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NO860746L - THERMAL REFORM OF GAS HYDROCARBON. - Google Patents

THERMAL REFORM OF GAS HYDROCARBON.

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Publication number
NO860746L
NO860746L NO860746A NO860746A NO860746L NO 860746 L NO860746 L NO 860746L NO 860746 A NO860746 A NO 860746A NO 860746 A NO860746 A NO 860746A NO 860746 L NO860746 L NO 860746L
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Norway
Prior art keywords
gas
plasma generator
reforming
water vapor
outlet
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Application number
NO860746A
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Norwegian (no)
Inventor
Sven Santen
Lars Bentell
Bjoern Hammarskog
Original Assignee
Skf Steel Eng Ab
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Publication of NO860746L publication Critical patent/NO860746L/en

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    • BPERFORMING OPERATIONS; TRANSPORTING
    • B01PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01JCHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J12/00Chemical processes in general for reacting gaseous media with gaseous media; Apparatus specially adapted therefor
    • B01J12/002Chemical processes in general for reacting gaseous media with gaseous media; Apparatus specially adapted therefor carried out in the plasma state
    • CCHEMISTRY; METALLURGY
    • C01INORGANIC CHEMISTRY
    • C01BNON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B3/00Hydrogen; Gaseous mixtures containing hydrogen; Separation of hydrogen from mixtures containing it; Purification of hydrogen
    • C01B3/02Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen
    • C01B3/32Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air
    • C01B3/34Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents
    • C01B3/342Production of hydrogen or of gaseous mixtures containing a substantial proportion of hydrogen by reaction of gaseous or liquid organic compounds with gasifying agents, e.g. water, carbon dioxide, air by reaction of hydrocarbons with gasifying agents with the aid of electrical means, electromagnetic or mechanical vibrations, or particle radiations
    • BPERFORMING OPERATIONS; TRANSPORTING
    • B01PHYSICAL OR CHEMICAL PROCESSES OR APPARATUS IN GENERAL
    • B01JCHEMICAL OR PHYSICAL PROCESSES, e.g. CATALYSIS OR COLLOID CHEMISTRY; THEIR RELEVANT APPARATUS
    • B01J2219/00Chemical, physical or physico-chemical processes in general; Their relevant apparatus
    • B01J2219/08Processes employing the direct application of electric or wave energy, or particle radiation; Apparatus therefor
    • B01J2219/0894Processes carried out in the presence of a plasma
    • CCHEMISTRY; METALLURGY
    • C01INORGANIC CHEMISTRY
    • C01BNON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/02Processes for making hydrogen or synthesis gas
    • C01B2203/0205Processes for making hydrogen or synthesis gas containing a reforming step
    • C01B2203/0211Processes for making hydrogen or synthesis gas containing a reforming step containing a non-catalytic reforming step
    • C01B2203/0222Processes for making hydrogen or synthesis gas containing a reforming step containing a non-catalytic reforming step containing a non-catalytic carbon dioxide reforming step
    • CCHEMISTRY; METALLURGY
    • C01INORGANIC CHEMISTRY
    • C01BNON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/04Integrated processes for the production of hydrogen or synthesis gas containing a purification step for the hydrogen or the synthesis gas
    • C01B2203/0465Composition of the impurity
    • C01B2203/049Composition of the impurity the impurity being carbon
    • CCHEMISTRY; METALLURGY
    • C01INORGANIC CHEMISTRY
    • C01BNON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/08Methods of heating or cooling
    • C01B2203/0805Methods of heating the process for making hydrogen or synthesis gas
    • C01B2203/0861Methods of heating the process for making hydrogen or synthesis gas by plasma
    • CCHEMISTRY; METALLURGY
    • C01INORGANIC CHEMISTRY
    • C01BNON-METALLIC ELEMENTS; COMPOUNDS THEREOF; METALLOIDS OR COMPOUNDS THEREOF NOT COVERED BY SUBCLASS C01C
    • C01B2203/00Integrated processes for the production of hydrogen or synthesis gas
    • C01B2203/12Feeding the process for making hydrogen or synthesis gas
    • C01B2203/1276Mixing of different feed components

