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CH106401A - Process for the production of a new intermediate product in the tar color industry. - Google Patents

Process for the production of a new intermediate product in the tar color industry.

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Publication number
CH106401A
CH106401A CH106401DA CH106401A CH 106401 A CH106401 A CH 106401A CH 106401D A CH106401D A CH 106401DA CH 106401 A CH106401 A CH 106401A
Authority
CH
Switzerland
Prior art keywords
sep
phenylenediamine
production
hol
intermediate product
Prior art date
Application number
Other languages
German (de)
Inventor
Gesellschaft Fuer Chemis Basel
Original Assignee
Chem Ind Basel
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Chem Ind Basel filed Critical Chem Ind Basel
Publication of CH106401A publication Critical patent/CH106401A/en

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Description

  

      Verfahren    zur Herstellung eines neuen Zwischenproduktes der Teerfarbenindustrie.    Es wurde gefunden, dass man ein neues  Zwischenprodukt, das symmetrische     ditertiäre     Kondensationsprodukt von zwei     Mol.        Cyanur-          ehlorid,    einem     Mol.        1,4-Phenylendiamin,    zwei       Mol.        1,3-Phenylendiamin    - 4 -     sulfosäure    und  zwei     Mol.        1,3-Phenylendi,amin,    erhält,

   wenn  man auf zwei     Mol.        Cyanurchlorid    in     beliebi-          ger    Reihenfolge ein     AIo1.        1,4-Phenylendi-amin,     zwei     Mol.        1,3-Phenylendia.min    - 4 -     sulfosäure     und zwei     Mod.        Monoformyl-1,3-Phenylendia-          min    einwirken     lässt,    und das so erhaltene Pro  dukt verseift.  



  Diese Kondensation wird durch Zusam  menrühren der Komponenten in einem geeig  neten Verdünnungsmittel durchgeführt, und  es wurde gefunden, dass Wasser als solches in  Überraschender Weise sehr gut     geeignet    ist.  Das symmetrische     ditertiäre    Kondensations  produkt aus zwei     Mol.        Cyanurchlorid    mit  einem     Mol.        1,4-Phenylendi.amin,    zwei     Mol.          1,3-Phenylendiamin    - 4 -     sulfosäure    und zwei       112o1.        1,3-Phenylendiamin    bildet als     Alkalisalz     ein in Wasser lösliches,

   fast farbloses Pulver.  Es enthält 4     diazotierbare        Aminogruppen,       kein reaktionsfähiges Chloratom mehr und  stellt ein wertvolles Ausgangsmaterial zur  Herstellung von Farbstoffen dar.  



  <I>Beispiel:</I>  In eine     Aussehlemmung    von 37 Teilen       Cyanurchlorid    und<B>1000</B> Teilen Wasser giesst.  man eine Lösung aus 37,8 Teilen     1,3-Phenyl-          endiamin-4-sulfosäure    und 10.8 Teilen Soda  in 1000 Teilen Wasser.

   Die Temperatur     -wird     bei 0  gehalten und die gebildete Mineralsäure       neutralisiert.    Sobald die Komponenten ver  schwunden sind, fügt man 10,8 Teile 1,4  Phenylendiamin hinzu und rührt mehrere  Stunden auf 40 bis<B>50'.</B> Hierauf neutralisiert  man genau, fügt 27,2 Teile     2lonoformyl-1.3-          Phenylendiamin    hinzu und kocht einige Zeit  am     RückfluZkühler.    Wenn das     Monoformyl-          1,3-Phenylendiamin    verschwunden ist, wer  den 20 Teile     Natronhydrat    zugegeben und  noch eine     Viertelstunde    gekocht.

   Nach dem  Erkalten wird das     symmetrische        ditertiäre     Kondensationsprodukt aus zwei     Mol.        Cyanur-          ,ehlorid,    einem     Mol.        1,4-Phenylendia.min,    zwei    
EMI0002.0001     
  
    Hol. <SEP> 1,3-Phenylendiamin <SEP> - <SEP> $ <SEP> - <SEP> sulfos*i.ure <SEP> und
<tb>  zwei <SEP> Mol. <SEP> 1,3-Phenylendiamin <SEP> durch <SEP> Aus  salzen <SEP> und <SEP> Aussäuern <SEP> isoliert.



