or a violation of the Narcotics Act the collection of urine is required. A clinic is usually required for blood sampling the urine is relatively easy to obtain by the patient manipulated. These are major drawbacks.

Weiterhin ist die Nutzung der Ausatemluft zur Feststellung einer Beeinträchtigung der Fahrtauglichkeit infolge des Vorhandenseins von Alkohol bekannt. Alkohol weist bei 37°C einen hohen Dampfdruck auf, so dass schon geringe Luftmengen eine für die Analyse ausreichende messbare Menge Alkohol aufweisen. Dies ist bei Arzneimitteln und insbesondere Drogen nicht der Fall, so dass diese Untersuchungsmethode ausscheidet. Furthermore, the use of exhaled air to determine an impairment of the Driveability known due to the presence of alcohol. Alcohol proves 37 ° C a high vapor pressure, so that even small amounts of air are one for the Analysis have sufficient measurable amount of alcohol. This is with medicines and Drugs in particular are not the case, so this method of examination is ruled out.

Aufgabe der Erfindung ist es, die qualitative und quantitative Feststellung des Vorhandenseins von Arzneimitteln oder Drogen im menschlichen oder tierischen Körper sicher direkt Vorort vorzunehmen, oder eine transportfähige körpereigene Substanz zu gewinnen, die einer späteren Auswertung im Labor unterzogen wird und sichere Messergebnisse liefert. The object of the invention is to determine the qualitative and quantitative of the Presence of drugs or drugs in the human or animal body safely carry out directly on site, or a transportable endogenous substance win, which is subjected to a later evaluation in the laboratory and safe Delivers measurement results.

Gelöst wird diese Aufgabe mit den kennzeichnenden Merkmalen des Verfahrensanspruches 1, vorteilhafte Ausgestaltungen sind Gegenstand der Unteransprüche. This object is achieved with the characterizing features of method claim 1 , advantageous embodiments are the subject of the dependent claims.

Das erfindungsgemäße Verfahren zur qualitativen und quantitativen Feststellung des Vorhandenseins von Arzneimitteln oder Drogen im menschlichen oder tierischen Körper sieht vor, dass als Untersuchungsmedium Atemkondensat, die bei der Ausatmung kondensierende Feuchtigkeit, verwendet wird. The method according to the invention for the qualitative and quantitative determination of the Presence of drugs or drugs in the human or animal body stipulates that as a test medium breathing condensate that occurs during exhalation condensing moisture is used.

Die Fachwelt beschränkte sich in der Vergangenheit bei der Analyse des Atemkondensats auf die Feststellung körpereigener Substanzen, um daraus Schlussfolgerungen im Hinblick auf die Ursache von Beschwerden und Funktionsstörungen zu ziehen. Über Jahre wurde die Möglichkeit der Nutzung des Atemkondensats zur qualitativen und quantitativen Feststellung des Vorhandenseins von Arzneimitteln oder Drogen im menschlichen oder tierischen Körper nicht gesehen. In the past, experts restricted themselves to analyzing the breath condensate on the detection of the body 's own substances in order to draw conclusions from it Draw attention to the cause of complaints and malfunctions. For years was the possibility of using the breath condensate for qualitative and quantitative determination of the presence of drugs or drugs in human or animal body not seen.

Atemkondensat ist prinzipiell nicht invasiv, beliebig oft und auch durch nichtmedizinisches Personal leicht zu gewinnen. Es enthält neben Wasser eine Vielzahl schwer- bzw nichtflüchtiger Substanzen, die größtenteils die biochemische Zusammensetzung der unteren Atemwege widerspiegeln. Derartige Substanzen sind bei Messungen der Ausatemluft wegen der geringen Konzentrationen in der Ausatemluft nicht nachweisbar, zumindest nicht mit vertretbarem apparativen Aufwand. In principle, breath condensate is not invasive, as often as required and also through easy to attract non-medical personnel. In addition to water, it contains a variety of heavy or non-volatile substances, which largely the biochemical composition of the reflect lower respiratory tract. Such substances are used in measurements of Exhaled air cannot be detected due to the low concentrations in the exhaled air, at least not with reasonable expenditure on equipment.

