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AR116905A1 - PYRROLIDINE-2-CARBOXYL ACID DERIVATIVES TO TREAT PAIN AND PAIN-RELATED CONDITIONS - Google Patents

PYRROLIDINE-2-CARBOXYL ACID DERIVATIVES TO TREAT PAIN AND PAIN-RELATED CONDITIONS

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Publication number
AR116905A1
AR116905A1 ARP190103622A ARP190103622A AR116905A1 AR 116905 A1 AR116905 A1 AR 116905A1 AR P190103622 A ARP190103622 A AR P190103622A AR P190103622 A ARP190103622 A AR P190103622A AR 116905 A1 AR116905 A1 AR 116905A1
Authority
AR
Argentina
Prior art keywords
radical
unbranched
branched
hydrogen atom
independently
Prior art date
Application number
ARP190103622A
Other languages
Spanish (es)
Inventor
Graaf Wouter De
Menno Monnee
- Torrens-Jover Antoni Cornelis-Franciscus
Carmen Almansa-Rosales
Anita Wegert
Original Assignee
Esteve Pharmaceuticals Sa
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Filing date
Publication date
Application filed by Esteve Pharmaceuticals Sa filed Critical Esteve Pharmaceuticals Sa
Publication of AR116905A1 publication Critical patent/AR116905A1/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07DHETEROCYCLIC COMPOUNDS
    • C07D401/00Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom
    • C07D401/02Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings
    • C07D401/12Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, at least one ring being a six-membered ring with only one nitrogen atom containing two hetero rings linked by a chain containing hetero atoms as chain links
    • AHUMAN NECESSITIES
    • A61MEDICAL OR VETERINARY SCIENCE; HYGIENE
    • A61PSPECIFIC THERAPEUTIC ACTIVITY OF CHEMICAL COMPOUNDS OR MEDICINAL PREPARATIONS
    • A61P1/00Drugs for disorders of the alimentary tract or the digestive system
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07DHETEROCYCLIC COMPOUNDS
    • C07D207/00Heterocyclic compounds containing five-membered rings not condensed with other rings, with one nitrogen atom as the only ring hetero atom
    • C07D207/02Heterocyclic compounds containing five-membered rings not condensed with other rings, with one nitrogen atom as the only ring hetero atom with only hydrogen or carbon atoms directly attached to the ring nitrogen atom
    • C07D207/04Heterocyclic compounds containing five-membered rings not condensed with other rings, with one nitrogen atom as the only ring hetero atom with only hydrogen or carbon atoms directly attached to the ring nitrogen atom having no double bonds between ring members or between ring members and non-ring members
    • C07D207/10Heterocyclic compounds containing five-membered rings not condensed with other rings, with one nitrogen atom as the only ring hetero atom with only hydrogen or carbon atoms directly attached to the ring nitrogen atom having no double bonds between ring members or between ring members and non-ring members with hetero atoms or with carbon atoms having three bonds to hetero atoms with at the most one bond to halogen, e.g. ester or nitrile radicals, directly attached to ring carbon atoms
    • C07D207/16Carbon atoms having three bonds to hetero atoms with at the most one bond to halogen, e.g. ester or nitrile radicals
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07DHETEROCYCLIC COMPOUNDS
    • C07D403/00Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, not provided for by group C07D401/00
    • C07D403/02Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, not provided for by group C07D401/00 containing two hetero rings
    • C07D403/04Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, not provided for by group C07D401/00 containing two hetero rings directly linked by a ring-member-to-ring-member bond
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07DHETEROCYCLIC COMPOUNDS
    • C07D403/00Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, not provided for by group C07D401/00
    • C07D403/02Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, not provided for by group C07D401/00 containing two hetero rings
    • C07D403/12Heterocyclic compounds containing two or more hetero rings, having nitrogen atoms as the only ring hetero atoms, not provided for by group C07D401/00 containing two hetero rings linked by a chain containing hetero atoms as chain links