      Process for the production of a new intermediate product in the tar color industry. It has been found that a new intermediate product, the symmetrical ditertiary condensation product of two moles of cyanuric chloride, one mole of 1,4-phenylenediamine, two moles of 1,3-phenylenediamine-4-sulfonic acid and two moles of 1,3 -Phenylenedi, amine, receives,

   if you add an Alo1 to two moles of cyanuric chloride in any order. 1,4-phenylenediamine, two moles. 1,3-phenylenediamine-4-sulfonic acid and two mod. Monoformyl-1,3-phenylenediamine are allowed to act, and the product thus obtained is saponified.



  This condensation is carried out by stirring the components together in a suitable diluent, and it has been found that water as such is surprisingly very suitable. The symmetrical ditertiary condensation product of two moles of cyanuric chloride with one mole of 1,4-phenylenediamine, two moles of 1,3-phenylenediamine-4-sulfonic acid and two 112o1. As an alkali salt, 1,3-phenylenediamine forms a water-soluble,

   almost colorless powder. It contains 4 diazotizable amino groups, no more reactive chlorine atom and is a valuable starting material for the production of dyes.



  <I> Example: </I> Pour 37 parts of cyanuric chloride and <B> 1000 </B> parts of water into a lockout. a solution of 37.8 parts of 1,3-phenylenediamine-4-sulfonic acid and 10.8 parts of soda in 1000 parts of water.

   The temperature is kept at 0 and the mineral acid formed is neutralized. As soon as the components have disappeared, 10.8 parts of 1.4 phenylenediamine are added and the mixture is stirred for several hours at 40 to 50 '. This is followed by precise neutralization, 27.2 parts of 2lonoformyl-1,3-phenylenediamine are added and boil for some time on the reflux condenser. When the monoformyl-1,3-phenylenediamine has disappeared, who added 20 parts of sodium hydrate and cooked for a quarter of an hour.

   After cooling, the symmetrical ditertiary condensation product of two moles of cyanuric chloride, one mole of 1,4-phenylenediamine, two
EMI0002.0001
  
    Hol. <SEP> 1,3-phenylenediamine <SEP> - <SEP> $ <SEP> - <SEP> sulfos * i.ure <SEP> and
<tb> two <SEP> moles <SEP> 1,3-phenylenediamine <SEP> isolated by <SEP> from salts <SEP> and <SEP> acidifying <SEP>.

 

Claims (1)

