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NL216658A - - Google Patents

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Publication number
NL216658A
NL216658A NL216658DA NL216658A NL 216658 A NL216658 A NL 216658A NL 216658D A NL216658D A NL 216658DA NL 216658 A NL216658 A NL 216658A
Authority
NL
Netherlands
Prior art keywords
component
compounds
organic
alloys
olefines
Prior art date
Application number
Inventor
Oskar E H Klopfer
Jr Oliver W Burke
Original Assignee
Oliver Wallis Burke Jr
Priority date (The priority date is an assumption and is not a legal conclusion. Google has not performed a legal analysis and makes no representation as to the accuracy of the date listed.)
Publication date
Publication of NL216658A publication Critical patent/NL216658A/xx
Priority claimed from US641047A external-priority patent/US3196116A/en

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Classifications

    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F10/00Homopolymers and copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07FACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
    • C07F1/00Compounds containing elements of Groups 1 or 11 of the Periodic Table
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07FACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
    • C07F1/00Compounds containing elements of Groups 1 or 11 of the Periodic Table
    • C07F1/02Lithium compounds
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07FACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
    • C07F1/00Compounds containing elements of Groups 1 or 11 of the Periodic Table
    • C07F1/08Copper compounds
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07FACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
    • C07F3/00Compounds containing elements of Groups 2 or 12 of the Periodic Table
    • CCHEMISTRY; METALLURGY
    • C07ORGANIC CHEMISTRY
    • C07FACYCLIC, CARBOCYCLIC OR HETEROCYCLIC COMPOUNDS CONTAINING ELEMENTS OTHER THAN CARBON, HYDROGEN, HALOGEN, OXYGEN, NITROGEN, SULFUR, SELENIUM OR TELLURIUM
    • C07F5/00Compounds containing elements of Groups 3 or 13 of the Periodic Table
    • C07F5/06Aluminium compounds
    • C07F5/061Aluminium compounds with C-aluminium linkage
    • C07F5/062Al linked exclusively to C
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F10/00Homopolymers and copolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond
    • C08F10/04Monomers containing three or four carbon atoms
    • C08F10/06Propene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F114/00Homopolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen
    • C08F114/02Monomers containing chlorine
    • C08F114/04Monomers containing two carbon atoms
    • C08F114/06Vinyl chloride
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F114/00Homopolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by a halogen
    • C08F114/18Monomers containing fluorine
    • C08F114/26Tetrafluoroethene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F12/00Homopolymers and copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring
    • C08F12/02Monomers containing only one unsaturated aliphatic radical
    • C08F12/04Monomers containing only one unsaturated aliphatic radical containing one ring
    • C08F12/06Hydrocarbons
    • C08F12/08Styrene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F12/00Homopolymers and copolymers of compounds having one or more unsaturated aliphatic radicals, each having only one carbon-to-carbon double bond, and at least one being terminated by an aromatic carbocyclic ring
    • C08F12/02Monomers containing only one unsaturated aliphatic radical
    • C08F12/04Monomers containing only one unsaturated aliphatic radical containing one ring
    • C08F12/14Monomers containing only one unsaturated aliphatic radical containing one ring substituted by hetero atoms or groups containing heteroatoms
    • C08F12/16Halogens
    • C08F12/18Chlorine
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F36/00Homopolymers and copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds
    • C08F36/02Homopolymers and copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds the radical having only two carbon-to-carbon double bonds
    • C08F36/04Homopolymers and copolymers of compounds having one or more unsaturated aliphatic radicals, at least one having two or more carbon-to-carbon double bonds the radical having only two carbon-to-carbon double bonds conjugated
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F4/00Polymerisation catalysts
    • C08F4/06Metallic compounds other than hydrides and other than metallo-organic compounds; Boron halide or aluminium halide complexes with organic compounds containing oxygen
    • C08F4/12Metallic compounds other than hydrides and other than metallo-organic compounds; Boron halide or aluminium halide complexes with organic compounds containing oxygen of boron, aluminium, gallium, indium, thallium or rare earths
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F8/00Chemical modification by after-treatment
    • C08F8/42Introducing metal atoms or metal-containing groups
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F110/00Homopolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond
    • C08F110/02Ethene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F110/00Homopolymers of unsaturated aliphatic hydrocarbons having only one carbon-to-carbon double bond
    • C08F110/04Monomers containing three or four carbon atoms
    • C08F110/06Propene
    • CCHEMISTRY; METALLURGY
    • C08ORGANIC MACROMOLECULAR COMPOUNDS; THEIR PREPARATION OR CHEMICAL WORKING-UP; COMPOSITIONS BASED THEREON
    • C08FMACROMOLECULAR COMPOUNDS OBTAINED BY REACTIONS ONLY INVOLVING CARBON-TO-CARBON UNSATURATED BONDS
    • C08F2410/00Features related to the catalyst preparation, the catalyst use or to the deactivation of the catalyst
    • C08F2410/04Dual catalyst, i.e. use of two different catalysts, where none of the catalysts is a metallocene