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  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Engineering & Computer Science (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • General Health & Medical Sciences (AREA)
  • Physics & Mathematics (AREA)
  • Health & Medical Sciences (AREA)
  • Combustion & Propulsion (AREA)
  • Electromagnetism (AREA)
  • Mechanical Engineering (AREA)
  • Toxicology (AREA)
  • Plasma & Fusion (AREA)
  • Inorganic Chemistry (AREA)
  • Hydrogen, Water And Hydrids (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
  • Catalysts (AREA)
  • Carbon And Carbon Compounds (AREA)
  • Physical Or Chemical Processes And Apparatus (AREA)

Description

Foreliggende oppfinnelse vedrører en fremgangsmåte ved fremstilling av en i det vesentlige CO + r^-inneholdende gass ved termisk reformering av gassformige hydrogenkarbon-er, foreksempel CH^, med vanndamp i tilnærmet støkiometr-isk forhold samt en anordning for gjennomførsel av fremgangsmåten i henhold til oppfinnelsen. The present invention relates to a method for the production of an essentially CO + r^-containing gas by thermal reforming of gaseous hydrocarbons, for example CH^, with water vapor in an approximately stoichiometric ratio as well as a device for carrying out the method according to the invention.

Reformering av gassformige hydrokarboner så som CH^ved fremstillingen av en CO + r^-inneholdende gass skjer i henhold til kjent teknikk ved katalytisk reformering ved temperaturer under ca. 1000°C. Ved fremstillingen av reduksjonsgass ved hjelp av en såkalt ett-trinnsreformering skjer reformeringen ved et tilnærmet støkiometrisk forhold mellom H^ O og C. Denne fremgangsmåte begunstiges av høy temperatur, men temperaturen begrenses av styrken til materialet i reformerrørene. Reforming of gaseous hydrocarbons such as CH^ in the production of a CO + r^-containing gas takes place according to known technology by catalytic reforming at temperatures below approx. 1000°C. In the production of reducing gas using a so-called one-stage reforming, the reforming takes place at an approximately stoichiometric ratio between H^O and C. This method is favored by high temperature, but the temperature is limited by the strength of the material in the reformer tubes.

En ulempe ved denne kjente fremgangsmåte er at katalysator-en er meget følsom for svovel, av hvilken hydrogenkarbon-ene må renses for svovel før reformeringen. A disadvantage of this known method is that the catalyst is very sensitive to sulphur, from which the hydrogen carbons must be purified of sulfur before the reforming.

Det er i og for seg allerede kjent at reformering av hydro-genkarboner kan skje uten katalysatorer ved temperaturer over 1200- 1300°C, men verken en egnet fremgangsmåte eller anordning for gjennomførsel av denne prosess er kjent. It is already known in and of itself that reforming of hydrocarbons can take place without catalysts at temperatures above 1200-1300°C, but neither a suitable method nor device for carrying out this process is known.

Hensikten med foreliggende oppfinnelse er således å frem-bringe en fremgangsmåte og en anordning for termisk reformering av hydrogenkarbon uten anvendelse av reformerrør og katalysatorer. The purpose of the present invention is thus to produce a method and a device for the thermal reforming of hydrogen carbon without the use of reformer tubes and catalysts.

Fremgangsmåten i henhold til oppfinnelsen kjennetegnes ved at gassformig hydrogenkarbon og vanndamp, separat eller i blanding og i tilnærmet støkiometriske forhold tilføres en reformeringsreaktor, og at gassen helt eller delvis oppvarmes med plasmagenerator, slik at gassblandingens temperatur overstiger 1200°C. The method according to the invention is characterized by the fact that gaseous hydrogen carbon and water vapour, separately or in a mixture and in approximately stoichiometric conditions, are supplied to a reforming reactor, and that the gas is fully or partially heated with a plasma generator, so that the temperature of the gas mixture exceeds 1200°C.

Foruten at tilførselen av ekstern energi ved hjelp av plasmageneratoren muliggjør den termiske reformering i henhold til oppfinnelsen, oppnås herved allerede fra be-gynnelsen et lavt innhold av CC^+ H20, ^vs-under 10% In addition to the fact that the supply of external energy by means of the plasma generator enables the thermal reforming according to the invention, a low content of CC^+ H20, ^vs-less than 10% is achieved from the start

i gassen.in the gas.