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  • Organic Chemistry (AREA)
  • Chemical & Material Sciences (AREA)
  • Health & Medical Sciences (AREA)
  • Nuclear Medicine, Radiotherapy & Molecular Imaging (AREA)
  • Bioinformatics & Cheminformatics (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Chemical & Material Sciences (AREA)
  • Medicinal Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Pharmacology & Pharmacy (AREA)
  • Life Sciences & Earth Sciences (AREA)
  • Animal Behavior & Ethology (AREA)
  • General Health & Medical Sciences (AREA)
  • Public Health (AREA)
  • Veterinary Medicine (AREA)
  • Pharmaceuticals Containing Other Organic And Inorganic Compounds (AREA)

Abstract

La presente se refiere a compuestos que muestran actividad farmacológica dual respecto a la subunidad a2d de canales de calcio dependientes de voltaje (VGCC), especialmente la subunidad a2d-1 de canales de calcio dependientes de voltaje, y el receptor de opioides m (MOR o mu-opioide). La presente también se refiere al proceso para la preparación de dichos compuestos, así como también a las composiciones que los comprenden y su uso como medicamentos. Reivindicación 1: Un compuesto de fórmula general (1), donde: W¹ es -O-, -NRᵃ o -CH₂-; Rᵃ es un átomo de hidrógeno o un radical alquilo C₁₋₆ ramificado o no ramificado; n y m son independientemente el uno del otro 0 ó 1; R¹, R² y R⁴ son independientemente el uno del otro un átomo de hidrógeno; un radical alquilo C₁₋₆ ramificado o no ramificado; un átomo de halógeno; un radical C(O)H; un radical alcoxi C₁₋₆ ramificado o no ramificado; un radical -NRᵇRᶜ; un radical -CN; un radical hidroxilo; o un radical haloalquilo C₁₋₆; Rᵇ y Rᶜ son independientemente el uno del otro un átomo de hidrógeno o un radical alquilo C₁₋₆ ramificado o no ramificado; R³ se selecciona entre: los compuestos de fórmula (2) y (3); W² es -C(O)-, -CH₂- o un enlace; A es C o N; la línea discontinua representa un doble enlace opcional; R³ᵃ y R³ᵇ son independientemente el uno del otro un átomo de hidrógeno o un radical alquilo C₁₋₆ ramificado o no ramificado; o R³ᵃ y R³ᵇ junto con el nitrógeno puente forman un radical heterocicloalquilo de 4, 5 ó 6 miembros que contiene opcionalmente un heteroátomo adicional seleccionado entre N, O y S sustituido opcionalmente con un radical alquilo C₁₋₆ ramificado o no ramificado o un radical alcoxi C₁₋₆ ramificado o no ramificado; R³ᶜ es un átomo de hidrógeno; un átomo de halógeno; un radical hidroxilo; un radical alquilo C₁₋₆ ramificado o no ramificado; un radical alcoxi C₁₋₆ ramificado o no ramificado; un radical -CN; un radical haloalquilo C₁₋₆; o un radical -NR³ᶜR³ᵈ; R³ᵈ y R³ᵉ son independientemente el uno del otro un átomo de hidrógeno o un radical alquilo C₁₋₆ ramificado o no ramificado; R⁵ es un átomo de hidrógeno o un radical -C(O)R⁵ᵃ; R⁵ᵃ es un átomo de hidrógeno; un radical alquilo C₁₋₆ ramificado o no ramificado; un radical alcoxi C₁₋₆ ramificado o no ramificado; un radical -(CH₂)ʳ-NR⁵ᵇR⁵ᶜ; un radical -OCH(CH₃)OC(O)CH(CH₃)₂; o un radical -NR⁵ᵍ-(CH₂)ₛ-CH(R⁵ᶠ)-NR⁵ᵉR⁵ᵈ; r es 1, 2, 3, 4, 5 ó 6; s es 1, 2, 3, 4, 5 ó 6; R⁵ᵇ, R⁵ᶜ, R⁵ᵈ, R⁵ᵉ, R⁵ᵍ son independientemente unos de otros un átomo de hidrógeno; o un radical alquilo C₁₋₆ ramificado o no ramificado; R⁵ᶠ es un átomo de hidrógeno o un radical -COR⁵ʰ; R⁵ʰ es un radical hidroxilo o un radical alquilo C₁₋₆ ramificado o no ramificado; R⁶ es un radical -C(O)R⁶ᵃ; un anillo heteroarilo de 5 ó 6 miembros sustituido opcionalmente que contiene al menos un heteroátomo seleccionado entre N, O y S; R⁶ᵃ es un radical hidroxilo, un radical alcoxi C₁₋₆ ramificado o no ramificado; un