Die messbare Menge derartiger Substanzen läßt sich jedoch im Atemkondensat deutlich erhöhen, da bei der Gewinnung wesentlich größere Mengen der Ausatemluft verarbeitet werden. Daher ist es möglich köperfremde Substanzen, wie Arzneimittel und Drogen, die in der Epithelflüssigkeit vorkommen, im Atemkondensat nachzuweisen. However, the measurable amount of such substances can be clearly seen in the breath condensate increase, since much larger quantities of exhaled air are processed during the extraction become. Therefore, it is possible for foreign substances such as drugs and drugs occur in the epithelial fluid, can be detected in the respiratory condensate.

Die Gewinnung des Atemkondensates kann durch kommerziell verfügbare Geräte erfolgen. The breathing condensate can be obtained by commercially available devices respectively.

Das Atemkondensat wird entweder direkt der Analyse zugeführt oder mit einem oder mehreren der folgenden Verfahren vorbehandelt:

  • - Filtration über oberflächenmodifizierte oder nichtmodifizierte Filtermaterialien;
  • - Extraktion durch organische Lösungsmittel, superkritische Flüssigkeiten
  • - oder modifizierte Festphasen;
  • - Anreicherung der Analysesubstanz durch Verdampfen der flüchtigen Bestandteile des Atemkondensates;
  • - Reaktionen zur Spaltung von Proteinbindungen;
  • - Hydrolysereaktionen zur Spaltung von Schwefelsäure- oder Glucoronsäureestern.
The breath condensate is either fed directly to the analysis or pretreated using one or more of the following methods:
  • - Filtration over surface modified or unmodified filter materials;
  • - extraction by organic solvents, supercritical liquids
  • - or modified solid phases;
  • - Enrichment of the analysis substance by evaporating the volatile components of the breath condensate;
  • - reactions to cleave protein bonds;
  • - Hydrolysis reactions for the cleavage of sulfuric acid or glucoronic acid esters.

Die Analyse selbst erfolgt mittels:

  • - Chromatographischer Verfahren mit verschiedenen Detektoren;
  • - colorimetrischer Verfahren;
  • - unter Verwendung von nach verschiednen Prinzipien funktionierenden Fertigtesten zum Drogenscreening;
  • - mittels immunologisch oder elektrochemisch arbeitender Biosensoren.
The analysis itself is carried out using:
  • - Chromatographic methods with different detectors;
  • - colorimetric method;
  • - using ready-made drug screening tests based on different principles;
  • - Using immunological or electrochemical biosensors.

Die genannten Probenvorbereitungs- und Analyseverfahren können teilweise oder vollständig automatisiert bzw. online oder offline mit der Gewinnung des Atemkondensates durchgeführt werden. The sample preparation and analysis methods mentioned can be partial or fully automated or online or offline with the extraction of the breath condensate be performed.

Neben der qualitativen und quantitativen Feststellung des Vorhandenseins von Arzneimitteln oder Drogen im menschlichen oder tierischen Körper durch die Analyse des Atemkondensates vorort, bietet die konzentrierte Probe auch den Vorteil einer Nachanalyse im Labor. In addition to the qualitative and quantitative determination of the presence of Medicines or drugs in the human or animal body by analyzing the Breathing condensate on site, the concentrated sample also offers the advantage of a Follow-up analysis in the laboratory.

Claims (7)