I henhold til en passende utføringsform av fremgangsmåten i henhold til oppfinnelsen bringes hydrokarbonene og/eller vanndampen til helt eller delvis å passere gjennom plasmageneratoren, mens resterende gass injiseres direkte i reaktoren. According to a suitable embodiment of the method according to the invention, the hydrocarbons and/or water vapor are made to pass completely or partially through the plasma generator, while the remaining gas is injected directly into the reactor.

Plasmageneratoren kan være utformet med to ringformige elektroder eller alternativt være av typen "transferred are " . The plasma generator can be designed with two annular electrodes or alternatively be of the "transferred are" type.

I henhold til en annen egnet utføringsform av fremgangsmåten i henhold til oppfinnelsen utnyttes varmetapet i fremgangsmåten og/eller den fysiske varmen i den genererte gassblanding i det minste delvis for fremstilling av den i prosessen anvendte vanndamp. According to another suitable embodiment of the method according to the invention, the heat loss in the method and/or the physical heat in the generated gas mixture is utilized at least partially for the production of the water vapor used in the process.

I henhold til en annen egnet utføringsform av fremgangsmåten i henhold til oppfinnelsen utnyttes den fysiske varmen i den genererte gassblanding i det minste delvis for avsvovling av den fremstilte gass. Herved kan avsvovlingen gjennomføres ved injisering av en svovelakseptor, som pulverforming kalksten eller dolomit, i reaktoren, hvoretter hoveddelen av svovelet avskilles med den forbrukte kalken i fast og/eller flytende form. According to another suitable embodiment of the method according to the invention, the physical heat in the generated gas mixture is utilized at least partially for desulfurization of the produced gas. Hereby, the desulphurization can be carried out by injecting a sulfur acceptor, such as pulverized limestone or dolomite, into the reactor, after which the main part of the sulfur is separated with the spent lime in solid and/or liquid form.

I henhold til en annen egnet utføringsform av fremgangsmåten i henhold til oppfinnelsen utnyttes den fysiske varmen i den genererte gassblanding i det minste delvis for karburering av den fremstilte gassen. Dette gjennomføres fortrinnsvis ved injisering av pulverformige reaktive karbonbærere, vanligvis koks, i reaktoren hvoretter til-bakeblivende aske avskilles i fast og/eller flytende form. Restinnholdet av CO^+ f^O kan herigjennom senkes ytterligere, teoretisk helt ned til 0%. According to another suitable embodiment of the method according to the invention, the physical heat in the generated gas mixture is utilized at least partially for carburizing the produced gas. This is preferably carried out by injecting powdered reactive carbon carriers, usually coke, into the reactor, after which remaining ash is separated in solid and/or liquid form. The residual content of CO^+ f^O can thereby be further lowered, theoretically down to 0%.

Det er i og for seg også tenkbart å gjennomføre svovelrens-ing og/eller karburering i separate reaktorer gjennom hvilke den varme, fremstilte gassen etter reformeringen. It is in and of itself also conceivable to carry out sulfur cleaning and/or carburisation in separate reactors through which the hot, produced gas after the reforming.

Oppfinnelsen gjennomføres således i en tom, varmeisolert reaktor i hvilken temperaturen overstiger 1200°C og fortrinnvis når opp til ca. 1300°C. Gassblandingens trykk i reaktoren tilpasses til gassens påtenkte anvendings -formål, for anvending som reduksjonsgass hensiktsmessig oppad til ca. 2-3 bar (a) og ved anvending som syntesegass vanligvis overstigende ca. 20 bar (a). Temperaturreguler-ingen av den fremstilte gassen skjer på for formålet hensiktsmessig måte, foreksempel ved varmeveksling og/eller avkjøling. The invention is thus carried out in an empty, heat-insulated reactor in which the temperature exceeds 1200°C and preferably reaches up to approx. 1300°C. The pressure of the gas mixture in the reactor is adapted to the intended use of the gas, for use as a reducing gas, suitably up to approx. 2-3 bar (a) and when used as synthesis gas usually exceeding approx. 20 bar (a). The temperature regulation of the produced gas takes place in a manner appropriate for the purpose, for example by heat exchange and/or cooling.