radical -(CH₂)ₜ-NR⁶ᵇR⁶ᶜ; un radical -OCH(CH₃)OC(O)CH(CH₃)₂; o un radical -NR⁶ᵍ-(CH₂)ᵛCH(R⁶ᶠ)-NR⁶ᵉR⁶ᵈ; t es 1, 2, 3, 4, 5 ó 6; v es 1, 2, 3, 4, 5 ó 6; R⁶ᵇ, R⁶ᶜ, R⁶ᵈ, R⁶ᵉ, R⁶ᵍ son independientemente unos de otros un átomo de hidrógeno; o un radical alquilo C₁₋₆ ramificado o no ramificado; R⁶ᶠ es un átomo de hidrógeno o un radical -COR⁶ʰ; R⁶ʰ es un radical hidroxilo o un radical alquilo C₁₋₆ ramificado o no ramificado; o una sal, isómero, profármaco o solvato farmacéuticamente aceptable de estos.This refers to compounds that show dual pharmacological activity with respect to the a2d voltage-gated calcium channel (VGCC) subunit, especially the a2d-1 voltage-gated calcium channel subunit, and the m-opioid receptor (MOR or mu-opioid). The present also refers to the process for the preparation of said compounds, as well as to the compositions comprising them and their use as medicaments. Claim 1: A compound of general formula (1), where: W¹ is -O-, -NRᵃ or -CH₂-; Rᵃ is a hydrogen atom or a branched or unbranched C₁₋₆ alkyl radical; n and m are independently of each other 0 or 1; R¹, R² and R⁴ are independently of each other a hydrogen atom; a branched or unbranched C₁₋₆ alkyl radical; a halogen atom; a C (O) H radical; a branched or unbranched C₁₋₆ alkoxy radical; a radical -NRᵇRᶜ; a -CN radical; a hydroxyl radical; or a C₁₋₆ haloalkyl radical; Rᵇ and Rᶜ are independently of each other a hydrogen atom or a branched or unbranched C₁₋₆ alkyl radical; R³ is selected from: the compounds of formula (2) and (3); W² is -C (O) -, -CH₂- or a bond; A is C or N; the dashed line represents an optional double bond; R³ᵃ and R³ᵇ are independently of each other a hydrogen atom or a branched or unbranched C₁₋₆ alkyl radical; or R³ᵃ and R³ᵇ together with the bridging nitrogen form a 4-, 5- or 6-membered heterocycloalkyl radical optionally containing an additional heteroatom selected from N, O and S optionally substituted with a branched or unbranched C₁₋₆ alkyl radical or an alkoxy radical C₁₋₆ branched or unbranched; R³ᶜ is a hydrogen atom; a halogen atom; a hydroxyl radical; a branched or unbranched C₁₋₆ alkyl radical; a branched or unbranched C₁₋₆ alkoxy radical; a -CN radical; a C₁₋₆ haloalkyl radical; or a radical -NR³ᶜR³ᵈ; R³ᵈ and R³ᵉ are independently of each other a hydrogen atom or a branched or unbranched C₁₋₆ alkyl radical; R⁵ is a hydrogen atom or a radical -C (O) R⁵ᵃ; R⁵ᵃ is a hydrogen atom; a branched or unbranched C₁₋₆ alkyl radical; a branched or unbranched C₁₋₆ alkoxy radical; a radical - (CH₂) ʳ-NR⁵ᵇR⁵ᶜ; a radical -OCH (CH₃) OC (O) CH (CH₃) ₂; or a radical -NR⁵ᵍ- (CH₂) ₛ-CH (R⁵ᶠ) -NR⁵ᵉR⁵ᵈ; r is 1, 2, 3, 4, 5, or 6; s is 1, 2, 3, 4, 5, or 6; R⁵ᵇ, R⁵ᶜ, R⁵ᵈ, R⁵ᵉ, R⁵ᵍ are independently of one another a hydrogen atom; or a branched or unbranched C₁₋₆ alkyl radical; R⁵ᶠ is a hydrogen atom or a radical -COR⁵ʰ; R⁵ʰ is a hydroxyl radical or a branched or unbranched C₁₋₆ alkyl radical; R⁶ is a radical -C (O) R⁶ᵃ; an optionally substituted 5- or 6-membered heteroaryl ring containing at least one heteroatom selected from N, O, and S; R⁶ᵃ is a hydroxyl radical, a branched or unbranched C₁₋₆ alkoxy radical; a radical - (CH₂) ₜ-NR⁶ᵇR⁶ᶜ; a radical -OCH (CH₃) OC (O) CH (CH₃) ₂; or a radical -NR⁶ᵍ- (CH₂) ᵛCH (R⁶ᶠ) -NR⁶ᵉR⁶ᵈ; t is 1, 2, 3, 4, 5, or 6; v is 1, 2, 3, 4, 5, or 6; R⁶ᵇ, R⁶ᶜ, R⁶ᵈ, R⁶ᵉ, R⁶ᵍ are independently of one another a hydrogen atom; or a branched or unbranched C₁₋₆ alkyl radical; R⁶ᶠ is a hydrogen atom or a radical -COR⁶ʰ; R⁶ʰ is a hydroxyl radical or a branched or unbranched C₁₋₆ alkyl radical; or a pharmaceutically acceptable salt, isomer, prodrug, or solvate thereof.