1. Verfahren zur qualitativen und quantitativen Feststellung des Vorhandenseins von Arzneimitteln oder Drogen im menschlichen oder tierischen Körper, dadurch gekennzeichnet, dass vom betreffenden Menschen oder Tier Atemkondensat gewonnen und einer Analyse unterzogen wird. 1. A method for the qualitative and quantitative determination of the presence of drugs or drugs in the human or animal body, characterized in that breath condensate is obtained from the person or animal in question and subjected to an analysis. 2. Verfahren nach Anspruch 1, dadurch gekennzeichnet, dass das Atemkondensat vor der Analyse einer Filtration über oberflächenmodifizierte oder nichtmodifizierte Filtermaterialien unterzogen wird. 2. The method according to claim 1, characterized in that the breath condensate before analyzing a filtration over surface modified or subjected to unmodified filter materials. 3. Verfahren nach Anspruch 1, dadurch gekennzeichnet, dass das Atemkondensat vor der Analyse einer Extraktion durch organische Lösungsmittel, superkritische Flüssigkeiten oder modifizierte Festphasen unterzogen wird. 3. The method according to claim 1, characterized in that the breath condensate before analyzing an extraction by organic Solvents, supercritical liquids or modified solid phases. 4. Verfahren nach Anspruch 1, dadurch gekennzeichnet, dass vor der Analyse eine Anreichung der Analysesubstanz durch Verdampfen der flüchtigen Bestandteile des Atemkondensates erfolgt. 4. The method according to claim 1, characterized in that before analysis, enrich the analysis substance by evaporating the volatile components of the breath condensate. 5. Verfahren nach Anspruch 1, dadurch gekennzeichnet, dass vor der Analyse Reaktionen zur Spaltung von Proteinbindungen des Atemkondensates erfolgen. 5. The method according to claim 1, characterized in that before analysis, reactions to cleave the protein bonds of the Respiratory condensates take place. 6. Verfahren nach Anspruch 1, dadurch gekennzeichnet, dass vor der Analyse Hydrolysereaktionen zur Spaltung von Schwefelsäure- oder Glucoronsäureestern vorgenommen werden. 6. The method according to claim 1, characterized in that before analysis hydrolysis reactions to cleave sulfuric acid or Glucoronic acid esters are made. 7. Verfahren nach Anspruch 1, dadurch gekennzeichnet, dass
die Analyse mittels
Chromatographischer Verfahren mit verschiedenen Detektoren;
colorimetrischer Verfahren;
unter Verwendung von nach verschiednen Prinzipien funktionierenden Fertigtesten zum Drogenscreening oder
mittels immunologisch oder elektrochemisch arbeitender Biosensoren erfolgt.
7. The method according to claim 1, characterized in that
the analysis by means of
Chromatographic process with different detectors;
colorimetric method;
using ready-made drug screening tests based on different principles or
by means of immunologically or electrochemically working biosensors.
DE2001137564 2001-07-30 2001-07-30 Screening for drugs in a human or animal, comprises taking the condensation from exhaled breath, to be prepared for quantitative and qualitative analysis on site or to give a sample for a laboratory Ceased DE10137564A1 (en)

Priority Applications (1)

Application Number Priority Date Filing Date Title
DE2001137564 DE10137564A1 (en) 2001-07-30 2001-07-30 Screening for drugs in a human or animal, comprises taking the condensation from exhaled breath, to be prepared for quantitative and qualitative analysis on site or to give a sample for a laboratory

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
DE2001137564 DE10137564A1 (en) 2001-07-30 2001-07-30 Screening for drugs in a human or animal, comprises taking the condensation from exhaled breath, to be prepared for quantitative and qualitative analysis on site or to give a sample for a laboratory

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DE10137564A1 true DE10137564A1 (en) 2003-02-27

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Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE102005020102B3 (en) * 2005-04-25 2006-11-30 Universität Potsdam Method and device for obtaining and analyzing respiratory condensates
US10052045B2 (en) 2012-12-21 2018-08-21 Colgate-Palmolive Company Method for testing oral malodor