Anordningen for gjennomførsel av fremgangsmåten i henhold til oppfinnelsen omfatter minst et reaksjonskammer, minst en plasmagenerator for tilførsel av ekstern energi i reaksjonskammeret, tilførselsanordninger for hydrogenkarbon og vanndamp som skal oppvarmes med plasmageneratoren, gass-uttak samt uttak for slagg og aske. The device for carrying out the method according to the invention comprises at least one reaction chamber, at least one plasma generator for supplying external energy in the reaction chamber, supply devices for hydrogen carbon and water vapor to be heated with the plasma generator, gas outlet and outlet for slag and ash.

I henhold til en foretrukket utføringsform av anordningen omfatter denne foruten dette tilførselsanordninger for reaktive karbonbærere og svovelakseptorer. According to a preferred embodiment of the device, this also includes supply devices for reactive carbon carriers and sulfur acceptors.

Plasmageneratoren kan inneholde sylindriske elektroder mellom hvilke det dannes en elektrisk lysbue. Alternativt kan plasmageneratoren være av typen "transferred are". The plasma generator can contain cylindrical electrodes between which an electric arc is formed. Alternatively, the plasma generator can be of the "transferred are" type.

I henhold til en annen hensiktsmessig utførsel av anordningen i henhold til oppfinnelsen omfatter denne en vertikal stående, sylindrisk sjakt inndelt i soner for reformering respektivt karburering, eventuelt utformet med en forsmalning mellom sonene, og utstyrt med et utløp i sjakt ens bunn for flytende slagg, et i sjaktens nedre anordnet gassutløp, forbundet med en etterfølgende avskilningsanordning med et i dens nedre del anordnet utløp for fast slagg og ufordampet materiale og et i dens øvre del anordnet gassutløp. Tilførselsanordninger for reaktive karbonbærere og svovelakseptorer er anordnet på et eller flere steder i sjakten og i tilslutning til gassutløpet av sjakten. According to another suitable embodiment of the device according to the invention, this comprises a vertical standing, cylindrical shaft divided into zones for reforming or carburizing, possibly designed with a narrowing between the zones, and equipped with an outlet in the bottom of the shaft for liquid slag, a gas outlet arranged in the lower part of the shaft, connected to a subsequent separation device with an outlet arranged in its lower part for solid slag and unvaporized material and a gas outlet arranged in its upper part. Supply devices for reactive carbon carriers and sulfur acceptors are arranged in one or more places in the shaft and in connection with the gas outlet of the shaft.

I henhold til en annen egnet utføringsform av anordningen i henhold til oppfinnelsen er plasmageneratoren eller plasma-generatorene anordnet i toppen av den vertikale sjakten. According to another suitable embodiment of the device according to the invention, the plasma generator or plasma generators are arranged at the top of the vertical shaft.

I henhold til en annen passende utføringsform av anordningen i henhold til oppfinnelsen er avskilleranordningen utformet som en syklon for å lette avskilning av faste partikler. According to another suitable embodiment of the device according to the invention, the separator device is designed as a cyclone to facilitate the separation of solid particles.

I henhold til en annen egnet utføringsform av anordningen i henhold til oppfinnelsen inneholder denne en varmeutveksler i gassutløpet fra det vertikale sjaktet og/eller fra av-skil ler anordningen . According to another suitable embodiment of the device according to the invention, this contains a heat exchanger in the gas outlet from the vertical shaft and/or from the separator device.

Ytterligere trekk, fordeler og utføringsformer av oppfinnelsen vil fremgå av den følgende detaljerte beskrivelse i tilslutning til de vedlagte tegninger på hvilken figuren viser en prinsippskisse av en anordning for gjennomføring av den termiske reformering i henhold til oppfinnelsen. Further features, advantages and embodiments of the invention will be apparent from the following detailed description in connection with the attached drawings, in which the figure shows a schematic diagram of a device for carrying out the thermal reforming according to the invention.