PATENTANSPRUCH EMI0002.0003 Verfahren <SEP> zur <SEP> Herstellung <SEP> eines <SEP> neuen <tb> Zwischenproduktes, <SEP> des <SEP> symmetrischen <SEP> diter tiären <SEP> Kondensationsproduktes <SEP> von <SEP> zwei <SEP> Mol. <tb> Cyanurchlorid, <SEP> einem <SEP> Hol. <SEP> 1; PATENT CLAIM EMI0002.0003 Procedure <SEP> for <SEP> production <SEP> of a <SEP> new one <tb> intermediate product, <SEP> of the <SEP> symmetrical <SEP> diter tiary <SEP> condensation product <SEP> of <SEP> two <SEP> mol. <tb> cyanuric chloride, <SEP> a <SEP> hol. <SEP> 1; 1-Phenylendia min, <SEP> zwei <SEP> Hol. <SEP> 1,3-Phenylendiasnin-4-sulfo säure <SEP> und <SEP> zwei <SEP> 1VIol. <SEP> 1,3-Phenylendiamin, <SEP> da durch <SEP> gekennzeiehnet, <SEP> dass <SEP> man <SEP> in <SEP> beliebiger <tb> Reihenfolge <SEP> auf <SEP> Cyanurchlorid <SEP> ein <SEP> 111o1. <SEP> 1,4 Phenylendiamin, <SEP> zwei <SEP> Hol. <SEP> 1,3-Phenylendia min-4-sulfosäure <SEP> und <SEP> zwei <SEP> Mo1. <SEP> Monoformyl- EMI0002.0004 1,3-Phenylendiamin <SEP> einwirken <SEP> lässt <SEP> und <SEP> das <tb> so <SEP> erhaltene <SEP> Produkt <SEP> verseift. <tb> Das <SEP> symmetris.ehe <SEP> ditertiäre <SEP> Kondensa tionsprodukt <SEP> aus <SEP> zwei <SEP> Mol. <SEP> Cyanurchloritl <SEP> mit <tb> einem <SEP> 112o1. 1-phenylenediamine, <SEP> two <SEP> Hol. <SEP> 1,3-phenylenediasnin-4-sulfo acid <SEP> and <SEP> two <SEP> 1Viol. <SEP> 1,3-phenylenediamine, <SEP> as marked by <SEP>, <SEP> that <SEP> one <SEP> in <SEP> any <tb> sequence <SEP> on <SEP> cyanuric chloride <SEP> on <SEP> 111o1. <SEP> 1,4 phenylenediamine, <SEP> two <SEP> Hol. <SEP> 1,3-phenylenediamine-4-sulfonic acid <SEP> and <SEP> two <SEP> Mo1. <SEP> monoformyl EMI0002.0004 1,3-Phenylenediamine <SEP> take effect <SEP> allows <SEP> and <SEP> that <tb> so <SEP> received <SEP> product <SEP> saponified. <tb> The <SEP> symmetric <SEP> ditertiary <SEP> condensation product <SEP> from <SEP> two <SEP> mol. <SEP> cyanuric chlorite <SEP> with <tb> a <SEP> 112o1. <SEP> 1,4-Phenylendiamin, <SEP> zwei <SEP> Hol. <tb> 1,3-Phenylendiamin <SEP> - <SEP> 4 <SEP> - <SEP> sulfosäure <SEP> und <SEP> zwei <tb> llTol. <SEP> 1,3-Phenylendia,min <SEP> bildet <SEP> als <SEP> Alkalisalz <tb> ein <SEP> in <SEP> Wasser <SEP> lösliches. <SEP> fast <SEP> farbloses <SEP> Pul ver. <SEP> Fs <SEP> enthält <SEP> vier <SEP> diazotierbare <SEP> Amino gruppen, <SEP> kein <SEP> reaktionsfähiges <SEP> Chloratom <tb> mehr <SEP> und <SEP> stellt <SEP> ein <SEP> wertvolles <SEP> Ausgangsma terial <SEP> zur <SEP> Herstellung <SEP> von <SEP> Farbstoffen <SEP> dar. <SEP> 1,4-phenylenediamine, <SEP> two <SEP> Hol. <tb> 1,3-phenylenediamine <SEP> - <SEP> 4 <SEP> - <SEP> sulfonic acid <SEP> and <SEP> two <tb> llTol. <SEP> 1,3-phenylenedia, min <SEP> forms <SEP> as <SEP> alkali salt <tb> a <SEP> soluble in <SEP> water <SEP>. <SEP> almost <SEP> colorless <SEP> powder. <SEP> Fs <SEP> contains <SEP> four <SEP> diazotizable <SEP> amino groups, <SEP> no <SEP> reactive <SEP> chlorine atom <tb> more <SEP> and <SEP> represent <SEP> a <SEP> valuable <SEP> base material <SEP> for <SEP> production <SEP> of <SEP> dyes <SEP>.
CH106401D 1922-09-07 1923-11-28 Process for the production of a new intermediate product in the tar color industry. CH106401A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
CH103430T 1922-09-07
FR106401X 1923-01-03

Publications (1)

Publication Number Publication Date
CH106401A true CH106401A (en) 1924-08-16

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Family Applications (1)

Application Number Title Priority Date Filing Date
CH106401D CH106401A (en) 1922-09-07 1923-11-28 Process for the production of a new intermediate product in the tar color industry.

Country Status (1)

Country Link
CH (1) CH106401A (en)

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2544071A (en) * 1951-03-06 Diethylenetrimelamine and method

Cited By (1)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
US2544071A (en) * 1951-03-06 Diethylenetrimelamine and method

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