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CN1366952A - Nano Fengshi Guanjie preparation medicine and preparation method - Google Patents

Nano Fengshi Guanjie preparation medicine and preparation method Download PDF

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Publication number
CN1366952A
CN1366952A CN 01102148 CN01102148A CN1366952A CN 1366952 A CN1366952 A CN 1366952A CN 01102148 CN01102148 CN 01102148 CN 01102148 A CN01102148 A CN 01102148A CN 1366952 A CN1366952 A CN 1366952A
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nanometer
parts
nano
part nanometer
radix
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杨孟君
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Abstract

The present invention discloses a nano Fengshi Guanjie preparation medicine. It is made up by using 23 Chinese medicinal materials of nano black-striped snake, nano wild aconite, nano cranesbill, nano Japanese dioscorea, nano notopterygium as raw material through the processes of microwave extraction, reduced pressure concentration and supersonic jet spray drying. Its grain fineness is up to 1200-1500 meshes, grain size is 0.1-200 nm, in which most of grain size is less than 100 nm.

Description

Nano Fengshi Guanjie preparation medicine and preparation method thereof
The present invention relates to the nano Fengshi Guanjie preparation medicine of a kind of wind dispelling cold expelling, promoting blood circulation and stopping pain, the invention still further relates to the method for this medication preparation.
Fengshi Guanjie wine is a kind of classical Chinese patent medicine, mainly contains effects such as wind dispelling cold expelling, promoting blood circulation and stopping pain, is used for wind-cold damp pathogen and causes: arthralgia, shoulder back of the body acid precipitation, lumbago rheumatism in the legs, numb limbs and tense tendons, the contracture of muscle arteries and veins.But traditional Fengshi Guanjie wine absorbs not exclusively, and bioavailability is not high, slow curative effect.
The object of the present invention is to provide a kind of bioavailability height, solid dispersion is good, absorbs fully the nano Fengshi Guanjie preparation medicine of increase evident in efficacy.
Another object of the present invention provides the preparation method of this nano Fengshi Guanjie preparation medicine.
To achieve these goals, the present invention takes following technical scheme:
Medicine of the present invention is to make (consumption is a weight portion) by following component:
Nanometer Zaocys 100-200 part nanometer Radix Aconiti Kusnezoffii 60-150 part nanometer Herba Erodii 150-400 part
Nanometer Rhizoma Dioscoreae Nipponicae 150-400 part nanometer Rhizoma Et Radix Notopterygii 60-150 part nanometer Radix Angelicae Pubescentis 60-150 part
Nanometer Radix Clematidis 40-95 part nanometer Cortex Periplocae 150-400 part nanometer Fructus Chaenomelis 40-90 part
Nanometer Rhizoma Atractylodis 100-200 part nanometer Radix Saposhnikoviae 80-180 part nanometer Pine Nodular Branch 100-200 part
Nano Chinese angelica 100-200 part nanometer Rhizoma Chuanxiong 100-200 part nanometer Ramulus Cinnamomi 60-150 part
Nanometer Caulis Spatholobi 80-180 part nanometer Radix Achyranthis Bidentatae 60-150 part nanometer Radix Paeoniae Alba 100-250 part
Nanometric Hypoglaucous Collett Yam Rhizome 100-250 part nanometer Fructus Citri Sarcodactylis 100-250 part nano ginseng 80-180 part
Nanometer Radix Glycyrrhizae 80-180 part nanometer Monas cuspurpureus Went 150-400 part
The formula optimization weight proportion scope of medicine of the present invention is:
Nanometer Zaocys 120-180 part nanometer Radix Aconiti Kusnezoffii 80-120 part nanometer Herba Erodii 200-300 part
Nanometer Rhizoma Dioscoreae Nipponicae 200-300 part nanometer Rhizoma Et Radix Notopterygii 80-120 part nanometer Radix Angelicae Pubescentis 80-120 part
Nanometer Radix Clematidis 50-90 part nanometer Cortex Periplocae 200-300 part nanometer Fructus Chaenomelis 50-80 part
Nanometer Rhizoma Atractylodis 120-180 part nanometer Radix Saposhnikoviae 100-150 part nanometer Pine Nodular Branch 120-180 part
Nano Chinese angelica 120-180 part nanometer Rhizoma Chuanxiong 120-180 part nanometer Ramulus Cinnamomi 80-120 part
Nanometer Caulis Spatholobi 100-150 part nanometer Radix Achyranthis Bidentatae 80-120 part nanometer Radix Paeoniae Alba 120-180 part
Nanometric Hypoglaucous Collett Yam Rhizome 120-180 part nanometer Fructus Citri Sarcodactylis 120-180 part nano ginseng 100-150 part
Nanometer Radix Glycyrrhizae 100-150 part nanometer Monas cuspurpureus Went 200-300 part
The optimum weight proportioning of medicine of the present invention is:
250 parts of 93.75 parts of nanometer Herba Erodiis of 156.25 parts of nanometer Radix Aconiti Kusnezoffii of nanometer Zaocys
93.75 parts of 93.75 parts of nanometer Radix Angelicae Pubescentiss of 250 parts of nanometer Rhizoma Et Radix Notopterygiis of nanometer Rhizoma Dioscoreae Nipponicae