Landscapes

  • Chemical & Material Sciences (AREA)
  • Organic Chemistry (AREA)
  • Health & Medical Sciences (AREA)
  • Chemical Kinetics & Catalysis (AREA)
  • Medicinal Chemistry (AREA)
  • Polymers & Plastics (AREA)
  • Engineering & Computer Science (AREA)
  • Materials Engineering (AREA)
  • General Chemical & Material Sciences (AREA)
  • Transition And Organic Metals Composition Catalysts For Addition Polymerization (AREA)
  • Organic Low-Molecular-Weight Compounds And Preparation Thereof (AREA)
  • Addition Polymer Or Copolymer, Post-Treatments, Or Chemical Modifications (AREA)

Abstract

A polymerization catalyst comprises a monometatalled organic compound "1" and Friedel Crafts compounds "2b" with or without a modifying polar compound "2a" and/or a carrier component "3". Component "1" is defined as containing a single metal atom bonded to the organic moiety by a carbon-metal bond; said moiety may be polymeric or nonpolymeric, while the metal atoms are selected from Li, Na, K, Rb, Cs, Cu, Ag, Be, Mg, Ca, Sr, Ba, Zn, Cd, Hg, B, Al, Sc, Yb, La, Ga, In, Tl, Ti, Zr, Th, Ge, Sn, Pb and the rare-earth metals. Component "2b" comprises mixed halides obtained by burning in halogen gases or vapours the ferro-alloys of metals of Periodic Group IV, V, VI, iron group VIII, and Mn, with or without reductive after treatment with metal powders, metal hydrides, metal carbides and/or hydrogen and the said halides may be partially reacted with oxygen water and/or reactive organic compounds such as alcohols. Component "2a" consists of organic donor compounds containing one or more of O, N, S, Se, Te, halogens; various classes of such compounds being mentioned and a number of peroxides and azo compounds being also specified; such donor compounds include those in which active hydrogen atoms have been replaced by metals. Component "3" is an organic or inorganic solid not detrimental to the polymerization and including shaped materials and carbon. Many metals and acid radicals suitable as constituents of this component are listed as are many specified oxides. The usual hydrocarbons and their halogenated derivatives are mentioned as solvents for catalyst formation and polymerization. In examples, ethylene and propylene are homopolymerized in presence of catalysts containing components selected from the following: "1": amyl barium, amyl sodium, p-xylene monosodium and a -methylstyrene trimer monosodium; "2a": ethyl ether; "2b" chlorides derived from Fe alloys with V, Mo, W or Cb; "3": NaCl. Also specified as alloys from which "2b" can be derived are Fe-Mn and Fe-Cr. The monomers which in general may be polymerized with the above catalyst contain at least one polymerizable ethylenic and/or acetylenic linkage; the monomer may itself form the diluent as an alternative to using a separate diluent. Numerous monomers are listed in the Specification; these include the following types: a -olefines; chloro-, fluoro-, chlorofluoro- and bromo-olefines including chloro- and bromo-aryl and alkaryl olefines; aryl and alkaryl olefines; conjugated dienes and trienes. Specifications 873,616 and 873,658 are referred to.ALSO:A polymerization catalyst comprises a mono-metallated organic compound "1" and Friedel Crafts compounds "2b" with or without a modifying polar compound "2a" and/or a carrier component "3". Component "1" is defined as containing a single metal atom bonded to the organic moiety by a carbon-metal bond; said moiety may be polymeric or non-polymeric, while the metal atom is selected from Li, Na, K, Rb, Cs, Cu, Ag, Be, Mg, Ca, Sr, Ba, Zn, Cd, Hg, B, Al, Sc, Yb, La, Ga, In, Tl, Ti, Zr, Th, Ge, Sn, Pb and the rare-earth metals. Component "2b" comprises mixed halides obtained by burning in halogen gases or vapours the ferro-alloys of metals of Periodic Group IV, V, VI, iron Group VIII, and Mn, with or without reductive after treatment with metal powders, metal hydrides, metal carbides and/or hydrogen and the said halides may be partially reacted with oxygen water and/or reactive organic compounds such as alcohols. Component "2a" consists of organic donor compounds containing one or more of O, N, S, Se, Te, halogens; various classes of such compounds being mentioned and a number of peroxides and azo-compounds being also specified; such donor compounds include those in which active hydrogen atoms have been replaced by metals. Component "3" is an organic or inorganic solid not detrimental to the polymerization and including shaped materials and carbon. Many metals and acid radicals suitable as constituents of this component are listed as are many specified oxides. The usual hydrocarbons and their halogenated derivatives are mentioned as solvents for catalyst formation and polymerization. In examples, ethylene and propylene are homopolymerized in presence of catalysts containing components selected from the following:-"1": amyl barium, amyl sodium, p-xylene monosodium and a -methylstyrene trimer monosodium; "2a": ethyl ether; "2b": chlorides derived from Fe alloys with V, Mo, W or Cb; "3": NaCl. Also specified as alloys from which "2b" can be derived are Fe-Mn and Fe-Cr. The monomers which in general may be polymerized with the above catalyst contain at least one polymerizable ethylenic and/or acetylonic linkage; the monomer may itself form the diluent as an alternative to using a separate diluent. Numerous monomers are listed in the Specification; these include the following types:-a -olefines; chloro, fluoro, chlorofluoro and bromo olefines including chloro and bromo aryl and alkaryl olefines; aryl and alkaryl olefins; conjugated dienes and trienes. Specifications 873,616 and 873,658 also are referred to.ALSO:The Specification describes analyses of certain ferro-alloys thus:- (1) Fe-W: W 81.02, Mn 0.13, Mo 0.70, C 0.51, Si 0.17; (2) Fe-V: V 62.0; (3) Fe-Mn: Mn 78.6, C 6.38, Si 1.38; (4) Fe-Mo: Mo 62.6, Si 0.56; (5) Fe-Cr: Cr 71.23, C 0.4, Si 0.57; (6) Fe-Cb: Cb 57.36, C 0.35, Si 6.47%. In all cases, iron constitutes the approximate balance. Specifications 873,658 and 873,616 also are referred to.
NL216658D 1956-04-25 NL216658A (en)