Anordningen omfatter en vertikal sylindrisk sjakt 1 som rommer en reformeringssone 2 og en karbureringssone 3. De to sonene vises delvis adskilt av en forsmalning 4 men står i direkte forbindelse med hverandre. I sjaktens topp er det anordnet minst en plasmagenerator 5. Hydrokarbon kan injiseres helt eller delvis direkte i sjakten gjennom ledningen 6 alternativt innføres gjennom ledningen 7 i en blandeanordning 8. I den på tegningen viste utføringsform varmeveksles vannet med den genererte gass og vanndamp kan innføres i blandeanordningen gjennom ledningen 9 alternativt helt eller delvis injiseres i reformeringssonen gjennom ledningen 10. En gassblanding kan genereres i blandeanordningen 8, hvilken helt eller delvis gjennom ledningen 11 kan bringes til å passere plasmageneratoren 5 alternativt kan en del av gassblåndingen injiseres direkte i reformeringssonen gjennom ledningen 12. The device comprises a vertical cylindrical shaft 1 which accommodates a reforming zone 2 and a carburizing zone 3. The two zones are shown partially separated by a narrowing 4 but are in direct connection with each other. At the top of the shaft, at least one plasma generator 5 is arranged. Hydrocarbon can be injected directly into the shaft in whole or in part through line 6, alternatively introduced through line 7 into a mixing device 8. In the embodiment shown in the drawing, heat is exchanged between the water and the generated gas and water vapor can be introduced into the mixing device through the line 9 is alternatively fully or partially injected into the reforming zone through the line 10. A gas mixture can be generated in the mixing device 8, which can be made to pass the plasma generator 5 in whole or in part through the line 11 alternatively part of the gas mixture can be injected directly into the reforming zone through the line 12 .

Utførelsesformen muliggjør selv at kun hydrogenkarbon respektivt vanndamp tilføres gjennom plasmageneratoren via blandeanordningen 8. The embodiment itself makes it possible for only hydrogen carbon or water vapor to be supplied through the plasma generator via the mixing device 8.

Den under fordampningssone 2 liggende karbureringssone 3 står via en gassledning 13 i forbindelse med en avskille-anordning 14, hvorved det oppnås en tilstrekkelig lang opp-holdstid for karburering av gassen til ønsket restinnhold av r^O og CO^-Avskilleanordningen utgjøres fortrinnsvis av en syklon for å lette avskilning av partikkelformede forurensninger i gassen, så som slaggdråper og ufordampet materiale. The carburizing zone 3 below the evaporation zone 2 is connected via a gas line 13 to a separation device 14, whereby a sufficiently long residence time is achieved for carburizing the gas to the desired residual content of r^O and CO^ The separation device preferably consists of a cyclone to facilitate separation of particulate contaminants in the gas, such as slag droplets and unvaporized material.

Hoveddelen av slaggen fra fordampningssonen 2 avskilles ved et slaggutløp 15 i den sylindriske, fordampningssonen rom-mende sjakt 1. I det de i gassen medførte partikler avskilles ved slaggutløpet 16 av avskilleanordningens bunn. The main part of the slag from the evaporation zone 2 is separated by a slag outlet 15 in the cylindrical chamber containing the evaporation zone 1. In it the particles entrained in the gas are separated at the slag outlet 16 by the bottom of the separation device.

Gassledningen 13 utgjør funksjonsmessig en del av karbureringssonen 3. Lanser 17, 18, 19 for tilførsel av reaktive karbonbaerere og/eller svovelakseptorer er anordnet i fordampningssonen, karbureringssone og nevnte gassledning. Eventuelt kan også slaggdannere injiseres gjennom de nevnte lanser. The gas line 13 functionally forms part of the carburization zone 3. Lances 17, 18, 19 for supplying reactive carbon carriers and/or sulfur acceptors are arranged in the evaporation zone, carburization zone and said gas line. Optionally, slag formers can also be injected through the aforementioned lances.

I gassutløpet 20 fra avskilleanordningen 14 vises på tegningen en varmeutveksler 21, hvilken utnyttes for varmeut-veksling eller avkjøling av den genererte gass. Som nevnt ovenfor kan denne varmeutveksler fortrinnsvis utnyttes for generering av vanndamp for reformeringen. Nevnte varmeut- veksling eller avkjøling av den genererte gassblanding kan alternativt eller foruten dette skje i gassledningen 13 som forbinder karbureringssonen med avskilleanordningen. In the gas outlet 20 from the separation device 14, a heat exchanger 21 is shown in the drawing, which is used for heat exchange or cooling of the generated gas. As mentioned above, this heat exchanger can preferably be used for the generation of steam for the reforming. Said heat exchange or cooling of the generated gas mixture can alternatively or in addition take place in the gas line 13 which connects the carburizing zone with the separation device.