62.5 parts of 250 parts of nanometer Fructus Chaenomeliss of 62.5 parts of nanometer Cortex Periplocaes of nanometer Radix Clematidis
156.25 parts of 125 parts of nanometer Pine Nodular Branchs of 156.25 parts of nanometer Radix Saposhnikoviaes of nanometer Rhizoma Atractylodis
93.75 parts of 156.25 parts of nanometer Ramulus Cinnamomi of 156.25 parts of nanometer Rhizoma Chuanxiongs of nano Chinese angelica
156.25 parts of 93.75 parts of nanometer Radix Paeoniae Albas of 125 parts of nanometer Radix Achyranthis Bidentataes of nanometer Caulis Spatholobi
125 parts of 156.25 parts of nano ginsengs of 156.25 parts of nanometer Fructus Citri Sarcodactylis of nanometric Hypoglaucous Collett Yam Rhizome
250 parts in 125 parts of nanometer Monas cuspurpureus Went of nanometer Radix Glycyrrhizae
Technical scheme of the present invention is based on the modern material technology.One of modern material Developing Trend in Technology is to develop to the more and more littler direction of yardstick.The granule of the past composition material, its size all are at micron or more than the millimeter magnitude, and have occurred the material to the nanoscale development now.Because extremely refinement of granule, the shared percentage by volume of crystal boundary increases, and makes some performance of material that outstanding variation take place.
The property of nano material be since special construction----the material grains size of nano material less than the ultra-micro powder of 100nm, its body surface area is very big, the atom number ratio at crystal boundary place makes it to produce four big effects up to 15--50%: i.e. small-size effect, quantum effect (containing macro quanta tunnel effect), skin effect and interfacial effect.Thereby has the not available physical and chemical performance of traditional material.Nanotechnology will bring a technological revolution of the field of Chinese medicines.
One of method of above-mentioned each component being made medicine of the present invention is:
1. divide and get the Chinese crude drug of respectively distinguishing the flavor of, be processed into the common Chinese decoction pieces according to process of preparing Chinese medicine of Chinese Pharmacopoeia version in 2000.
2. divide and get the common Chinese decoction pieces of respectively distinguishing the flavor of, be processed into the nanometer prepared slices of Chinese crude drugs, its method comprises the following steps:
1. the common Chinese decoction pieces is placed extraction pot, solubilizer also imports microwave extracting, makes its speed with 20--30 hundred million times/second do the change in polarity motion, and the temperature of its microwave extracting is 30 ℃--and 60 ℃, time 1-10 hour;
2. above-mentioned extract is carried out concentrating under reduced pressure, temperature is 30 ℃--60 ℃, the time is 3-72 hour, collects volatile material in the Chinese medicine simultaneously in addition;
3. decompressed concentrate and volatile material merging are placed spray drying tower, use the supersonic jet technology, 330 meters of effluxvelocities--990 meter per seconds, at 30 ℃--60 ℃ of temperature, under 0 to the 0.05MPa pressure,, promptly make the nanometer prepared slices of Chinese crude drugs with hypersonic velocity instantaneous jet drying.
3. the nanometer prepared slices of Chinese crude drugs (powder) are prepared mixing in described ratio, according to Chinese Pharmacopoeia version two-shift system in 2000 agent standard, make pill, powder, tablet, suppository, granule, membrane, capsule, microcapsule, drop pill, aerosol, injection, unguentum, medicated wine, syrup, oral solution.
Two of medicine method for making of the present invention is:
1. be equipped with whole common Chinese decoction pieces in the proportioning ratio, place extraction pot, solubilizer also imports microwave extracting, makes its speed with 20--30 hundred million times/second do the change in polarity motion, and the temperature of its little liquid extraction is 30 ℃-60 ℃, time 1-10 hour:
2. above-mentioned extract is carried out concentrating under reduced pressure, temperature is 30 ℃--60 ℃, the time is 3-72 hour, collects volatile material in the Chinese medicine simultaneously in addition;
3. decompressed concentrate and volatile material merging are placed spray drying tower, use the supersonic jet technology, 330 meters of effluxvelocities--990 meter per seconds, at 30 ℃--60 ℃ of temperature, under 0 to the 0.05MPa pressure,, get Fengshi Guanjie preparation nano powder with hypersonic velocity instantaneous jet drying;
4. its nano powder is made aforementioned various preparation according to Chinese Pharmacopoeia version standard preparation in 2000.
The pharmacological effect that above-mentioned two kinds of methods are made the nano Fengshi Guanjie preparation medicine is identical.