Applications Claiming Priority (2)

Application Number Priority Date Filing Date Title
US58064256A 1956-04-25 1956-04-25
US641047A US3196116A (en) 1956-04-25 1957-02-19 Multiply metallated polymerization catalysts

Publications (1)

Publication Number Publication Date
NL216658A true NL216658A (en) 1900-01-01

Family

ID=27078095

Family Applications (1)

Application Number Title Priority Date Filing Date
NL216658D NL216658A (en) 1956-04-25

Country Status (5)

Country Link
BE (1) BE556975A (en)
DE (3) DE1158067B (en)
FR (1) FR1187677A (en)
GB (4) GB873657A (en)
NL (1) NL216658A (en)

Families Citing this family (2)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
NL265477A (en) * 1961-03-10
CN114656628B (en) * 2022-03-28 2023-11-17 浙江皇马科技股份有限公司 High molecular weight allyl alcohol polyoxyethylene polyoxypropylene ether and preparation method thereof

Family Cites Families (3)

* Cited by examiner, † Cited by third party
Publication number Priority date Publication date Assignee Title
DE538782C (en) * 1931-11-16 Patra Patent Treuhand Electric arc lamp with a series resistor serving as a light body
US1938180A (en) * 1931-06-23 1933-12-05 Shell Dev Process for the manufacture of organic metallo compounds
DE1003731B (en) 1955-02-25 1957-03-07 Basf Ag Process for the stabilization of organosodium compounds

Also Published As

Publication number Publication date
GB873661A (en) 1961-07-26
DE1172429B (en) 1964-06-18
DE1158067B (en) 1963-11-28
FR1187677A (en) 1959-09-15
DE1168428B (en) 1964-04-23
GB873662A (en) 1961-07-26
BE556975A (en) 1957-10-25
GB873657A (en) 1961-07-26
GB873660A (en) 1961-07-26

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