Claims (16)

1. Fremgangsmåte ved fremstilling av en i det hovedsaklige CO + r^ -holdig gass ved teknisk reformering av gassformige hydrokarboner, foreksempel CH^ , med vanndamp i tilnærmet støkiometrisk forhold, karakterisert ved at gassformig hydrokarbon og vanndamp, separat eller i blanding og i tilnærmet støkiometrisk forhold, tilføres en reformeringsreaktor, og at gassen helt eller delvis oppvarmes med plasmagenerator slik at gassblandingens temperatur overstiger 1200°C.1. Procedure for the production of a mainly CO + r^ -containing gas by technical reforming of gaseous hydrocarbons, for example CH^ , with water vapor in an approximately stoichiometric ratio, characterized in that gaseous hydrocarbon and water vapour, separately or in a mixture and in an approximately stoichiometric ratio, are supplied to a reforming reactor, and that the gas is fully or partially heated with a plasma generator so that the temperature of the gas mixture exceeds 1200°C. 2. Fremgangsmåte i henhold til krav 1, karakterisert ved at hydrokarbon og/eller vanndamp helt eller delvis bringes til å passere gjennom plasmageneratoren mens den resterende gass injiseres direkte i reaktoren.2. Method according to claim 1, characterized in that hydrocarbon and/or water vapor is completely or partially caused to pass through the plasma generator while the remaining gas is injected directly into the reactor. 3. Fremgangsmåte i henhold til krav 1-2, karakterisert ved at plasmageneratoren er utformet med to ringformige elektroder.3. Method according to claims 1-2, characterized in that the plasma generator is designed with two annular electrodes. 4. Fremgangsmåte i henhold til krav 1-2, karakterisert ved at plasmageneratoren er av typen "transferred are".4. Method according to claims 1-2, characterized in that the plasma generator is of the "transferred are" type. 5. Fremgangsmåte i henhold til krav 1-4, karakterisert ved at varmetapet i prosessen og/eller det fysiske varmeinnholdet i den genererte gassblanding i det minste delvis utnyttes for fremstilling av i prosessen anvendt vanndamp.5. Method according to claims 1-4, characterized in that the heat loss in the process and/or the physical heat content in the generated gas mixture is at least partially utilized for the production of water vapor used in the process. 6. Fremgangsmåte i henhold til krav 1-5, karakterisert ved at det fysiske varmeinnholdet i den genererte gassblanding i det minste delvis nyttes for avsvovling av den fremstilte gassen.6. Method according to claims 1-5, characterized in that the physical heat content in the generated gas mixture is at least partially used for desulfurization of the produced gas. 7. Fremgangsmåte i henhold til krav 6, karakterisert ved at avsvovlingen gjenn-omføres ved injisering av en sovelakseptor, som pulverform-ig kalksten eller dolomit, i reaktoren, hvoretter hoveddelen av svovelet adskilles sammen med den forbrukte kalken i fast og/eller flytende form.7. Procedure according to claim 6, characterized in that the desulphurisation is recycled by injecting a sleeper acceptor, such as powdered limestone or dolomite, into the reactor, after which the main part of the sulfur is separated together with the spent lime in solid and/or liquid form. 8. Fremgangsmåte i henhold til krav 1-7, karakterisert ved at det fysiske varmeinnholdet i den genererte gassblanding i det minste delvis utnyttes for karborering av den fremstilte gassen.8. Method according to claims 1-7, characterized in that the physical heat content in the generated gas mixture is at least partially utilized for carburizing the produced gas. 9. Fremgangsmåte i henhold til krav 8, karakterisert ved at karbureringen ut-føres ved injisering av pulverformige reaktive karbonbærere, fortrinnsvis koks, i reaktoren, hvoretter tilbake-blivende aske adskilles i fast og/eller flytende form.9. Method according to claim 8, characterized in that the carburization is carried out by injecting powdered reactive carbon carriers, preferably coke, into the reactor, after which residual ash is separated in solid and/or liquid form. 10. Fremgangsmåte i henhold til krav 9, karakterisert ved at karburering av gass-blandingen skjer ned til et restinnhold av CO,, + H^ O som ligger under 10%.10. Method according to claim 9, characterized in that carburization of the gas mixture takes place down to a residual content of CO,, + H^O which is below 10%. 