A kind of important feature of the present invention is: the made drug material of the present invention has reached nanoscale, common Fengshi Guanjie liquor preparation material is micron or the above particle diameter of millimeter, can only cross the 80-120 mesh sieve, the drug material that the present invention is made, particle diameter is at 0.1--200nm, the overwhelming majority can be crossed the 1200--1500 mesh sieve less than 100nm.
Another important feature of the present invention is: solid preparation of the present invention disintegrate rapidly, and solid dispersion is good in water, absorb fully, the bioavailability height, the pharmacological action effect that mainly contains effective constituent is significantly higher than conventional formulation.
The pharmaceutical preparation that the present invention is made does not need to add any adjuvant, and is more favourable to human body.
The present invention has also created the novel form that pill, powder, tablet, suppository, granule, membrane, capsule, microcapsule, drop pill, aerosol, injection, unguentum, syrup, oral solution of nano Fengshi Guanjie preparation medicine etc. had no precedent in the past.
Pharmaceutical preparation of the present invention can be used for wind-cold damp pathogen and causes: treatment of conditions such as arthralgia, shoulder back of the body acid precipitation, lumbago rheumatism in the legs, numb limbs and tense tendons, the contracture of muscle arteries and veins, clinical efficacy significantly is better than traditional Fengshi Guanjie wine.
The present invention's added solvent in microwave extracting is water or ethanol.
The present invention carries out in the concentrating under reduced pressure step at extract, and its concentrating under reduced pressure is conventional scheme.
Embodiment 1:
Prepare nano raw material by preceding method:
250 parts of 93.75 parts of nanometer Herba Erodiis of 156.25 parts of nanometer Radix Aconiti Kusnezoffii of nanometer Zaocys
93.75 parts of 93.75 parts of nanometer Radix Angelicae Pubescentiss of 250 parts of nanometer Rhizoma Et Radix Notopterygiis of nanometer Rhizoma Dioscoreae Nipponicae
62.5 parts of 250 parts of nanometer Fructus Chaenomeliss of 62.5 parts of nanometer Cortex Periplocaes of nanometer Radix Clematidis
156.25 parts of 125 parts of nanometer Pine Nodular Branchs of 156.25 parts of nanometer Radix Saposhnikoviaes of nanometer Rhizoma Atractylodis
93.75 parts of 156.25 parts of nanometer Ramulus Cinnamomi of 156.25 parts of nanometer Rhizoma Chuanxiongs of nano Chinese angelica
156.25 parts of 93.75 parts of nanometer Radix Paeoniae Albas of 125 parts of nanometer Radix Achyranthis Bidentataes of nanometer Caulis Spatholobi
125 parts of 156.25 parts of nano ginsengs of 156.25 parts of nanometer Fructus Citri Sarcodactylis of nanometric Hypoglaucous Collett Yam Rhizome
250 parts in 125 parts of nanometer Monas cuspurpureus Went of nanometer Radix Glycyrrhizae
Production method is as follows:
In the GMP cleaning shop, after the above-mentioned nanometer prepared slices of Chinese crude drugs or powder prepared mixing in described ratio, according to Chinese Pharmacopoeia version two-shift system in 2000 agent capsules agent standard, do not add adjuvant, do not granulate, directly divide encapsulated with the fully-automatic capsule racking machine, make capsule, every capsules content of dispersion is the 0.1--0.6 gram, and the patient takes the 1-5 grain at every turn, and take 1-4 every day.
Embodiment 2:
Prepare nano raw material by preceding method:
250 parts of 93.75 parts of nanometer Herba Erodiis of 156.25 parts of nanometer Radix Aconiti Kusnezoffii of nanometer Zaocys
93.75 parts of 93.75 parts of nanometer Radix Angelicae Pubescentiss of 250 parts of nanometer Rhizoma Et Radix Notopterygiis of nanometer Rhizoma Dioscoreae Nipponicae
62.5 parts of 250 parts of nanometer Fructus Chaenomeliss of 62.5 parts of nanometer Cortex Periplocaes of nanometer Radix Clematidis
156.25 parts of 125 parts of nanometer Pine Nodular Branchs of 156.25 parts of nanometer Radix Saposhnikoviaes of nanometer Rhizoma Atractylodis
93.75 parts of 156.25 parts of nanometer Ramulus Cinnamomi of 156.25 parts of nanometer Rhizoma Chuanxiongs of nano Chinese angelica
156.25 parts of 93.75 parts of nanometer Radix Paeoniae Albas of 125 parts of nanometer Radix Achyranthis Bidentataes of nanometer Caulis Spatholobi
125 parts of 156.25 parts of nano ginsengs of 156.25 parts of nanometer Fructus Citri Sarcodactylis of nanometric Hypoglaucous Collett Yam Rhizome
250 parts in 125 parts of nanometer Monas cuspurpureus Went of nanometer Radix Glycyrrhizae
Production method is as follows:
In the GMP cleaning shop, with the above-mentioned nanometer prepared slices of Chinese crude drugs or powder by described mixed good after, according to 2000 editions two-shift system agent of Chinese Pharmacopoeia membrane standard, filmogen adopts polyvinyl alcohol, make the nano Fengshi Guanjie membrane, every membrane area size is the 2-100 square centimeter, and content of dispersion is the 1-50 gram, every medicine film pasted 1-7 days, pasted the medicine position: the affected part.