ARP190103622A 2018-12-12 2019-12-11 PYRROLIDINE-2-CARBOXYL ACID DERIVATIVES TO TREAT PAIN AND PAIN-RELATED CONDITIONS AR116905A1 (en)

Applications Claiming Priority (1)

Application Number Priority Date Filing Date Title
EP18382915 2018-12-12

Publications (1)

Publication Number Publication Date
AR116905A1 true AR116905A1 (en) 2021-06-23

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ID=64746482

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Application Number Title Priority Date Filing Date
ARP190103622A AR116905A1 (en) 2018-12-12 2019-12-11 PYRROLIDINE-2-CARBOXYL ACID DERIVATIVES TO TREAT PAIN AND PAIN-RELATED CONDITIONS

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AR (1) AR116905A1 (en)
TW (1) TW202026281A (en)
WO (1) WO2020120539A1 (en)

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* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
AR112463A1 (en) * 2017-07-27 2019-10-30 Esteve Pharmaceuticals Sa PROPANAMINE DERIVATIVES TO TREAT PAIN AND PAIN RELATED STATES
CN115190815B (en) 2019-12-26 2024-06-18 吉尔伽美什制药公司 Arylcyclohexylamine derivatives and their use in the treatment of psychotic disorders
WO2021168082A1 (en) 2020-02-18 2021-08-26 Gilgamesh Pharmaceuticals, Inc. Specific tryptamines for use in the treatment of mood disorders
US12129234B1 (en) 2023-08-03 2024-10-29 Gilgamesh Pharmaceuticals, Inc. Crystalline salts of N-ethyl-(5-fluoro-1H-indol-3-yl)-N-methylethan-1-amine
US12157722B1 (en) 2023-08-03 2024-12-03 Gilgamesh Pharmaceuticals, Inc. Crystalline hydrochloride salts of N-ethyl-2-(5-fluoro-1H-indol-3-yl)-N-methylethan-1-amine

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GB0225379D0 (en) * 2002-10-31 2002-12-11 Pfizer Ltd Therapeutic proline derivatives
DE10252666A1 (en) * 2002-11-11 2004-08-05 Grünenthal GmbH N-piperidyl-cyclohexane derivatives
WO2004043900A2 (en) * 2002-11-12 2004-05-27 Grünenthal GmbH 4-alkyl/4-alkenyl/4-alkynyl methyl/-1-arylcyclohexylamine derivatives

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WO2020120539A1 (en) 2020-06-18

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