Citations (12)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
FR2587497A1 (en) * 1985-09-17 1987-03-20 Marelli Autronica ACCELERATION OR VIBRATION SENSOR
EP0269709B1 (en) * 1986-06-14 1992-01-29 LION LABORATORIES plc Alcohol or drugs breath detecting devices
DE9421065U1 (en) * 1994-05-13 1995-05-11 Filt Forschungsgesellschaft für Lungen- und Thoraxerkrankungen mbH, 13125 Berlin Device for collecting exhaled breath condensate
DE19607646A1 (en) * 1996-02-29 1997-09-11 Joerg Volkmann Detection of consumption of hashish or marijuana
DE29712836U1 (en) * 1997-07-10 1997-09-18 Filt Forschungsgesellschaft für Lungen- und Thoraxerkrankungen mbH, 13125 Berlin Condensate trap to collect exhaled breath condensate
DE29803485U1 (en) * 1998-03-04 1998-05-14 Bionorica Arzneimittel GmbH, 92318 Neumarkt Device for determining at least one substance contained in the exhaled air of a living being
DE19718925A1 (en) * 1997-04-28 1998-10-29 Medium Sensor Gmbh Recovery of component fractions from exhaled air
WO1999028743A1 (en) * 1997-12-03 1999-06-10 Ufz-Umweltforschungszentrum Leipzig-Halle Gmbh Device for investigating respiratory tract diseases and diagnostic agents
US5962335A (en) * 1997-01-03 1999-10-05 Oridion Medical Ltd. Breath test for detection of drug metabolism
DE20001995U1 (en) * 2000-02-03 2000-07-13 Filt Forschungsgesellschaft für Lungen- und Thoraxerkrankungen mbH, 13125 Berlin Device for analyzing exhaled air and / or for collecting samples
DE19951204A1 (en) * 1999-10-15 2001-05-10 Filt Forschungsgesellschaft Fu Apparatus to analyze the components in the exhaled air of a patient forms a condensation to be caught by a filter or storage layer to give a sample passed directly to electrochemical sensors for measurement
WO2001034024A1 (en) * 1999-11-08 2001-05-17 University Of Florida Research Foundation, Inc. Marker detection method and apparatus to monitor drug compliance

Patent Citations (14)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
FR2587497A1 (en) * 1985-09-17 1987-03-20 Marelli Autronica ACCELERATION OR VIBRATION SENSOR
EP0269709B1 (en) * 1986-06-14 1992-01-29 LION LABORATORIES plc Alcohol or drugs breath detecting devices
DE9421065U1 (en) * 1994-05-13 1995-05-11 Filt Forschungsgesellschaft für Lungen- und Thoraxerkrankungen mbH, 13125 Berlin Device for collecting exhaled breath condensate
DE19607646A1 (en) * 1996-02-29 1997-09-11 Joerg Volkmann Detection of consumption of hashish or marijuana
US5962335A (en) * 1997-01-03 1999-10-05 Oridion Medical Ltd. Breath test for detection of drug metabolism
US6180414B1 (en) * 1997-01-03 2001-01-30 Oridion Medical Ltd. Breath test for detection of drug metabolism
DE19718925A1 (en) * 1997-04-28 1998-10-29 Medium Sensor Gmbh Recovery of component fractions from exhaled air
DE29712836U1 (en) * 1997-07-10 1997-09-18 Filt Forschungsgesellschaft für Lungen- und Thoraxerkrankungen mbH, 13125 Berlin Condensate trap to collect exhaled breath condensate
WO1999028743A1 (en) * 1997-12-03 1999-06-10 Ufz-Umweltforschungszentrum Leipzig-Halle Gmbh Device for investigating respiratory tract diseases and diagnostic agents
DE19755471A1 (en) * 1997-12-03 1999-06-17 Ufz Leipzighalle Gmbh Device for examining respiratory diseases and diagnostic means
DE29803485U1 (en) * 1998-03-04 1998-05-14 Bionorica Arzneimittel GmbH, 92318 Neumarkt Device for determining at least one substance contained in the exhaled air of a living being
DE19951204A1 (en) * 1999-10-15 2001-05-10 Filt Forschungsgesellschaft Fu Apparatus to analyze the components in the exhaled air of a patient forms a condensation to be caught by a filter or storage layer to give a sample passed directly to electrochemical sensors for measurement
WO2001034024A1 (en) * 1999-11-08 2001-05-17 University Of Florida Research Foundation, Inc. Marker detection method and apparatus to monitor drug compliance
DE20001995U1 (en) * 2000-02-03 2000-07-13 Filt Forschungsgesellschaft für Lungen- und Thoraxerkrankungen mbH, 13125 Berlin Device for analyzing exhaled air and / or for collecting samples

Cited By (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE102005020102B3 (en) * 2005-04-25 2006-11-30 Universität Potsdam Method and device for obtaining and analyzing respiratory condensates
US10052045B2 (en) 2012-12-21 2018-08-21 Colgate-Palmolive Company Method for testing oral malodor

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