Claims (6)

1, a kind of nano Fengshi Guanjie preparation medicine is characterized in that it is the medicament that the nano raw material of following weight proportioning is made:
Nanometer Zaocys 100-200 part nanometer Radix Aconiti Kusnezoffii 60-150 part nanometer Herba Erodii 150-400 part
Nanometer Rhizoma Dioscoreae Nipponicae 150-400 part nanometer Rhizoma Et Radix Notopterygii 60-150 part nanometer Radix Angelicae Pubescentis 60-150 part
Nanometer Radix Clematidis 40-95 part nanometer Cortex Periplocae 150-400 part nanometer Fructus Chaenomelis 40-90 part
Nanometer Rhizoma Atractylodis 100-200 part nanometer Radix Saposhnikoviae 80-180 part nanometer Pine Nodular Branch 100-200 part
Nano Chinese angelica 100-200 part nanometer Rhizoma Chuanxiong 100-200 part nanometer Ramulus Cinnamomi 60-150 part
Nanometer Caulis Spatholobi 80-180 part nanometer Radix Achyranthis Bidentatae 60-150 part nanometer Radix Paeoniae Alba 100-250 part
Nanometric Hypoglaucous Collett Yam Rhizome 100-250 part nanometer Fructus Citri Sarcodactylis 100-250 part nano ginseng 80-180 part
Nanometer Radix Glycyrrhizae 80-180 part nanometer Monas cuspurpureus Went 150-400 part
And adopt following method to make: to select the formula Chinese drug material to concoct and be processed into the prepared slices of Chinese crude drugs; Place extraction pot, solubilizer also imports microwave extracting, makes it do the change in polarity motion with hundred million times/second speed of 20--30, and the temperature of its microwave extracting is 30--60 ℃, time 1-10 hour; Above-mentioned extract is carried out concentrating under reduced pressure, and temperature is 30--60 ℃, and the time is 3-72 hour, collects volatile material in the Chinese medicine simultaneously in addition; Decompressed concentrate and volatile material merging are placed spray drying tower, use the supersonic jet technology, 30--60 ℃ of temperature, under 0 to the 0.05MPa pressure, with hypersonic velocity instantaneous jet drying, wherein supersonic jet speed is 330 meters-990 meter per seconds, promptly makes the nanometer prepared slices of Chinese crude drugs.
2, nano Fengshi Guanjie preparation medicine according to claim 1, wherein the weight proportion of each nano raw material is:
Nanometer Zaocys 120-180 part nanometer Radix Aconiti Kusnezoffii 80-120 part nanometer Herba Erodii 200-300 part
Nanometer Rhizoma Dioscoreae Nipponicae 200-300 part nanometer Rhizoma Et Radix Notopterygii 80-120 part nanometer Radix Angelicae Pubescentis 80-120 part
Nanometer Radix Clematidis 50-90 part nanometer Cortex Periplocae 200-300 part nanometer Fructus Chaenomelis 50-80 part
Nanometer Rhizoma Atractylodis 120-180 part nanometer Radix Saposhnikoviae 100-150 part nanometer Pine Nodular Branch 120-180 part
Nano Chinese angelica 120-180 part nanometer Rhizoma Chuanxiong 120-180 part nanometer Ramulus Cinnamomi 80-120 part
Nanometer Caulis Spatholobi 100-150 part nanometer Radix Achyranthis Bidentatae 80-120 part nanometer Radix Paeoniae Alba 120-180 part
Nanometric Hypoglaucous Collett Yam Rhizome 120-180 part nanometer Fructus Citri Sarcodactylis 120-180 part nano ginseng 100-150 part
Nanometer Radix Glycyrrhizae 100-150 part nanometer Monas cuspurpureus Went 200-300 part
3, nano Fengshi Guanjie preparation medicine according to claim 1, wherein the weight proportion of each nano raw material is:
250 parts of 93.75 parts of nanometer Herba Erodiis of 156.25 parts of nanometer Radix Aconiti Kusnezoffii of nanometer Zaocys