11. Anordning for fremstilling av en hovedsaklig CO + H^ -holdig gass ved teknisk reformering av gassformige hydrokarboner, foreksempel CH^ med vanndamp i tilnærmet støkiometrisk forhold for gjennomførsel av fremgangsmåten i henhold til krav 1, karakterisert ved at den omfatter minst et reaksjonskammer, minst en plasmagenerator (5) for til-fø rsel av ekstern energi i reaksjonskammeret, tilførsels-anordninger for hydrokarboner og vanndamp som skal oppvarmes med plasmagenerator samt utløp (15, 16) for slagg og aske.11. Device for the production of a mainly CO + H^ -containing gas by technical reforming of gaseous hydrocarbons, for example CH^ with water vapor in an approximately stoichiometric ratio for carrying out the method according to claim 1, characterized in that it comprises at least one reaction chamber, at least one plasma generator (5) for the supply of external energy in the reaction chamber, supply devices for hydrocarbons and water vapor to be heated with a plasma generator and outlets (15, 16) for slag and ash. 12. Anordning i henhold til krav 11, karakterisert ved at tilfø rselsanordning-er (17, 18, 19) for reaktive karbonbærere og/eller svovelakseptorer.12. Device according to claim 11, characterized in that supply devices (17, 18, 19) are for reactive carbon carriers and/or sulfur acceptors. 13. Anordning i henhold til krav 11 - 12, karakterisert ved at den omfatter en vertikal stående sylindrisk sjakt (1) inndelt i soner for reformering (2) respektive karburering (3), eventuelt utformet med en forsmalning (4) mellom sonene, og utstyrt med utløp (15) i sjaktens bunn for flytende slagg, et i sjaktens nedre del anordnet gassutløp (13) forbundet med en etterfølgende avskilningsanordning (14) med et i dens nedre del anordnet utløp (16) for fast slagg og ufordampet materiale og et i dets øvre del anordnet gassutløp (20).13. Device according to claims 11 - 12, characterized in that it comprises a vertical standing cylindrical shaft (1) divided into zones for reforming (2) and carburizing (3), possibly designed with a narrowing (4) between the zones, and equipped with an outlet (15) in the bottom of the shaft for liquid slag, a gas outlet (13) arranged in the lower part of the shaft connected to a subsequent separation device (14) with an outlet (16) arranged in its lower part for solid slag and unvaporized material and a in its upper part arranged gas outlet (20). 14. Anordning i henhold til krav 11 - 13, karakterisert ved at plasmageneratoren eller generatorene (5) er anordnet i toppen av den vertikale sjakten (1) .14. Device according to claims 11 - 13, characterized in that the plasma generator or generators (5) are arranged at the top of the vertical shaft (1). 15. Anordning i henhold til krav 11 - 14, karakterisert ved at avskilningsanordn-ingen (14) er utformet som en syklon.15. Device according to claims 11 - 14, characterized in that the separation device (14) is designed as a cyclone. 16. Anordning i henhold til krav 11 - 15, karakterisert ved at den omfatter en varmeutveksler (21) i gassutlø pet (13) fra den vertikale sjakten (1) og/eller i gassutlø pet (20) fra avskilleanordningen (14 ) .16. Device according to claims 11 - 15, characterized in that it comprises a heat exchanger (21) in the gas outlet (13) from the vertical shaft (1) and/or in the gas outlet (20) from the separation device (14).
NO860746A 1985-03-01 1986-02-28 THERMAL REFORM OF GAS HYDROCARBON. NO860746L (en)

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CN86101235A (en) 1986-10-01
SE8501005D0 (en) 1985-03-01
FR2578237B1 (en) 1990-07-13
DE3606108A1 (en) 1986-09-04
GB2172011B (en) 1989-06-14
NL8600429A (en) 1986-10-01
SE8501005L (en) 1986-09-02
GB8604844D0 (en) 1986-04-03
FR2578237A1 (en) 1986-09-05
AU5400886A (en) 1986-09-04
GB2172011A (en) 1986-09-10

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