93.75 parts of 93.75 parts of nanometer Radix Angelicae Pubescentiss of 250 parts of nanometer Rhizoma Et Radix Notopterygiis of nanometer Rhizoma Dioscoreae Nipponicae
62.5 parts of 250 parts of nanometer Fructus Chaenomeliss of 62.5 parts of nanometer Cortex Periplocaes of nanometer Radix Clematidis
156.25 parts of 125 parts of nanometer Pine Nodular Branchs of 156.25 parts of nanometer Radix Saposhnikoviaes of nanometer Rhizoma Atractylodis
93.75 parts of 156.25 parts of nanometer Ramulus Cinnamomi of 156.25 parts of nanometer Rhizoma Chuanxiongs of nano Chinese angelica
156.25 parts of 93.75 parts of nanometer Radix Paeoniae Albas of 125 parts of nanometer Radix Achyranthis Bidentataes of nanometer Caulis Spatholobi
125 parts of 156.25 parts of nano ginsengs of 156.25 parts of nanometer Fructus Citri Sarcodactylis of nanometric Hypoglaucous Collett Yam Rhizome
250 parts in 125 parts of nanometer Monas cuspurpureus Went of nanometer Radix Glycyrrhizae
4,, it is characterized in that said medicine is pill, powder, tablet, suppository, granule, membrane, capsule, microcapsule, drop pill, aerosol, injection, unguentum, medicated wine, syrup, oral solution according to claim 1 or 2 or 3 described nano Fengshi Guanjie preparation medicines.
5,, it is characterized in that this method comprises the steps: to select the formula Chinese drug material to concoct and is processed into the prepared slices of Chinese crude drugs according to the pharmaceutical methods of claim 1 or 2 or 3 described nano Fengshi Guanjie preparation medicines; Place extraction pot, solubilizer also imports microwave extracting, makes it do the change in polarity motion with hundred million times/second speed of 20--30, and the temperature of its microwave extracting is 30--60 ℃, time 1-10 hour; Above-mentioned extract is carried out concentrating under reduced pressure, and temperature is 30--60 ℃, and the time is 3-72 hour, collects volatile material in the Chinese medicine simultaneously in addition; Decompressed concentrate and volatile material merging are placed spray drying tower, use the supersonic jet technology, 30--60 ℃ of temperature, under 0 to the 0.05MPa pressure, with hypersonic velocity instantaneous jet drying, wherein supersonic jet speed is 330 meters-990 meter per seconds, promptly makes the nanometer prepared slices of Chinese crude drugs.
6, wherein respectively distinguish the flavor of Chinese medicine in the ratio of prescription or Chinese crude drug concoct be processed into the prepared slices of Chinese crude drugs after mixing, or after making the nanometer prepared slices of Chinese crude drugs mixing.
CN 01102148 2001-01-20 2001-01-20 Nano Fengshi Guanjie preparation medicine and preparation method Pending CN1366952A (en)

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Application Number Priority Date Filing Date Title
CN 01102148 CN1366952A (en) 2001-01-20 2001-01-20 Nano Fengshi Guanjie preparation medicine and preparation method

Publications (1)

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CN1366952A true CN1366952A (en) 2002-09-04

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Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN1322877C (en) * 2003-09-16 2007-06-27 郁华堂 Caspule for treating fibrositis

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
CN1322877C (en) * 2003-09-16 2007-06-27 郁华堂 Caspule for treating fibrositis

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